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Performance and post-test characterization of an OTM system in an experimental coal gasifier

Author

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  • Gupta, Sapna
  • Adams, Joseph J.
  • Wilson, Jamie R.
  • Eddings, Eric G.
  • Mahapatra, Manoj K.
  • Singh, Prabhakar

Abstract

An early design of oxygen transport membranes (OTM) developed and fabricated by Praxair have been tested at 850–900°C in an experimental coal gasifier using a blend of Illinois and Powder River Basin (PRB) coals. Oxygen flux was measured and found to be stable over approximately 80h of gasifier operation. Study of interactions between the OTM and coal ash and gas phase impurities indicated that the OTM components remain chemically and structurally stable against coal ash and do not show any indication of solid or liquid (slagging) compound formation. The structure of the active fuel oxidation layer in the OTM exposed to the coal gas also remained stable and no interactions between the consecutive layers (porous support/fuel oxidation layer/gas separation layer/oxygen incorporation layer) were identified in the tested OTM system.

Suggested Citation

  • Gupta, Sapna & Adams, Joseph J. & Wilson, Jamie R. & Eddings, Eric G. & Mahapatra, Manoj K. & Singh, Prabhakar, 2016. "Performance and post-test characterization of an OTM system in an experimental coal gasifier," Applied Energy, Elsevier, vol. 165(C), pages 72-80.
  • Handle: RePEc:eee:appene:v:165:y:2016:i:c:p:72-80
    DOI: 10.1016/j.apenergy.2015.12.077
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    References listed on IDEAS

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    1. Hu, Yukun & Li, Xun & Li, Hailong & Yan, Jinyue, 2013. "Peak and off-peak operations of the air separation unit in oxy-coal combustion power generation systems," Applied Energy, Elsevier, vol. 112(C), pages 747-754.
    2. Hu, Yukun & Yan, Jinyue, 2012. "Characterization of flue gas in oxy-coal combustion processes for CO2 capture," Applied Energy, Elsevier, vol. 90(1), pages 113-121.
    3. Li, H. & Yan, J., 2009. "Evaluating cubic equations of state for calculation of vapor-liquid equilibrium of CO2 and CO2-mixtures for CO2 capture and storage processes," Applied Energy, Elsevier, vol. 86(6), pages 826-836, June.
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    5. Hu, Boxun & Keane, Michael & Patil, Kailash & Mahapatra, Manoj K. & Pasaogullari, Ugur & Singh, Prabhakar, 2014. "Direct methanol utilization in intermediate temperature liquid-tin anode solid oxide fuel cells," Applied Energy, Elsevier, vol. 134(C), pages 342-348.
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    Cited by:

    1. Singh, Surinder P. & Ohara, Brandon & Ku, Anthony Y., 2021. "Prospects for cost-competitive integrated gasification fuel cell systems," Applied Energy, Elsevier, vol. 290(C).

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