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Catalytic deoxygenation co-pyrolysis of bamboo wastes and microalgae with biochar catalyst

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  • Chen, Wei
  • Li, Kaixu
  • Xia, Mingwei
  • Yang, Haiping
  • Chen, Yingquan
  • Chen, Xu
  • Che, Qingfeng
  • Chen, Hanping

Abstract

Catalytic deoxygenation co-pyrolysis of bamboo wastes and microalgae with biochar catalyst was investigated in a fixed bed reactor to explore the deoxygenation effect and possible deoxygenation mechanism of biochar catalyst (resulted from bamboo wastes pyrolysis). Results showed that oil fraction yields from co-pyrolysis of bamboo wastes and microalgae decreased largely with biochar addition, but still maintained at 35–37 wt.%, while gas yields were enhanced greatly. As catalytic co-pyrolysis promoted the decomposition of long-chain fatty acids and O-species, and the formation of aromatics and phenols, therefore most oxygen in bio-oil vapor transformed to CO, CO2 and H2O, and only 7–9 wt.% oxygen retained in oil fraction. It indicated that biochar catalytic co-pyrolysis could not only efficiently remove oxygen (over 90 wt.%), but also keep oil fraction yields. Moreover, the active O-containing groups and specific surface area of biochar catalyst decreased largely after catalytic co-pyrolysis. The possible reaction pathways of catalytic co-pyrolysis with biochar catalyst were proposed.

Suggested Citation

  • Chen, Wei & Li, Kaixu & Xia, Mingwei & Yang, Haiping & Chen, Yingquan & Chen, Xu & Che, Qingfeng & Chen, Hanping, 2018. "Catalytic deoxygenation co-pyrolysis of bamboo wastes and microalgae with biochar catalyst," Energy, Elsevier, vol. 157(C), pages 472-482.
    • Handle: RePEc:eee:energy:v:157:y:2018:i:c:p:472-482
    DOI: 10.1016/j.energy.2018.05.149
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    6. Liu, Huidong & Xu, Guoren & Li, Guibai, 2021. "Autocatalytic sludge pyrolysis by biochar derived from pharmaceutical sludge for biogas upgrading," Energy, Elsevier, vol. 229(C).
    7. Zhang, Zhikun & Zhu, Zongyuan & Shen, Boxiong & Liu, Lina, 2019. "Insights into biochar and hydrochar production and applications: A review," Energy, Elsevier, vol. 171(C), pages 581-598.
    8. Yang, Haiping & Chen, Zhiqun & Chen, Wei & Chen, Yingquan & Wang, Xianhua & Chen, Hanping, 2020. "Role of porous structure and active O-containing groups of activated biochar catalyst during biomass catalytic pyrolysis," Energy, Elsevier, vol. 210(C).
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    10. Wan Mahari, Wan Adibah & Chong, Cheng Tung & Cheng, Chin Kui & Lee, Chern Leing & Hendrata, Kristian & Yuh Yek, Peter Nai & Ma, Nyuk Ling & Lam, Su Shiung, 2018. "Production of value-added liquid fuel via microwave co-pyrolysis of used frying oil and plastic waste," Energy, Elsevier, vol. 162(C), pages 309-317.
    11. Chen, Wei & Fang, Yang & Li, Kaixu & Chen, Zhiqun & Xia, Mingwei & Gong, Meng & Chen, Yingquan & Yang, Haiping & Tu, Xin & Chen, Hanping, 2020. "Bamboo wastes catalytic pyrolysis with N-doped biochar catalyst for phenols products," Applied Energy, Elsevier, vol. 260(C).
    12. Ooi, Xian Yih & Gao, Wei & Ong, Hwai Chyuan & Lee, Hwei Voon & Juan, Joon Ching & Chen, Wei Hsin & Lee, Keat Teong, 2019. "Overview on catalytic deoxygenation for biofuel synthesis using metal oxide supported catalysts," Renewable and Sustainable Energy Reviews, Elsevier, vol. 112(C), pages 834-852.
    13. Douvartzides, Savvas & Charisiou, Nikolaos D. & Wang, Wen & Papadakis, Vagelis G. & Polychronopoulou, Kyriaki & Goula, Maria A., 2022. "Catalytic fast pyrolysis of agricultural residues and dedicated energy crops for the production of high energy density transportation biofuels. Part II: Catalytic research," Renewable Energy, Elsevier, vol. 189(C), pages 315-338.
    14. Chen, Wei & Gong, Meng & Li, Kaixu & Xia, Mingwei & Chen, Zhiqun & Xiao, Haoyu & Fang, Yang & Chen, Yingquan & Yang, Haiping & Chen, Hanping, 2020. "Insight into KOH activation mechanism during biomass pyrolysis: Chemical reactions between O-containing groups and KOH," Applied Energy, Elsevier, vol. 278(C).
    15. Elena Spennati & Alessandro Alberto Casazza & Attilio Converti & Guido Busca, 2020. "Thermocatalytic Pyrolysis of Exhausted Arthrospira platensis Biomass after Protein or Lipid Recovery," Energies, MDPI, vol. 13(20), pages 1-17, October.

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