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Effects of plate electrode materials on hydrogen production by pulsed discharge in ethanol solution

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  • Xin, Yanbin
  • Sun, Bing
  • Zhu, Xiaomei
  • Yan, Zhiyu
  • Liu, Hui
  • Liu, Yongjun

Abstract

Hydrogen production from an ethanol solution by pulsed high voltage spark discharge was optimized by varying the material of plate electrode. It is the first time that metal work function has been used in hydrogen production by plasma reforming. With low work function metal plate electrode, both energy efficiency and hydrogen yield can be increased. The flow rate and the percentage concentration of hydrogen were achieved 1.3L/min and 75% respectively while discharging with zinc plate electrode for hydrogen production, which is much better than traditional stainless steel electrodes at the same conditions. The analysis of emission spectra was also accomplished in this work. All the intensity of existing spectral lines showed a decline with higher work function metal as plate electrode, and H may be the key to the process of hydrogen production. Additionally, electron temperature and density were also estimated. Both of which were increased with lower work function metal plate electrodes. The electron temperature and density can reach 24,000K, 7.5×1018cm−3 respectively.

Suggested Citation

  • Xin, Yanbin & Sun, Bing & Zhu, Xiaomei & Yan, Zhiyu & Liu, Hui & Liu, Yongjun, 2016. "Effects of plate electrode materials on hydrogen production by pulsed discharge in ethanol solution," Applied Energy, Elsevier, vol. 181(C), pages 75-82.
    • Handle: RePEc:eee:appene:v:181:y:2016:i:c:p:75-82
    DOI: 10.1016/j.apenergy.2016.08.047
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    References listed on IDEAS

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    Cited by:

    1. Wang, Qiuying & Zhu, Xiaomei & Sun, Bing & Li, Zhi & Liu, Jinglin, 2022. "Hydrogen production from methane via liquid phase microwave plasma: A deoxidation strategy," Applied Energy, Elsevier, vol. 328(C).
    2. Xin, Yanbin & Sun, Bing & Liu, Jingyu & Wang, Quanli & Zhu, Xiaomei & Yan, Zhiyu, 2021. "Effects of electrode configurations, solution pH, TiO2 addition on hydrogen production by in-liquid discharge plasma," Renewable Energy, Elsevier, vol. 171(C), pages 728-734.
    3. Xin, Yanbin & Sun, Bing & Zhu, Xiaomei & Yan, Zhiyu & Zhao, Xiaotong & Sun, Xiaohang, 2017. "Hydrogen production from ethanol decomposition by pulsed discharge with needle-net configurations," Applied Energy, Elsevier, vol. 206(C), pages 126-133.
    4. Zhao, Xiaotong & Sun, Bing & Zhu, Tonghui & Zhu, Xiaomei & Yan, Zhiyu & Xin, Yanbin & Sun, Xiaohang, 2020. "Pathways of hydrogen-rich gas produced by microwave discharge in ethanol-water mixtures," Renewable Energy, Elsevier, vol. 156(C), pages 768-776.
    5. Wang, Xiaoling & Gao, Yuan & Zhang, Shuai & Sun, Hao & Li, Jie & Shao, Tao, 2019. "Nanosecond pulsed plasma assisted dry reforming of CH4: The effect of plasma operating parameters," Applied Energy, Elsevier, vol. 243(C), pages 132-144.
    6. Gao, Yuan & Zhang, Shuai & Sun, Hao & Wang, Ruixue & Tu, Xin & Shao, Tao, 2018. "Highly efficient conversion of methane using microsecond and nanosecond pulsed spark discharges," Applied Energy, Elsevier, vol. 226(C), pages 534-545.
    7. Wu, Angjian & Li, Xiaodong & Yan, Jianhua & Yang, Jian & Du, Changming & Zhu, Fengsen & Qian, Jinyuan, 2017. "Co-generation of hydrogen and carbon aerosol from coalbed methane surrogate using rotating gliding arc plasma," Applied Energy, Elsevier, vol. 195(C), pages 67-79.
    8. Wu, Tianyi & Wang, Junfeng & Zhang, Wei & Zuo, Lei & Xu, Haojie & Li, Bin, 2023. "Plasma bubble characteristics and hydrogen production performance of methanol decomposition by liquid phase discharge," Energy, Elsevier, vol. 273(C).
    9. Xin, Yanbin & Sun, Bing & Zhu, Xiaomei & Yan, Zhiyu & Sun, Xiaohang, 2021. "Hydrogen-rich syngas production by liquid phase pulsed electrodeless discharge," Energy, Elsevier, vol. 214(C).
    10. Xin, Yanbin & Wang, Quanli & Sun, Jiabao & Sun, Bing, 2022. "Plasma in aqueous methanol: Influence of plasma initiation mechanism on hydrogen production," Applied Energy, Elsevier, vol. 325(C).

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