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Methane decomposition under a corona discharge to generate COx-free hydrogen

Author

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  • Aleknaviciute, I.
  • Karayiannis, T.G.
  • Collins, M.W.
  • Xanthos, C.

Abstract

A non-thermal plasma reforming unit operating at atmospheric pressure has been developed for converting methane to COx-free hydrogen. Argon was used to provide additional electrons and photons for higher reaction rates. A series of experiments was performed for positive corona discharge at a fixed inter-electrode distance (15 mm) to study the effects of discharge power (range of 14–20 W) and residence time (60, 120, 180 and 240 s). A second series of experiments studied the effect of inter-electrode distance on hydrogen production, with distances of 15, 20, 25, 30 and 35 mm tested. The analysis of the results shows that both discharge power and residence time, have a positive influence on methane conversion, hydrogen selectivity and energy conversion efficiency. Longer discharge gaps favour hydrogen production. A final series of experiments on corona polarity showed that a positive discharge was preferable.

Suggested Citation

  • Aleknaviciute, I. & Karayiannis, T.G. & Collins, M.W. & Xanthos, C., 2013. "Methane decomposition under a corona discharge to generate COx-free hydrogen," Energy, Elsevier, vol. 59(C), pages 432-439.
    • Handle: RePEc:eee:energy:v:59:y:2013:i:c:p:432-439
    DOI: 10.1016/j.energy.2013.06.059
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    References listed on IDEAS

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    Cited by:

    1. Ray, Debjyoti & Nepak, Devadutta & Vinodkumar, T. & Subrahmanyam, Ch., 2019. "g-C3N4 promoted DBD plasma assisted dry reforming of methane," Energy, Elsevier, vol. 183(C), pages 630-638.
    2. Alves, Luís & Pereira, Vítor & Lagarteira, Tiago & Mendes, Adélio, 2021. "Catalytic methane decomposition to boost the energy transition: Scientific and technological advancements," Renewable and Sustainable Energy Reviews, Elsevier, vol. 137(C).
    3. Raza, Jehangeer & Khoja, Asif Hussain & Anwar, Mustafa & Saleem, Faisal & Naqvi, Salman Raza & Liaquat, Rabia & Hassan, Muhammad & Javaid, Rahat & Qazi, Umair Yaqub & Lumbers, Brock, 2022. "Methane decomposition for hydrogen production: A comprehensive review on catalyst selection and reactor systems," Renewable and Sustainable Energy Reviews, Elsevier, vol. 168(C).
    4. Xin, Yanbin & Sun, Bing & Zhu, Xiaomei & Yan, Zhiyu & Sun, Xiaohang, 2021. "Hydrogen-rich syngas production by liquid phase pulsed electrodeless discharge," Energy, Elsevier, vol. 214(C).
    5. Khalifeh, Omid & Mosallanejad, Amin & Taghvaei, Hamed & Rahimpour, Mohammad Reza & Shariati, Alireza, 2016. "Decomposition of methane to hydrogen using nanosecond pulsed plasma reactor with different active volumes, voltages and frequencies," Applied Energy, Elsevier, vol. 169(C), pages 585-596.
    6. Czylkowski, Dariusz & Hrycak, Bartosz & Jasiński, Mariusz & Dors, Mirosław & Mizeraczyk, Jerzy, 2016. "Microwave plasma-based method of hydrogen production via combined steam reforming of methane," Energy, Elsevier, vol. 113(C), pages 653-661.

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