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Promoted ketonization of bagasse pyrolysis gas over red mud-based oxides

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  • Shao, Shanshan
  • Zhang, Pengfei
  • Xiang, Xianliang
  • Li, Xiaohua
  • Zhang, Huiyan

Abstract

Ketonization of bagasse pyrolysis gas was performed over red mud-based oxides. The maximum yield of ketones in the catalytic conversion of bagasse pyrolysis gas over original red mud was 18.66% at 420 °C. To promote the oxidability of red mud and obtain a higher yield of ketones, the effect of metal oxides (CeO2, MnO2, TiO2, CaO, ZrO2) loading and loading amount of CeO2 on red mud on ketonization of bagasse pyrolysis gas were studied. The highest yield of ketones of 27.86% was obtained over red mud-based oxides with 40 wt% CeO2 loading. The oxidability of the catalyst was enhanced greatly by the high loading of CeO2, leading to the peroxidation of acetone as the side reaction. To control the oxidability and cut costs, bimetallic oxides were loaded on red mud. The yield of ketones reached 30.12% over the composite red mud catalyst with the loading of 20 wt% CeO2 and 20 wt% MnO2. The rough coating of MnO2 on the surface of red mud was beneficial to the loading of CeO2, resulting in smaller and more uniform grains. This study provides the efficient utilization of red mud and biomass as solid wastes for high-valued chemicals and fuels.

Suggested Citation

  • Shao, Shanshan & Zhang, Pengfei & Xiang, Xianliang & Li, Xiaohua & Zhang, Huiyan, 2022. "Promoted ketonization of bagasse pyrolysis gas over red mud-based oxides," Renewable Energy, Elsevier, vol. 190(C), pages 11-18.
  • Handle: RePEc:eee:renene:v:190:y:2022:i:c:p:11-18
    DOI: 10.1016/j.renene.2022.02.105
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    References listed on IDEAS

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    1. Shao, Shanshan & Liu, Chengyue & Xiang, Xianliang & Li, Xiaohua & Zhang, Huiyan & Xiao, Rui & Cai, Yixi, 2021. "In situ catalytic fast pyrolysis over CeO2 catalyst: Impact of biomass source, pyrolysis temperature and metal ion," Renewable Energy, Elsevier, vol. 177(C), pages 1372-1381.
    2. Kan, Tao & Strezov, Vladimir & Evans, Tim J., 2016. "Lignocellulosic biomass pyrolysis: A review of product properties and effects of pyrolysis parameters," Renewable and Sustainable Energy Reviews, Elsevier, vol. 57(C), pages 1126-1140.
    3. Ly, Hoang Vu & Park, Jeong Woo & Kim, Seung-Soo & Hwang, Hyun Tae & Kim, Jinsoo & Woo, Hee Chul, 2020. "Catalytic pyrolysis of bamboo in a bubbling fluidized-bed reactor with two different catalysts: HZSM-5 and red mud for upgrading bio-oil," Renewable Energy, Elsevier, vol. 149(C), pages 1434-1445.
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    1. Shuai Yuan & Ruofeng Wang & Hao Zhang & Yanjun Li & Liu Liu & Yafeng Fu, 2022. "Investigation of Mineral Phase Transformation Technology Followed by Magnetic Separation for Recovery of Iron Values from Red Mud," Sustainability, MDPI, vol. 14(21), pages 1-15, October.

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