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Optimization of hydrogen production with CO2 capture by autothermal chemical-looping reforming using different bioethanol purities

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  • García-Díez, E.
  • García-Labiano, F.
  • de Diego, L.F.
  • Abad, A.
  • Gayán, P.
  • Adánez, J.
  • Ruíz, J.A.C.

Abstract

Autothermal Chemical-Looping Reforming (a-CLR) is a process which allows hydrogen production avoiding the environmental penalty of CO2 emission typically produced in other processes. The major advantage of this technology is that the heat needed for syngas production is generated by the process itself. The heat necessary for the endothermic reactions is supplied by a Ni-based oxygen-carrier (OC) circulating between two reactors: the air reactor (AR), where the OC is oxidized by air, and the fuel reactor (FR), where the fuel is converted to syngas. Other important advantage is that this process also allows the production of pure N2 in the AR outlet stream. A renewable fuel such as bioethanol was chosen in this work due to their increasing worldwide production and the current excess of this fuel presented by different countries.

Suggested Citation

  • García-Díez, E. & García-Labiano, F. & de Diego, L.F. & Abad, A. & Gayán, P. & Adánez, J. & Ruíz, J.A.C., 2016. "Optimization of hydrogen production with CO2 capture by autothermal chemical-looping reforming using different bioethanol purities," Applied Energy, Elsevier, vol. 169(C), pages 491-498.
    • Handle: RePEc:eee:appene:v:169:y:2016:i:c:p:491-498
    DOI: 10.1016/j.apenergy.2016.02.061
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    References listed on IDEAS

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    1. Dou, Binlin & Song, Yongchen & Wang, Chao & Chen, Haisheng & Yang, Mingjun & Xu, Yujie, 2014. "Hydrogen production by enhanced-sorption chemical looping steam reforming of glycerol in moving-bed reactors," Applied Energy, Elsevier, vol. 130(C), pages 342-349.
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    Cited by:

    1. Xin, Yanbin & Sun, Bing & Zhu, Xiaomei & Yan, Zhiyu & Liu, Hui & Liu, Yongjun, 2016. "Effects of plate electrode materials on hydrogen production by pulsed discharge in ethanol solution," Applied Energy, Elsevier, vol. 181(C), pages 75-82.
    2. Luo, Ming & Yi, Yang & Wang, Shuzhong & Wang, Zhuliang & Du, Min & Pan, Jianfeng & Wang, Qian, 2018. "Review of hydrogen production using chemical-looping technology," Renewable and Sustainable Energy Reviews, Elsevier, vol. 81(P2), pages 3186-3214.
    3. Mendiara, T. & García-Labiano, F. & Abad, A. & Gayán, P. & de Diego, L.F. & Izquierdo, M.T. & Adánez, J., 2018. "Negative CO2 emissions through the use of biofuels in chemical looping technology: A review," Applied Energy, Elsevier, vol. 232(C), pages 657-684.
    4. Shi, Bin & Wu, Erdorng & Wu, Wei, 2017. "Novel design of chemical looping air separation process for generating electricity and oxygen," Energy, Elsevier, vol. 134(C), pages 449-457.

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