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Long-lived electronic spin qubits in single-walled carbon nanotubes

Author

Listed:
  • Jia-Shiang Chen

    (Argonne National Laboratory
    Northwestern University)

  • Kasidet Jing Trerayapiwat

    (Boston University)

  • Lei Sun

    (Argonne National Laboratory)

  • Matthew D. Krzyaniak

    (Northwestern University
    Northwestern University)

  • Michael R. Wasielewski

    (Argonne National Laboratory
    Northwestern University
    Northwestern University)

  • Tijana Rajh

    (Argonne National Laboratory
    Arizona State University)

  • Sahar Sharifzadeh

    (Boston University)

  • Xuedan Ma

    (Argonne National Laboratory
    Northwestern University
    University of Chicago)

Abstract

Electron spins in solid-state systems offer the promise of spin-based information processing devices. Single-walled carbon nanotubes (SWCNTs), an all-carbon one-dimensional material whose spin-free environment and weak spin-orbit coupling promise long spin coherence times, offer a diverse degree of freedom for extended range of functionality not available to bulk systems. A key requirement limiting spin qubit implementation in SWCNTs is disciplined confinement of isolated spins. Here, we report the creation of highly confined electron spins in SWCNTs via a bottom-up approach. The record long coherence time of 8.2 µs and spin-lattice relaxation time of 13 ms of these electronic spin qubits allow demonstration of quantum control operation manifested as Rabi oscillation. Investigation of the decoherence mechanism reveals an intrinsic coherence time of tens of milliseconds. These findings evident that combining molecular approaches with inorganic crystalline systems provides a powerful route for reproducible and scalable quantum materials suitable for qubit applications.

Suggested Citation

  • Jia-Shiang Chen & Kasidet Jing Trerayapiwat & Lei Sun & Matthew D. Krzyaniak & Michael R. Wasielewski & Tijana Rajh & Sahar Sharifzadeh & Xuedan Ma, 2023. "Long-lived electronic spin qubits in single-walled carbon nanotubes," Nature Communications, Nature, vol. 14(1), pages 1-8, December.
  • Handle: RePEc:nat:natcom:v:14:y:2023:i:1:d:10.1038_s41467-023-36031-z
    DOI: 10.1038/s41467-023-36031-z
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    References listed on IDEAS

    as
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    Cited by:

    1. Xingyu Gao & Sumukh Vaidya & Saakshi Dikshit & Peng Ju & Kunhong Shen & Yuanbin Jin & Shixiong Zhang & Tongcang Li, 2024. "Nanotube spin defects for omnidirectional magnetic field sensing," Nature Communications, Nature, vol. 15(1), pages 1-8, December.

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