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Synthetic gas production from dry black liquor gasification process using direct causticization with CO2 capture

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  • Naqvi, Muhammad
  • Yan, Jinyue
  • Dahlquist, Erik

Abstract

Synthetic natural gas (SNG) production from dry black liquor gasification (DBLG) system is an attractive option to reduce CO2 emissions replacing natural gas. This article evaluates the energy conversion performance of SNG production from oxygen blown circulating fluidized bed (CFB) black liquor gasification process with direct causticization by investigating system integration with a reference pulp mill producing 1000 air dried tonnes (ADt) of pulp per day. The direct causticization process eliminates use of energy intensive lime kiln that is a main component required in the conventional black liquor recovery cycle with the recovery boiler. The paper has estimated SNG production potential, the process energy ratio of black liquor (BL) conversion to SNG, and quantified the potential CO2 abatement. Based on reference pulp mill capacity, the results indicate a large potential of SNG production (about 162MW) from black liquor but at a cost of additional biomass import (36.7MW) to compensate the total energy deficit. The process shows cold gas energy efficiency of about 58% considering black liquor and biomass import as major energy inputs. About 700ktonnes per year of CO2 abatement i.e. both possible CO2 capture and CO2 offset from bio-fuel use replacing natural gas, is estimated. Moreover, the SNG production offers a significant fuel replacement in transport sector especially in countries with large pulp and paper industry e.g. in Sweden, about 72% of motor gasoline and 40% of total motor fuel could be replaced.

Suggested Citation

  • Naqvi, Muhammad & Yan, Jinyue & Dahlquist, Erik, 2012. "Synthetic gas production from dry black liquor gasification process using direct causticization with CO2 capture," Applied Energy, Elsevier, vol. 97(C), pages 49-55.
    • Handle: RePEc:eee:appene:v:97:y:2012:i:c:p:49-55
    DOI: 10.1016/j.apenergy.2011.11.082
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    References listed on IDEAS

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    1. Möllersten, Kenneth & Gao, Lin & Yan, Jinyue & Obersteiner, Michael, 2004. "Efficient energy systems with CO2 capture and storage from renewable biomass in pulp and paper mills," Renewable Energy, Elsevier, vol. 29(9), pages 1583-1598.
    2. Andersson, E. & Harvey, S., 2006. "System analysis of hydrogen production from gasified black liquor," Energy, Elsevier, vol. 31(15), pages 3426-3434.
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    Cited by:

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    5. Ganesan, T. & Elamvazuthi, I. & Ku Shaari, Ku Zilati & Vasant, P., 2013. "Swarm intelligence and gravitational search algorithm for multi-objective optimization of synthesis gas production," Applied Energy, Elsevier, vol. 103(C), pages 368-374.
    6. Naqvi, Muhammad & Yan, Jinyue & Dahlquist, Erik, 2013. "System analysis of dry black liquor gasification based synthetic gas production comparing oxygen and air blown gasification systems," Applied Energy, Elsevier, vol. 112(C), pages 1275-1282.
    7. Nong, Guangzai & Huang, Lijie & Mo, Haitao & Wang, Shuangfei, 2013. "Investigate the variability of gas compositions and thermal efficiency of bagasse black liquor gasification," Energy, Elsevier, vol. 49(C), pages 178-181.
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    9. Xu, Z.R. & Zhu, W. & Li, M. & Zhang, H.W. & Gong, M., 2013. "Quantitative analysis of polycyclic aromatic hydrocarbons in solid residues from supercritical water gasification of wet sewage sludge," Applied Energy, Elsevier, vol. 102(C), pages 476-483.
    10. Yi, Qun & Wu, Guo-sheng & Gong, Min-hui & Huang, Yi & Feng, Jie & Hao, Yan-hong & Li, Wen-ying, 2017. "A feasibility study for CO2 recycle assistance with coke oven gas to synthetic natural gas," Applied Energy, Elsevier, vol. 193(C), pages 149-161.
    11. Ribeiro Domingos, Meire Ellen Gorete & Flórez-Orrego, Daniel & dos Santos, Moisés Teles & de Oliveira Junior, Silvio & Maréchal, François, 2023. "Process modeling and integration of hydrogen and synthetic natural gas production in a kraft pulp mill via black liquor gasification," Renewable Energy, Elsevier, vol. 219(P1).
    12. Darmawan, Arif & Hardi, Flabianus & Yoshikawa, Kunio & Aziz, Muhammad & Tokimatsu, Koji, 2017. "Enhanced process integration of black liquor evaporation, gasification, and combined cycle," Applied Energy, Elsevier, vol. 204(C), pages 1035-1042.
    13. Haro, Pedro & Aracil, Cristina & Vidal-Barrero, Fernando & Ollero, Pedro, 2015. "Rewarding of extra-avoided GHG emissions in thermochemical biorefineries incorporating Bio-CCS," Applied Energy, Elsevier, vol. 157(C), pages 255-266.
    14. Carminati, Hudson Bolsoni & Milão, Raquel de Freitas D. & de Medeiros, José Luiz & Araújo, Ofélia de Queiroz F., 2019. "Bioenergy and full carbon dioxide sinking in sugarcane-biorefinery with post-combustion capture and storage: Techno-economic feasibility," Applied Energy, Elsevier, vol. 254(C).
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