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The search of proper oxygen carriers for chemical looping partial oxidation of carbon

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  • Zhang, Jinzhi
  • He, Tao
  • Wang, Zhiqi
  • Zhu, Min
  • Zhang, Ke
  • Li, Bin
  • Wu, Jinhu

Abstract

Chemical looping partial oxidation process has more advantages over conventional chemical looping process, which can not only completely avoid the problem of greenhouse gas emissions, but also supply syngas products for chemical industry. The aim of the present work is to perform fundamental investigation on chemical looping partial oxidation of solid fuels. Production of CO through chemical looping partial oxidation of carbon was investigated in order to find proper oxygen carrier with good reactivity and high selectivity. A simple and easy to use method based on the zone division of Ellingham diagram was offered to distinguish the oxidation ability of various metal oxides, and three zones including complete oxidation, partial oxidation and inert zones were divided. CaFe2O4, Ca2Fe2O5 and FeAl2O4 in partial oxidation zone together with Fe2O3 in complete oxidation zone were chosen as target oxygen carriers (OCs) for chemical looping partial oxidation of carbon in this work. Of the target metal oxides, CaFe2O4 and Ca2Fe2O5 were found to have fast reaction rate, large oxygen-carrying capacity, high CO selectivity, and good regeneration performance, which made them very attractive for the purpose of chemical looping partial oxidation of solid fuels in real applications.

Suggested Citation

  • Zhang, Jinzhi & He, Tao & Wang, Zhiqi & Zhu, Min & Zhang, Ke & Li, Bin & Wu, Jinhu, 2017. "The search of proper oxygen carriers for chemical looping partial oxidation of carbon," Applied Energy, Elsevier, vol. 190(C), pages 1119-1125.
    • Handle: RePEc:eee:appene:v:190:y:2017:i:c:p:1119-1125
    DOI: 10.1016/j.apenergy.2017.01.024
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    2. Miller, Duane D. & Siriwardane, Ranjani, 2018. "CaFe2O4 oxygen carrier characterization during the partial oxidation of coal in the chemical looping gasification application," Applied Energy, Elsevier, vol. 224(C), pages 708-716.
    3. Mendiara, T. & García-Labiano, F. & Abad, A. & Gayán, P. & de Diego, L.F. & Izquierdo, M.T. & Adánez, J., 2018. "Negative CO2 emissions through the use of biofuels in chemical looping technology: A review," Applied Energy, Elsevier, vol. 232(C), pages 657-684.
    4. Liu, Guicai & Liao, Yanfen & Wu, Yuting & Ma, Xiaoqian, 2018. "Synthesis gas production from microalgae gasification in the presence of Fe2O3 oxygen carrier and CaO additive," Applied Energy, Elsevier, vol. 212(C), pages 955-965.
    5. Lei, Zhiping & Yan, Jingchong & Fang, Jia & Shui, Hengfu & Ren, Shibiao & Wang, Zhicai & Li, Zhanku & Kong, Ying & Kang, Shigang, 2021. "Catalytic combustion of coke and NO reduction in-situ under the action of Fe, Fe–CaO and Fe–CeO2," Energy, Elsevier, vol. 216(C).
    6. Liu, Shuai & Xiang, Dong & Xu, Ying & Sun, Zhe & Cao, Yan, 2017. "Relationship between electronic properties of Fe3O4 substituted by Ca and Ba and their reactivity in chemical looping process: A first-principles study," Applied Energy, Elsevier, vol. 202(C), pages 550-557.
    7. Li, Gang & Lv, Xuewei & Ding, Chengyi & Zhou, Xuangeng & Zhong, Dapeng & Qiu, Guibao, 2020. "Non-isothermal carbothermic reduction kinetics of calcium ferrite and hematite as oxygen carriers for chemical looping gasification applications," Applied Energy, Elsevier, vol. 262(C).

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