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Modeling of CH4 combustion with NiO/NiAl2O4 in a 10kWth CLC pilot plant

Author

Listed:
  • Yazdanpanah, M.M.
  • Forret, A.
  • Gauthier, T.
  • Delebarre, A.

Abstract

This paper presents a reactor model for combustion of CH4 with NiO/NiAl2O4 oxygen carriers in the Fuel Reactor of Chemical Looping Combustion (CLC) process. The model hydrodynamics is based on the two phase bubble - emulsion concept of bubbling fluidized beds, validated by residence time distribution tests conducted in a 10kWth equivalent cold flow prototype. The model kinetics is based on the literature and adjusted based on experimental results from a 10kWth CLC pilot plant. Results show the necessity of including both non-direct catalytic and non-catalytic direct reaction of gases on the oxygen carriers. The model shows good agreement with experimental results if some kinetic and hydrodynamic modifications are considered, including impact of gas adsorption by falling particles in the bubble phase on the gas exchange coefficient and thermodynamic limitation of CO and H2 combustion.

Suggested Citation

  • Yazdanpanah, M.M. & Forret, A. & Gauthier, T. & Delebarre, A., 2014. "Modeling of CH4 combustion with NiO/NiAl2O4 in a 10kWth CLC pilot plant," Applied Energy, Elsevier, vol. 113(C), pages 1933-1944.
    • Handle: RePEc:eee:appene:v:113:y:2014:i:c:p:1933-1944
    DOI: 10.1016/j.apenergy.2013.06.054
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    References listed on IDEAS

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    1. Siriwardane, Ranjani V. & Ksepko, Ewelina & Tian, Hanjing & Poston, James & Simonyi, Thomas & Sciazko, Marek, 2013. "Interaction of iron–copper mixed metal oxide oxygen carriers with simulated synthesis gas derived from steam gasification of coal," Applied Energy, Elsevier, vol. 107(C), pages 111-123.
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    Cited by:

    1. Jafarian, Mehdi & Arjomandi, Maziar & Nathan, Graham J., 2014. "A hybrid solar chemical looping combustion system with a high solar share," Applied Energy, Elsevier, vol. 126(C), pages 69-77.
    2. Chang, F.C. & Liao, P.H. & Tsai, C.K. & Hsiao, M.C. & Paul Wang, H., 2014. "Chemical-looping combustion of syngas with nano CuO–NiO on chabazite," Applied Energy, Elsevier, vol. 113(C), pages 1731-1736.
    3. Nandy, Anirban & Loha, Chanchal & Gu, Sai & Sarkar, Pinaki & Karmakar, Malay K. & Chatterjee, Pradip K., 2016. "Present status and overview of Chemical Looping Combustion technology," Renewable and Sustainable Energy Reviews, Elsevier, vol. 59(C), pages 597-619.

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