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Catalytic pyrolysis of bamboo in a bubbling fluidized-bed reactor with two different catalysts: HZSM-5 and red mud for upgrading bio-oil

Author

Listed:
  • Ly, Hoang Vu
  • Park, Jeong Woo
  • Kim, Seung-Soo
  • Hwang, Hyun Tae
  • Kim, Jinsoo
  • Woo, Hee Chul

Abstract

Bamboo has been considered a potential feedstock of energy for the future. It can be subjected to the pyrolysis for biofuels production. The thermogravimetric analysis (TGA) combined with differential thermogravimetric analysis (DTG) for bamboo was carried out prior to pyrolysis. The thermal degradation of bamboo was mainly between 230 and 420 °C. The conventional pyrolysis of bamboo was investigated in a bubbling fluidized-bed reactor using silica sand. The product distribution and composition of pyrolysis bio-oil were dependent on biomass component and operating conditions such as pyrolysis temperature, fluidization velocity, and particle size of biomass. The fractional catalytic pyrolysis of bamboo was also studied to upgrade the pyrolysis vapor, using HZSM-5 and red mud. The highest yield of bio-oil was 54.03 wt% compared to 49.14 wt% and 50.34 wt% of HZSM-5 and red mud catalyst, respectively. In the red mud catalytic pyrolysis, the oxygen content was rejected from pyrolysis vapor mostly via decarboxylation to produce more CO2 than CO; in contrast, for the HZSM-5 catalytic pyrolysis, the production of CO through decarbonylation was more favored than CO2. The main composition of catalytic pyrolysis bio-oil was 4-vinylphenol, which was employed as a raw material source to synthesize valuable material for energy storage.

Suggested Citation

  • Ly, Hoang Vu & Park, Jeong Woo & Kim, Seung-Soo & Hwang, Hyun Tae & Kim, Jinsoo & Woo, Hee Chul, 2020. "Catalytic pyrolysis of bamboo in a bubbling fluidized-bed reactor with two different catalysts: HZSM-5 and red mud for upgrading bio-oil," Renewable Energy, Elsevier, vol. 149(C), pages 1434-1445.
  • Handle: RePEc:eee:renene:v:149:y:2020:i:c:p:1434-1445
    DOI: 10.1016/j.renene.2019.10.141
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    References listed on IDEAS

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    1. Ly, Hoang Vu & Kim, Seung-Soo & Woo, Hee Chul & Choi, Jae Hyung & Suh, Dong Jin & Kim, Jinsoo, 2015. "Fast pyrolysis of macroalga Saccharina japonica in a bubbling fluidized-bed reactor for bio-oil production," Energy, Elsevier, vol. 93(P2), pages 1436-1446.
    2. Park, Young-Kwon & Yoo, Myung Lang & Jin, Sung Ho & Park, Sung Hoon, 2015. "Catalytic fast pyrolysis of waste pepper stems over HZSM-5," Renewable Energy, Elsevier, vol. 79(C), pages 20-27.
    3. Ly, Hoang Vu & Kim, Jinsoo & Kim, Seung-Soo, 2013. "Pyrolysis characteristics and kinetics of palm fiber in a closed reactor," Renewable Energy, Elsevier, vol. 54(C), pages 91-95.
    4. Ly, Hoang Vu & Choi, Jae Hyung & Woo, Hee Chul & Kim, Seung-Soo & Kim, Jinsoo, 2019. "Upgrading bio-oil by catalytic fast pyrolysis of acid-washed Saccharina japonica alga in a fluidized-bed reactor," Renewable Energy, Elsevier, vol. 133(C), pages 11-22.
    5. Ly, Hoang Vu & Lim, Dong-Hyeon & Sim, Jae Wook & Kim, Seung-Soo & Kim, Jinsoo, 2018. "Catalytic pyrolysis of tulip tree (Liriodendron) in bubbling fluidized-bed reactor for upgrading bio-oil using dolomite catalyst," Energy, Elsevier, vol. 162(C), pages 564-575.
    6. Chen, Wei & Li, Kaixu & Xia, Mingwei & Yang, Haiping & Chen, Yingquan & Chen, Xu & Che, Qingfeng & Chen, Hanping, 2018. "Catalytic deoxygenation co-pyrolysis of bamboo wastes and microalgae with biochar catalyst," Energy, Elsevier, vol. 157(C), pages 472-482.
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    Cited by:

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    2. Shao, Shanshan & Zhang, Pengfei & Xiang, Xianliang & Li, Xiaohua & Zhang, Huiyan, 2022. "Promoted ketonization of bagasse pyrolysis gas over red mud-based oxides," Renewable Energy, Elsevier, vol. 190(C), pages 11-18.
    3. Tran, Quoc Khanh & Vo, Thuan Anh & Ly, Hoang Vu & Kwon, Byeongwan & Kim, Kwang Ho & Kim, Seung-Soo & Kim, Jinsoo, 2022. "Pyrolysis kinetics and product distribution of α-cellulose: Effect of potassium and calcium impregnation," Renewable Energy, Elsevier, vol. 181(C), pages 329-340.
    4. Bhattacharyya, Munmi & Shadangi, Krushna Prasad & Purkayastha, Rishiraj & Mahanta, Pinakeswar & Mohanty, Kaustubha, 2024. "Catalytic upgradation of pyrolytic products by catalytic pyrolysis of sawdust using a synthesized composite catalyst of NiO and Ni (II) aluminates," Renewable Energy, Elsevier, vol. 221(C).
    5. Zhang, Jun & Li, Chengyu & Yuan, Haoran & Chen, Yong, 2022. "Enhancement of aromatics production via cellulose fast pyrolysis over Ru modified hierarchical zeolites," Renewable Energy, Elsevier, vol. 184(C), pages 280-290.
    6. Douvartzides, Savvas & Charisiou, Nikolaos D. & Wang, Wen & Papadakis, Vagelis G. & Polychronopoulou, Kyriaki & Goula, Maria A., 2022. "Catalytic fast pyrolysis of agricultural residues and dedicated energy crops for the production of high energy density transportation biofuels. Part II: Catalytic research," Renewable Energy, Elsevier, vol. 189(C), pages 315-338.

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