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Decomposition of methane to hydrogen using nanosecond pulsed plasma reactor with different active volumes, voltages and frequencies

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  • Khalifeh, Omid
  • Mosallanejad, Amin
  • Taghvaei, Hamed
  • Rahimpour, Mohammad Reza
  • Shariati, Alireza

Abstract

In this paper, the methane conversion into hydrogen is investigated experimentally in a nanosecond pulsed DBD reactor. In order to achieve pure hydrogen production with minimum power consumption, effects of some operating parameters including external electrode length, applied voltage and pulse repetition frequency have been evaluated. Results show that although higher CH4 conversion and H2 concentration can be obtained at longer electrode lengths, higher applied voltages and pulse repetition frequencies, these parameters should be optimized for efficient hydrogen production. Actually, the maximum CH4 conversion of 87.2% and maximum hydrogen percentage of 80% are obtained at the external electrode length, discharge power, voltage and frequency of 15cm, 268.92W, 12kV and 10kHz, respectively. However, the maximum efficiency of 7.23% is achieved at the external electrode length of 15cm, applied voltage of 6kV, pulse repetition frequency of 0.9kHz and discharge power of 4W. Furthermore, at this condition, due to low temperature of discharge zone very little amount of solid carbon was observed on the inner electrode surface of the reactor.

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  • Khalifeh, Omid & Mosallanejad, Amin & Taghvaei, Hamed & Rahimpour, Mohammad Reza & Shariati, Alireza, 2016. "Decomposition of methane to hydrogen using nanosecond pulsed plasma reactor with different active volumes, voltages and frequencies," Applied Energy, Elsevier, vol. 169(C), pages 585-596.
    • Handle: RePEc:eee:appene:v:169:y:2016:i:c:p:585-596
    DOI: 10.1016/j.apenergy.2016.02.017
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    3. Gao, Yuan & Zhang, Shuai & Sun, Hao & Wang, Ruixue & Tu, Xin & Shao, Tao, 2018. "Highly efficient conversion of methane using microsecond and nanosecond pulsed spark discharges," Applied Energy, Elsevier, vol. 226(C), pages 534-545.
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    5. Xin, Yanbin & Sun, Bing & Zhu, Xiaomei & Yan, Zhiyu & Liu, Hui & Liu, Yongjun, 2016. "Effects of plate electrode materials on hydrogen production by pulsed discharge in ethanol solution," Applied Energy, Elsevier, vol. 181(C), pages 75-82.
    6. Hafizi, A. & Rahimpour, M.R. & Hassanajili, S., 2016. "High purity hydrogen production via sorption enhanced chemical looping reforming: Application of 22Fe2O3/MgAl2O4 and 22Fe2O3/Al2O3 as oxygen carriers and cerium promoted CaO as CO2 sorbent," Applied Energy, Elsevier, vol. 169(C), pages 629-641.
    7. Rahmati, Hamed & Ghorbanzadeh, Atamalek, 2021. "Parallel electrodes gliding plasma: Working principles and application in dry reforming of methane," Energy, Elsevier, vol. 230(C).
    8. Rincón, R. & Muñoz, J. & Morales-Calero, F.J. & Orejas, J. & Calzada, M.D., 2021. "Assessment of two atmospheric-pressure microwave plasma sources for H2 production from ethanol decomposition," Applied Energy, Elsevier, vol. 294(C).
    9. Wu, Angjian & Li, Xiaodong & Yan, Jianhua & Yang, Jian & Du, Changming & Zhu, Fengsen & Qian, Jinyuan, 2017. "Co-generation of hydrogen and carbon aerosol from coalbed methane surrogate using rotating gliding arc plasma," Applied Energy, Elsevier, vol. 195(C), pages 67-79.

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