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Fluidized bed testing of commercially prepared MgO-promoted hematite and CuO–Fe2O3 mixed metal oxide oxygen carriers for methane and coal chemical looping combustion

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  • Siriwardane, Ranjani
  • Tian, Hanjing
  • Miller, Duane
  • Richards, George

Abstract

Performance data of two commercially prepared oxygen carriers, MgO-promoted natural mineral hematite (Fe2O3) and synthetic mixed metal CuO–Fe2O3/alumina, are described in this paper. Large, 180-kg (400-pound) batches of both oxygen carriers were successfully prepared at a commercial catalyst preparation facility.

Suggested Citation

  • Siriwardane, Ranjani & Tian, Hanjing & Miller, Duane & Richards, George, 2015. "Fluidized bed testing of commercially prepared MgO-promoted hematite and CuO–Fe2O3 mixed metal oxide oxygen carriers for methane and coal chemical looping combustion," Applied Energy, Elsevier, vol. 157(C), pages 348-357.
    • Handle: RePEc:eee:appene:v:157:y:2015:i:c:p:348-357
    DOI: 10.1016/j.apenergy.2015.04.042
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    1. Miller, Duane D. & Siriwardane, Ranjani & Poston, James, 2015. "Fluidized-bed and fixed-bed reactor testing of methane chemical looping combustion with MgO-promoted hematite," Applied Energy, Elsevier, vol. 146(C), pages 111-121.
    2. Siriwardane, Ranjani V. & Ksepko, Ewelina & Tian, Hanjing & Poston, James & Simonyi, Thomas & Sciazko, Marek, 2013. "Interaction of iron–copper mixed metal oxide oxygen carriers with simulated synthesis gas derived from steam gasification of coal," Applied Energy, Elsevier, vol. 107(C), pages 111-123.
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    1. Görke, R.H. & Hu, W. & Dunstan, M.T. & Dennis, J.S. & Scott, S.A., 2018. "Exploration of the material property space for chemical looping air separation applied to carbon capture and storage," Applied Energy, Elsevier, vol. 212(C), pages 478-488.
    2. Mengjun Li & Teng Zheng & Daofeng Mei & Baowen Wang & Jingjing Ma, 2022. "Selecting and Testing of Cement-Bonded Magnetite and Chalcopyrite as Oxygen Carrier for Chemical-Looping Combustion," Energies, MDPI, vol. 15(14), pages 1-18, July.
    3. Lin, Shen & Gu, Zhenhua & Zhu, Xing & Wei, Yonggang & Long, Yanhui & Yang, Kun & He, Fang & Wang, Hua & Li, Kongzhai, 2020. "Synergy of red mud oxygen carrier with MgO and NiO for enhanced chemical-looping combustion," Energy, Elsevier, vol. 197(C).
    4. Nakano, Anna & Nakano, Jinichiro & Bennett, James, 2020. "Real-time high temperature investigations of an individual natural hematite ore particle for chemical looping oxygen exchange," Applied Energy, Elsevier, vol. 268(C).
    5. Benincosa, William & Siriwardane, Ranjani & Tian, Hanjing & Riley, Jarrett, 2017. "Unique phase identification of trimetallic copper iron manganese oxygen carrier using simultaneous differential scanning calorimetry/thermogravimetric analysis during chemical looping combustion react," Applied Energy, Elsevier, vol. 203(C), pages 522-534.
    6. Samuel Bayham & Ronald Breault & Justin Weber, 2017. "Chemical Looping Combustion of Hematite Ore with Methane and Steam in a Fluidized Bed Reactor," Energies, MDPI, vol. 10(8), pages 1-22, August.
    7. Riley, Jarrett & Siriwardane, Ranjani & Tian, Hanjing & Benincosa, William & Poston, James, 2018. "Experimental and kinetic analysis for particle scale modeling of a CuO-Fe2O3-Al2O3 oxygen carrier during reduction with H2 in chemical looping combustion applications," Applied Energy, Elsevier, vol. 228(C), pages 1515-1530.
    8. Cho, Won Chul & Lee, Jun Kyu & Nam, Gyeong Duk & Kim, Chang Hee & Cho, Hyun-Seok & Joo, Jong Hoon, 2019. "Degradation analysis of mixed ionic-electronic conductor-supported iron-oxide oxygen carriers for chemical-looping conversion of methane," Applied Energy, Elsevier, vol. 239(C), pages 644-657.
    9. Miccio, Francesco & Natali Murri, Annalisa & Landi, Elena, 2017. "Synthesis and characterization of geopolymer oxygen carriers for chemical looping combustion," Applied Energy, Elsevier, vol. 194(C), pages 136-147.
    10. He, Renze & Deng, Jin & Deng, Xiaoling & Xie, Xiaoguang & Li, Yun & Yuan, Shenfu, 2022. "Effects of alkali and alkaline earth metals of inherent minerals on Fe-catalyzed coal pyrolysis," Energy, Elsevier, vol. 238(PC).
    11. Ridha, Firas N. & Duchesne, Marc A. & Lu, Xuao & Lu, Dennis Y. & Filippou, Dimitrios & Hughes, Robin W., 2016. "Characterization of an ilmenite ore for pressurized chemical looping combustion," Applied Energy, Elsevier, vol. 163(C), pages 323-333.
    12. Khakpoor, Nima & Mostafavi, Ehsan & Mahinpey, Nader & De la Hoz Siegler, Hector, 2019. "Oxygen transport capacity and kinetic study of ilmenite ores for methane chemical-looping combustion," Energy, Elsevier, vol. 169(C), pages 329-337.
    13. Siriwardane, Ranjani & Riley, Jarrett & Bayham, Samuel & Straub, Douglas & Tian, Hanjing & Weber, Justin & Richards, George, 2018. "50-kWth methane/air chemical looping combustion tests with commercially prepared CuO-Fe2O3-alumina oxygen carrier with two different techniques," Applied Energy, Elsevier, vol. 213(C), pages 92-99.
    14. Huang, Xin & Fan, Maohong & Wang, Xingjun & Wang, Yonggang & Argyle, Morris D. & Zhu, Yufei, 2018. "A cost-effective approach to realization of the efficient methane chemical-looping combustion by using coal fly ash as a support for oxygen carrier," Applied Energy, Elsevier, vol. 230(C), pages 393-402.
    15. Siriwardane, Ranjani & Benincosa, William & Riley, Jarrett & Tian, Hanjing & Richards, George, 2016. "Investigation of reactions in a fluidized bed reactor during chemical looping combustion of coal/steam with copper oxide-iron oxide-alumina oxygen carrier," Applied Energy, Elsevier, vol. 183(C), pages 1550-1564.
    16. Lu, Xuao & Rahman, Ryad A. & Lu, Dennis Y. & Ridha, Firas N. & Duchesne, Marc A. & Tan, Yewen & Hughes, Robin W., 2016. "Pressurized chemical looping combustion with CO: Reduction reactivity and oxygen-transport capacity of ilmenite ore," Applied Energy, Elsevier, vol. 184(C), pages 132-139.

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