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Advances in autothermal reformer design

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  • Pasel, Joachim
  • Samsun, Remzi Can
  • Tschauder, Andreas
  • Peters, Ralf
  • Stolten, Detlef

Abstract

Together with the high-temperature polymer electrolyte fuel cell, the reactor for the autothermal reforming (ATR) of liquid hydrocarbons, such as diesel fuel or kerosene, is the key component of the Jülich fuel cell system in the 5kWe power class. This paper presents some of Jülich’s most recent development in the field of ATR reactors, specifically the ATR 12. ATR 12 is characterized by a new concept for the internal generation of superheated steam as one of the ATR reactants using concentric shells instead of coiled tubing and particularly by the integration of an electric heating wire to enable fast and autonomous start-up. Three different experimental procedures for heating up the ATR 12 are presented and discussed, the most suitable of which enables the start-up of the ATR 12 within approximately 15min. As a consequence, from the system perspective, the bulky start-up burner, which is also difficult to control, along with the corresponding heat exchanger unit, can be dispensed with. Additionally, comprehensive steady-state experiments identify suitable reaction conditions for the operation of the ATR 12.

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  • Pasel, Joachim & Samsun, Remzi Can & Tschauder, Andreas & Peters, Ralf & Stolten, Detlef, 2017. "Advances in autothermal reformer design," Applied Energy, Elsevier, vol. 198(C), pages 88-98.
    • Handle: RePEc:eee:appene:v:198:y:2017:i:c:p:88-98
    DOI: 10.1016/j.apenergy.2017.04.055
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    1. Wang, Tiejun & Yang, Yong & Ding, Mingyue & Liu, Qiying & Ma, Longlong, 2013. "Auto-thermal reforming of biomass raw fuel gas to syngas in a novel reformer: Promotion of hot-electron," Applied Energy, Elsevier, vol. 112(C), pages 448-453.
    2. Peters, R. & Samsun, R.C., 2013. "Evaluation of multifunctional fuel cell systems in aviation using a multistep process analysis methodology," Applied Energy, Elsevier, vol. 111(C), pages 46-63.
    3. Wierzbicki, Teresa A. & Lee, Ivan C. & Gupta, Ashwani K., 2016. "Recent advances in catalytic oxidation and reformation of jet fuels," Applied Energy, Elsevier, vol. 165(C), pages 904-918.
    4. Samsun, Remzi Can & Pasel, Joachim & Janßen, Holger & Lehnert, Werner & Peters, Ralf & Stolten, Detlef, 2014. "Design and test of a 5kWe high-temperature polymer electrolyte fuel cell system operated with diesel and kerosene," Applied Energy, Elsevier, vol. 114(C), pages 238-249.
    5. Ercolino, Giuliana & Ashraf, Muhammad A. & Specchia, Vito & Specchia, Stefania, 2015. "Performance evaluation and comparison of fuel processors integrated with PEM fuel cell based on steam or autothermal reforming and on CO preferential oxidation or selective methanation," Applied Energy, Elsevier, vol. 143(C), pages 138-153.
    6. Chen, Xuejing & Jiang, Jianguo & Li, Kaimin & Tian, Sicong & Yan, Feng, 2017. "Energy-efficient biogas reforming process to produce syngas: The enhanced methane conversion by O2," Applied Energy, Elsevier, vol. 185(P1), pages 687-697.
    7. Walluk, Mark R. & Lin, Jiefeng & Waller, Michael G. & Smith, Daniel F. & Trabold, Thomas A., 2014. "Diesel auto-thermal reforming for solid oxide fuel cell systems: Anode off-gas recycle simulation," Applied Energy, Elsevier, vol. 130(C), pages 94-102.
    8. Xu, Xinhai & Li, Peiwen & Shen, Yuesong, 2013. "Small-scale reforming of diesel and jet fuels to make hydrogen and syngas for fuel cells: A review," Applied Energy, Elsevier, vol. 108(C), pages 202-217.
    9. Han, Gwangwoo & Lee, Sangho & Bae, Joongmyeon, 2015. "Diesel autothermal reforming with hydrogen peroxide for low-oxygen environments," Applied Energy, Elsevier, vol. 156(C), pages 99-106.
    10. Pasel, Joachim & Samsun, Remzi Can & Tschauder, Andreas & Peters, Ralf & Stolten, Detlef, 2015. "A novel reactor type for autothermal reforming of diesel fuel and kerosene," Applied Energy, Elsevier, vol. 150(C), pages 176-184.
    11. Pregelj, Boštjan & Micor, Michał & Dolanc, Gregor & Petrovčič, Janko & Jovan, Vladimir, 2016. "Impact of fuel cell and battery size to overall system performance – A diesel fuel-cell APU case study," Applied Energy, Elsevier, vol. 182(C), pages 365-375.
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    Cited by:

    1. Samsun, Remzi Can & Prawitz, Matthias & Tschauder, Andreas & Pasel, Joachim & Pfeifer, Peter & Peters, Ralf & Stolten, Detlef, 2018. "An integrated diesel fuel processing system with thermal start-up for fuel cells," Applied Energy, Elsevier, vol. 226(C), pages 145-159.
    2. Samsun, Remzi Can & Prawitz, Matthias & Tschauder, Andreas & Meißner, Jan & Pasel, Joachim & Peters, Ralf, 2020. "Reforming of diesel and jet fuel for fuel cells on a systems level: Steady-state and transient operation," Applied Energy, Elsevier, vol. 279(C).
    3. Tokimatsu, Koji & Höök, Mikael & McLellan, Benjamin & Wachtmeister, Henrik & Murakami, Shinsuke & Yasuoka, Rieko & Nishio, Masahiro, 2018. "Energy modeling approach to the global energy-mineral nexus: Exploring metal requirements and the well-below 2 °C target with 100 percent renewable energy," Applied Energy, Elsevier, vol. 225(C), pages 1158-1175.
    4. Abdin, Zainul & Zafaranloo, Ali & Rafiee, Ahmad & Mérida, Walter & Lipiński, Wojciech & Khalilpour, Kaveh R., 2020. "Hydrogen as an energy vector," Renewable and Sustainable Energy Reviews, Elsevier, vol. 120(C).

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