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Nanotube spin defects for omnidirectional magnetic field sensing

Author

Listed:
  • Xingyu Gao

    (Purdue University)

  • Sumukh Vaidya

    (Purdue University)

  • Saakshi Dikshit

    (Purdue University)

  • Peng Ju

    (Purdue University)

  • Kunhong Shen

    (Purdue University)

  • Yuanbin Jin

    (Purdue University)

  • Shixiong Zhang

    (Indiana University
    Indiana University)

  • Tongcang Li

    (Purdue University
    Purdue University
    Purdue University
    Purdue University)

Abstract

Optically addressable spin defects in three-dimensional (3D) crystals and two-dimensional (2D) van der Waals (vdW) materials are revolutionizing nanoscale quantum sensing. Spin defects in one-dimensional (1D) vdW nanotubes will provide unique opportunities due to their small sizes in two dimensions and absence of dangling bonds on side walls. However, optically detected magnetic resonance of localized spin defects in a nanotube has not been observed. Here, we report the observation of single spin color centers in boron nitride nanotubes (BNNTs) at room temperature. Our findings suggest that these BNNT spin defects possess a spin S = 1/2 ground state without an intrinsic quantization axis, leading to orientation-independent magnetic field sensing. We harness this unique feature to observe anisotropic magnetization of a 2D magnet in magnetic fields along orthogonal directions, a challenge for conventional spin S = 1 defects such as diamond nitrogen-vacancy centers. Additionally, we develop a method to deterministically transfer a BNNT onto a cantilever and use it to demonstrate scanning probe magnetometry. Further refinement of our approach will enable atomic scale quantum sensing of magnetic fields in any direction.

Suggested Citation

  • Xingyu Gao & Sumukh Vaidya & Saakshi Dikshit & Peng Ju & Kunhong Shen & Yuanbin Jin & Shixiong Zhang & Tongcang Li, 2024. "Nanotube spin defects for omnidirectional magnetic field sensing," Nature Communications, Nature, vol. 15(1), pages 1-8, December.
    • Handle: RePEc:nat:natcom:v:15:y:2024:i:1:d:10.1038_s41467-024-51941-2
    DOI: 10.1038/s41467-024-51941-2
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