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Synthetic gas production from dry black liquor gasification process using direct causticization with CO2 capture

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  • Naqvi, Muhammad
  • Yan, Jinyue
  • Dahlquist, Erik

Abstract

Synthetic natural gas (SNG) production from dry black liquor gasification (DBLG) system is an attractive option to reduce CO2 emissions replacing natural gas. This article evaluates the energy conversion performance of SNG production from oxygen blown circulating fluidized bed (CFB) black liquor gasification process with direct causticization by investigating system integration with a reference pulp mill producing 1000 air dried tonnes (ADt) of pulp per day. The direct causticization process eliminates use of energy intensive lime kiln that is a main component required in the conventional black liquor recovery cycle with the recovery boiler. The paper has estimated SNG production potential, the process energy ratio of black liquor (BL) conversion to SNG, and quantified the potential CO2 abatement. Based on reference pulp mill capacity, the results indicate a large potential of SNG production (about 162MW) from black liquor but at a cost of additional biomass import (36.7MW) to compensate the total energy deficit. The process shows cold gas energy efficiency of about 58% considering black liquor and biomass import as major energy inputs. About 700ktonnes per year of CO2 abatement i.e. both possible CO2 capture and CO2 offset from bio-fuel use replacing natural gas, is estimated. Moreover, the SNG production offers a significant fuel replacement in transport sector especially in countries with large pulp and paper industry e.g. in Sweden, about 72% of motor gasoline and 40% of total motor fuel could be replaced.

Suggested Citation

  • Naqvi, Muhammad & Yan, Jinyue & Dahlquist, Erik, 2012. "Synthetic gas production from dry black liquor gasification process using direct causticization with CO2 capture," Applied Energy, Elsevier, vol. 97(C), pages 49-55.
    • Handle: RePEc:eee:appene:v:97:y:2012:i:c:p:49-55
    DOI: 10.1016/j.apenergy.2011.11.082
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    References listed on IDEAS

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    1. Andersson, E. & Harvey, S., 2006. "System analysis of hydrogen production from gasified black liquor," Energy, Elsevier, vol. 31(15), pages 3426-3434.
    2. Möllersten, Kenneth & Gao, Lin & Yan, Jinyue & Obersteiner, Michael, 2004. "Efficient energy systems with CO2 capture and storage from renewable biomass in pulp and paper mills," Renewable Energy, Elsevier, vol. 29(9), pages 1583-1598.
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    Cited by:

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    3. Darmawan, Arif & Hardi, Flabianus & Yoshikawa, Kunio & Aziz, Muhammad & Tokimatsu, Koji, 2017. "Enhanced process integration of black liquor evaporation, gasification, and combined cycle," Applied Energy, Elsevier, vol. 204(C), pages 1035-1042.
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    8. Cao, Changqing & Guo, Liejin & Jin, Hui & Cao, Wen & Jia, Yi & Yao, Xiangdong, 2017. "System analysis of pulping process coupled with supercritical water gasification of black liquor for combined hydrogen, heat and power production," Energy, Elsevier, vol. 132(C), pages 238-247.
    9. Zhang, Yuming & Yao, Meiqin & Gao, Shiqiu & Sun, Guogang & Xu, Guangwen, 2015. "Reactivity and kinetics for steam gasification of petroleum coke blended with black liquor in a micro fluidized bed," Applied Energy, Elsevier, vol. 160(C), pages 820-828.
    10. Darmawan, Arif & Ajiwibowo, Muhammad W. & Yoshikawa, Kunio & Aziz, Muhammad & Tokimatsu, Koji, 2018. "Energy-efficient recovery of black liquor through gasification and syngas chemical looping," Applied Energy, Elsevier, vol. 219(C), pages 290-298.
    11. Chaiwatanodom, Paphonwit & Vivanpatarakij, Supawat & Assabumrungrat, Suttichai, 2014. "Thermodynamic analysis of biomass gasification with CO2 recycle for synthesis gas production," Applied Energy, Elsevier, vol. 114(C), pages 10-17.
    12. Ganesan, T. & Elamvazuthi, I. & Ku Shaari, Ku Zilati & Vasant, P., 2013. "Swarm intelligence and gravitational search algorithm for multi-objective optimization of synthesis gas production," Applied Energy, Elsevier, vol. 103(C), pages 368-374.
    13. Naqvi, Muhammad & Yan, Jinyue & Dahlquist, Erik, 2013. "System analysis of dry black liquor gasification based synthetic gas production comparing oxygen and air blown gasification systems," Applied Energy, Elsevier, vol. 112(C), pages 1275-1282.
    14. Nong, Guangzai & Huang, Lijie & Mo, Haitao & Wang, Shuangfei, 2013. "Investigate the variability of gas compositions and thermal efficiency of bagasse black liquor gasification," Energy, Elsevier, vol. 49(C), pages 178-181.
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    17. Ribeiro Domingos, Meire Ellen Gorete & Flórez-Orrego, Daniel & dos Santos, Moisés Teles & de Oliveira Junior, Silvio & Maréchal, François, 2023. "Process modeling and integration of hydrogen and synthetic natural gas production in a kraft pulp mill via black liquor gasification," Renewable Energy, Elsevier, vol. 219(P1).

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