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Performance evaluation of an air-breathing high-temperature proton exchange membrane fuel cell

Author

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  • Wu, Qixing
  • Li, Haiyang
  • Yuan, Wenxiang
  • Luo, Zhongkuan
  • Wang, Fang
  • Sun, Hongyuan
  • Zhao, Xuxin
  • Fu, Huide

Abstract

The air-breathing proton exchange membrane fuel cell (PEMFC) is of great interest in mobile power sources because of its simple system design and low parasitic power consumption. Different from previous low-temperature air-breathing PEMFCs, a high-temperature PEMFC with a phosphoric acid doped polybenzimidazole (PBI) membrane as the polymer electrolyte is designed and investigated under air-breathing conditions. The preliminary results show that a peak power density of 220.5mWcm−2 at 200°C can be achieved without employing any water managements, which is comparable to those with conventional Nafion® membranes operated at low temperatures. In addition, it is found that with the present cell design, the limiting current density arising from the oxygen transfer limitation is around 700mAcm−2 even at 200°C. The short-term durability test at 200mAcm−2 and 180°C reveals that all the cells exhibit a gradual decrease in the voltage along with a rise in the internal resistance. The degradation rate of continuous operation is around 58.32μVh−1, which is much smaller than those of start/stop cycling operations.

Suggested Citation

  • Wu, Qixing & Li, Haiyang & Yuan, Wenxiang & Luo, Zhongkuan & Wang, Fang & Sun, Hongyuan & Zhao, Xuxin & Fu, Huide, 2015. "Performance evaluation of an air-breathing high-temperature proton exchange membrane fuel cell," Applied Energy, Elsevier, vol. 160(C), pages 146-152.
    • Handle: RePEc:eee:appene:v:160:y:2015:i:c:p:146-152
    DOI: 10.1016/j.apenergy.2015.09.042
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    References listed on IDEAS

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    1. Sun, Hong & Xie, Chen & Chen, Hao & Almheiri, Saif, 2015. "A numerical study on the effects of temperature and mass transfer in high temperature PEM fuel cells with ab-PBI membrane," Applied Energy, Elsevier, vol. 160(C), pages 937-944.
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    5. Kim, Sung Han & Miesse, Craig M. & Lee, Hee Bum & Chang, Ik Whang & Hwang, Yong Sheen & Jang, Jae Hyuk & Cha, Suk Won, 2014. "Ultra compact direct hydrogen fuel cell prototype using a metal hydride hydrogen storage tank for a mobile phone," Applied Energy, Elsevier, vol. 134(C), pages 382-391.
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    4. Kurnia, Jundika C. & Chaedir, Benitta A. & Sasmito, Agus P. & Shamim, Tariq, 2021. "Progress on open cathode proton exchange membrane fuel cell: Performance, designs, challenges and future directions," Applied Energy, Elsevier, vol. 283(C).
    5. Wu, Q.X. & Pan, Z.F. & An, L., 2018. "Recent advances in alkali-doped polybenzimidazole membranes for fuel cell applications," Renewable and Sustainable Energy Reviews, Elsevier, vol. 89(C), pages 168-183.
    6. Jiang, H.R. & Shyy, W. & Wu, M.C. & Zhang, R.H. & Zhao, T.S., 2019. "A bi-porous graphite felt electrode with enhanced surface area and catalytic activity for vanadium redox flow batteries," Applied Energy, Elsevier, vol. 233, pages 105-113.
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