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Novel design of chemical looping air separation process for generating electricity and oxygen

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  • Shi, Bin
  • Wu, Erdorng
  • Wu, Wei

Abstract

The continuous- and batch-types chemical looping air separation (CLAS) processes are developed by using Aspen Plus® software. Through the heat integration of CLAS systems and oxy-fuel combustion of methane (OCM), new continuous- and batch-types of stand-alone electricity/oxygen production systems are denoted as Designs 1 and 2, respectively. The redox performances of both CLAS processes regarding Cu-, Mn-, and Co-based oxygen carriers with different ratios of inert binders are evaluated in terms of power/oxygen production ratios and specific CO2 emissions. A few comparisons show that (i) Design 1 using Cu- or Mn-based oxygen carriers at prescribed temperatures and normal pressures of oxidation and reduction can ensure almost zero CO2 emissions if the outlet 97 vol% of CO2 can be captured, (ii) Design 2 using Cu-based oxygen carrier with 83 wt% MgAl2O4 at a pressure of 8 atm and a temperature of 1070 °C during oxidation ensures almost zero CO2 emissions as well as the highest power production ratio, and (iii) Design 2 using Mn-based oxygen carrier with 37 wt% MgAl2O4 at a pressure of 15 atm and a temperature of 930 °C during oxidation ensures almost zero CO2 emissions as well as the largest oxygen production ratio.

Suggested Citation

  • Shi, Bin & Wu, Erdorng & Wu, Wei, 2017. "Novel design of chemical looping air separation process for generating electricity and oxygen," Energy, Elsevier, vol. 134(C), pages 449-457.
    • Handle: RePEc:eee:energy:v:134:y:2017:i:c:p:449-457
    DOI: 10.1016/j.energy.2017.05.080
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    Cited by:

    1. Tao, Ye & Tian, Wende & Kong, Lingqi & Sun, Suli & Fan, Chenyang, 2022. "Energy, exergy, economic, environmental (4E) and dynamic analysis based global optimization of chemical looping air separation for oxygen and power co-production," Energy, Elsevier, vol. 261(PB).
    2. Calin-Cristian Cormos, 2018. "Techno-Economic Evaluations of Copper-Based Chemical Looping Air Separation System for Oxy-Combustion and Gasification Power Plants with Carbon Capture," Energies, MDPI, vol. 11(11), pages 1-17, November.
    3. Szabolcs Szima & Carlos Arnaiz del Pozo & Schalk Cloete & Szabolcs Fogarasi & Ángel Jiménez Álvaro & Ana-Maria Cormos & Calin-Cristian Cormos & Shahriar Amini, 2021. "Techno-Economic Assessment of IGCC Power Plants Using Gas Switching Technology to Minimize the Energy Penalty of CO 2 Capture," Clean Technol., MDPI, vol. 3(3), pages 1-24, August.

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