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Auto-thermal reforming of biomass raw fuel gas to syngas in a novel reformer: Promotion of hot-electron

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Listed:
  • Wang, Tiejun
  • Yang, Yong
  • Ding, Mingyue
  • Liu, Qiying
  • Ma, Longlong

Abstract

A novel reformer with porous ceramic oxygen distribution tube circled by electric wire for inspiring hot electron was designed for auto-thermal reforming of biomass raw fuel gas to produce syngas (H2+CO). The temperature of auto-thermal reformer was nearly uniform due to the excellent performance of partial oxygenation reaction in the reformer with porous ceramic tube for oxygen partitioning. The hot-electron inspired by electric wire promoted the cracking of biomass tar to form radical species, which were converted effectively to syngas over nickel based catalyst. The hot-electron also played an essential role in decreasing coke deposition on the surface of nickel based catalyst, which prolonged the lifetime of the reforming catalyst.

Suggested Citation

  • Wang, Tiejun & Yang, Yong & Ding, Mingyue & Liu, Qiying & Ma, Longlong, 2013. "Auto-thermal reforming of biomass raw fuel gas to syngas in a novel reformer: Promotion of hot-electron," Applied Energy, Elsevier, vol. 112(C), pages 448-453.
    • Handle: RePEc:eee:appene:v:112:y:2013:i:c:p:448-453
    DOI: 10.1016/j.apenergy.2013.05.054
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    References listed on IDEAS

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    1. Zhang, Qing & Wang, Tiejun & Li, Bing & Jiang, Ting & Ma, Longlong & Zhang, Xinghua & Liu, Qiying, 2012. "Aqueous phase reforming of sorbitol to bio-gasoline over Ni/HZSM-5 catalysts," Applied Energy, Elsevier, vol. 97(C), pages 509-513.
    2. Namioka, Tomoaki & Saito, Atsushi & Inoue, Yukiharu & Park, Yeongsu & Min, Tai-jin & Roh, Seon-ah & Yoshikawa, Kunio, 2011. "Hydrogen-rich gas production from waste plastics by pyrolysis and low-temperature steam reforming over a ruthenium catalyst," Applied Energy, Elsevier, vol. 88(6), pages 2019-2026, June.
    3. Rahimpour, Mohammad Reza & Jafari, Mitra & Iranshahi, Davood, 2013. "Progress in catalytic naphtha reforming process: A review," Applied Energy, Elsevier, vol. 109(C), pages 79-93.
    4. Qiu, Minghuang & Li, Yuping & Wang, Tiejun & Zhang, Qing & Wang, Chenguang & Zhang, Xinghua & Wu, Chuangzhi & Ma, Longlong & Li, Kai, 2012. "Upgrading biomass fuel gas by reforming over Ni–MgO/γ-Al2O3 cordierite monolithic catalysts in the lab-scale reactor and pilot-scale multi-tube reformer," Applied Energy, Elsevier, vol. 90(1), pages 3-10.
    5. Li, Chunlin & Xu, Hengyong & Hou, Shoufu & Sun, Jian & Meng, Fanqiong & Ma, Junguo & Tsubaki, Noritatsu, 2013. "SiC foam monolith catalyst for pressurized adiabatic methane reforming," Applied Energy, Elsevier, vol. 107(C), pages 297-303.
    6. Xu, Xinhai & Li, Peiwen & Shen, Yuesong, 2013. "Small-scale reforming of diesel and jet fuels to make hydrogen and syngas for fuel cells: A review," Applied Energy, Elsevier, vol. 108(C), pages 202-217.
    7. Liu, Qibin & Hong, Hui & Yuan, Jianli & Jin, Hongguang & Cai, Ruixian, 2009. "Experimental investigation of hydrogen production integrated methanol steam reforming with middle-temperature solar thermal energy," Applied Energy, Elsevier, vol. 86(2), pages 155-162, February.
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    Cited by:

    1. Hakawati, Rawan & Smyth, Beatrice M. & McCullough, Geoffrey & De Rosa, Fabio & Rooney, David, 2017. "What is the most energy efficient route for biogas utilization: Heat, electricity or transport?," Applied Energy, Elsevier, vol. 206(C), pages 1076-1087.
    2. Hu, Fu-Xiang & Yang, Guo-Hua & Ding, Guo-Zhu & Li, Zhen & Du, Ka-Shuai & Hu, Zhi-Fa & Tian, Su-Rui, 2016. "Experimental study on catalytic cracking of model tar compounds in a dual layer granular bed filter," Applied Energy, Elsevier, vol. 170(C), pages 47-57.
    3. Pasel, Joachim & Samsun, Remzi Can & Tschauder, Andreas & Peters, Ralf & Stolten, Detlef, 2017. "Advances in autothermal reformer design," Applied Energy, Elsevier, vol. 198(C), pages 88-98.
    4. Wang, Tiejun & Li, Kai & Liu, Qiying & Zhang, Qing & Qiu, Songbai & Long, Jinxing & Chen, Lungang & Ma, Longlong & Zhang, Qi, 2014. "Aviation fuel synthesis by catalytic conversion of biomass hydrolysate in aqueous phase," Applied Energy, Elsevier, vol. 136(C), pages 775-780.

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