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System analysis of pulping process coupled with supercritical water gasification of black liquor for combined hydrogen, heat and power production

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  • Cao, Changqing
  • Guo, Liejin
  • Jin, Hui
  • Cao, Wen
  • Jia, Yi
  • Yao, Xiangdong

Abstract

Supercritical water gasification is an innovative black liquor treatment method for hydrogen production. In the present study, an integrated system of pulping and SCWG of black liquor was simulated. Combined hydrogen, power, MP and LP steam are produced for pulping process. The gas product after H2 extraction was burned with imported natural gas to supply more heat. For a reference pulp mill producing 1000 ADt pulp/day, potentially 37126 Nm3/h hydrogen can be produced. The generated MP and LP steam can fully meet the requirement of pulping process. Using air as oxidant in gas combustion is more energy-efficient than using oxygen for being free of oxygen production process. In the case of using air, 22604 kW power can be exported after balancing the consumptions and 219 kgce energy can be produced with 1t pulp production. While using oxygen, 10723 kW power needs be imported and 288 kgce energy can be consumed to produce 1t pulp. However, using air as oxidant may bring N2 and NOx in the exhaust gas, posing a challenge to the subsequent processing. Scaling-up of the system improved the energy efficiency, but the influence is very small when the capacity is above 250ADt/day.

Suggested Citation

  • Cao, Changqing & Guo, Liejin & Jin, Hui & Cao, Wen & Jia, Yi & Yao, Xiangdong, 2017. "System analysis of pulping process coupled with supercritical water gasification of black liquor for combined hydrogen, heat and power production," Energy, Elsevier, vol. 132(C), pages 238-247.
    • Handle: RePEc:eee:energy:v:132:y:2017:i:c:p:238-247
    DOI: 10.1016/j.energy.2017.05.104
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    11. Wang, Cui & Jin, Hui & Peng, Pai & Chen, Jia, 2019. "Thermodynamics and LCA analysis of biomass supercritical water gasification system using external recycle of liquid residual," Renewable Energy, Elsevier, vol. 141(C), pages 1117-1126.
    12. Guo, Shenghui & Wang, Yu & Shang, Fei & Yi, Lei & Chen, Yunan & Chen, Bin & Guo, Liejin, 2023. "Thermodynamic analysis of the series system for the supercritical water gasification of coal-water slurry," Energy, Elsevier, vol. 283(C).
    13. Magdeldin, Mohamed & Järvinen, Mika, 2020. "Supercritical water gasification of Kraft black liquor: Process design, analysis, pulp mill integration and economic evaluation," Applied Energy, Elsevier, vol. 262(C).
    14. Chen, Zhewen & Gao, Lin & Zhang, Xiaosong & Han, Wei & Li, Sheng, 2018. "High-efficiency power generation system with integrated supercritical water gasification of coal," Energy, Elsevier, vol. 159(C), pages 810-816.
    15. Wang, Yu & Ren, Changyifan & Guo, Shenghui & Liu, Shi & Du, Mingming & Chen, Yunan & Guo, Liejin, 2023. "Thermodynamic and environmental analysis of heat supply in pig manure supercritical water gasification system," Energy, Elsevier, vol. 263(PA).
    16. Özdenkçi, Karhan & Prestipino, Mauro & Björklund-Sänkiaho, Margareta & Galvagno, Antonio & De Blasio, Cataldo, 2020. "Alternative energy valorization routes of black liquor by stepwise supercritical water gasification: Effect of process parameters on hydrogen yield and energy efficiency," Renewable and Sustainable Energy Reviews, Elsevier, vol. 134(C).
    17. Kumar, Vineet & Malyan, Sandeep Kumar & Apollon, Wilgince & Verma, Pradeep, 2024. "Valorization of pulp and paper industry waste streams into bioenergy and value-added products: An integrated biorefinery approach," Renewable Energy, Elsevier, vol. 228(C).
    18. Qi, Xingang & Li, Xujun & Liu, Fan & Lu, Libo & Jin, Hui & Wei, Wenwen & Chen, Yunan & Guo, Liejin, 2023. "Hydrogen production by kraft black liquor supercritical water gasification: Reaction pathway and kinetic," Energy, Elsevier, vol. 282(C).
    19. Darmawan, Arif & Ajiwibowo, Muhammad W. & Biddinika, Muhammad Kunta & Tokimatsu, Koji & Aziz, Muhammad, 2019. "Black liquor-based hydrogen and power co-production: Combination of supercritical water gasification and syngas chemical looping," Applied Energy, Elsevier, vol. 252(C), pages 1-1.

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