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Plasma reforming of bio-ethanol for hydrogen rich gas production

Author

Listed:
  • Du, ChangMing
  • Mo, JianMin
  • Tang, Jun
  • Huang, DongWei
  • Mo, ZhiXing
  • Wang, QingKun
  • Ma, ShiZhe
  • Chen, ZhongJie

Abstract

Hydrogen production from ethanol by non-thermal arc discharge was investigated in a novel miniaturized plasma reactor. It is observed that ethanol–water mixture was converted into hydrogen, carbon monoxide and other products. The V–I characteristic was recorded by an oscilloscope to study the effect of discharge on the ethanol reforming. In the experiments, ethanol–water mixture entered the reaction chamber through a special gas–liquid spray nozzle for a quick evaporation and a rapid mixing with air at room temperature. Assisted by a Laval nozzle electrode, non-thermal arc plasma can improve the performance of ethanol reforming. It is found that the maximum conversion rate of ethanol was 90.9% at O/C=1.4, S/C=1.2 and ethanol flow rate=0.05g/s, and the maximum hydrogen yield was 40.9% at O/C=1.4, S/C=1.2 and ethanol flow rate=0.10g/s. The ethanol reforming process produced little coke and nitrogen oxide which was less than 10ppm in the supersonic/subsonic plasma working condition.

Suggested Citation

  • Du, ChangMing & Mo, JianMin & Tang, Jun & Huang, DongWei & Mo, ZhiXing & Wang, QingKun & Ma, ShiZhe & Chen, ZhongJie, 2014. "Plasma reforming of bio-ethanol for hydrogen rich gas production," Applied Energy, Elsevier, vol. 133(C), pages 70-79.
    • Handle: RePEc:eee:appene:v:133:y:2014:i:c:p:70-79
    DOI: 10.1016/j.apenergy.2014.07.088
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    References listed on IDEAS

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    1. Xin, Yanbin & Sun, Bing & Zhu, Xiaomei & Yan, Zhiyu & Liu, Hui & Liu, Yongjun, 2016. "Effects of plate electrode materials on hydrogen production by pulsed discharge in ethanol solution," Applied Energy, Elsevier, vol. 181(C), pages 75-82.
    2. Xin, Yanbin & Sun, Bing & Zhu, Xiaomei & Yan, Zhiyu & Zhao, Xiaotong & Sun, Xiaohang, 2017. "Hydrogen production from ethanol decomposition by pulsed discharge with needle-net configurations," Applied Energy, Elsevier, vol. 206(C), pages 126-133.
    3. Xin, Yanbin & Sun, Bing & Zhu, Xiaomei & Yan, Zhiyu & Liu, Yongjun & Liu, Hui, 2016. "Characteristics of hydrogen produced by pulsed discharge in ethanol solution," Applied Energy, Elsevier, vol. 168(C), pages 122-129.
    4. Wu, Angjian & Li, Xiaodong & Yan, Jianhua & Yang, Jian & Du, Changming & Zhu, Fengsen & Qian, Jinyuan, 2017. "Co-generation of hydrogen and carbon aerosol from coalbed methane surrogate using rotating gliding arc plasma," Applied Energy, Elsevier, vol. 195(C), pages 67-79.
    5. Lin, Bingxuan & Wu, Yun & Zhu, Yifei & Song, Feilong & Bian, Dongliang, 2019. "Experimental investigation of gliding arc plasma fuel injector for ignition and extinction performance improvement," Applied Energy, Elsevier, vol. 235(C), pages 1017-1026.
    6. Khalifeh, Omid & Mosallanejad, Amin & Taghvaei, Hamed & Rahimpour, Mohammad Reza & Shariati, Alireza, 2016. "Decomposition of methane to hydrogen using nanosecond pulsed plasma reactor with different active volumes, voltages and frequencies," Applied Energy, Elsevier, vol. 169(C), pages 585-596.

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