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Coherent control of an ultrabright single spin in hexagonal boron nitride at room temperature

Author

Listed:
  • Nai-Jie Guo

    (University of Science and Technology of China
    University of Science and Technology of China
    University of Science and Technology of China)

  • Song Li

    (Wigner Research Centre for Physics)

  • Wei Liu

    (University of Science and Technology of China
    University of Science and Technology of China
    University of Science and Technology of China)

  • Yuan-Ze Yang

    (University of Science and Technology of China
    University of Science and Technology of China
    University of Science and Technology of China)

  • Xiao-Dong Zeng

    (University of Science and Technology of China
    University of Science and Technology of China
    University of Science and Technology of China)

  • Shang Yu

    (University of Science and Technology of China
    University of Science and Technology of China
    University of Science and Technology of China)

  • Yu Meng

    (University of Science and Technology of China
    University of Science and Technology of China
    University of Science and Technology of China)

  • Zhi-Peng Li

    (University of Science and Technology of China
    University of Science and Technology of China
    University of Science and Technology of China)

  • Zhao-An Wang

    (University of Science and Technology of China
    University of Science and Technology of China
    University of Science and Technology of China)

  • Lin-Ke Xie

    (University of Science and Technology of China
    University of Science and Technology of China
    University of Science and Technology of China)

  • Rong-Chun Ge

    (Sichuan University)

  • Jun-Feng Wang

    (University of Science and Technology of China
    University of Science and Technology of China
    University of Science and Technology of China
    Sichuan University)

  • Qiang Li

    (University of Science and Technology of China
    University of Science and Technology of China
    University of Science and Technology of China)

  • Jin-Shi Xu

    (University of Science and Technology of China
    University of Science and Technology of China
    University of Science and Technology of China)

  • Yi-Tao Wang

    (University of Science and Technology of China
    University of Science and Technology of China
    University of Science and Technology of China)

  • Jian-Shun Tang

    (University of Science and Technology of China
    University of Science and Technology of China
    University of Science and Technology of China)

  • Adam Gali

    (Wigner Research Centre for Physics
    Budapest University of Technology and Economics)

  • Chuan-Feng Li

    (University of Science and Technology of China
    University of Science and Technology of China
    University of Science and Technology of China)

  • Guang-Can Guo

    (University of Science and Technology of China
    University of Science and Technology of China
    University of Science and Technology of China)

Abstract

Hexagonal boron nitride (hBN) is a remarkable two-dimensional (2D) material that hosts solid-state spins and has great potential to be used in quantum information applications, including quantum networks. However, in this application, both the optical and spin properties are crucial for single spins but have not yet been discovered simultaneously for hBN spins. Here, we realize an efficient method for arraying and isolating the single defects of hBN and use this method to discover a new spin defect with a high probability of 85%. This single defect exhibits outstanding optical properties and an optically controllable spin, as indicated by the observed significant Rabi oscillation and Hahn echo experiments at room temperature. First principles calculations indicate that complexes of carbon and oxygen dopants may be the origin of the single spin defects. This provides a possibility for further addressing spins that can be optically controlled.

Suggested Citation

  • Nai-Jie Guo & Song Li & Wei Liu & Yuan-Ze Yang & Xiao-Dong Zeng & Shang Yu & Yu Meng & Zhi-Peng Li & Zhao-An Wang & Lin-Ke Xie & Rong-Chun Ge & Jun-Feng Wang & Qiang Li & Jin-Shi Xu & Yi-Tao Wang & Ji, 2023. "Coherent control of an ultrabright single spin in hexagonal boron nitride at room temperature," Nature Communications, Nature, vol. 14(1), pages 1-8, December.
    • Handle: RePEc:nat:natcom:v:14:y:2023:i:1:d:10.1038_s41467-023-38672-6
    DOI: 10.1038/s41467-023-38672-6
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    References listed on IDEAS

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    1. Hannah L. Stern & Qiushi Gu & John Jarman & Simone Eizagirre Barker & Noah Mendelson & Dipankar Chugh & Sam Schott & Hoe H. Tan & Henning Sirringhaus & Igor Aharonovich & Mete Atatüre, 2022. "Room-temperature optically detected magnetic resonance of single defects in hexagonal boron nitride," Nature Communications, Nature, vol. 13(1), pages 1-9, December.
    2. Nikhil Mathur & Arunabh Mukherjee & Xingyu Gao & Jialun Luo & Brendan A. McCullian & Tongcang Li & A. Nick Vamivakas & Gregory D. Fuchs, 2022. "Excited-state spin-resonance spectroscopy of V $${}_{{{{{{{{\rm{B}}}}}}}}}^{-}$$ B − defect centers in hexagonal boron nitride," Nature Communications, Nature, vol. 13(1), pages 1-7, December.
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    1. Ruotian Gong & Xinyi Du & Eli Janzen & Vincent Liu & Zhongyuan Liu & Guanghui He & Bingtian Ye & Tongcang Li & Norman Y. Yao & James H. Edgar & Erik A. Henriksen & Chong Zu, 2024. "Isotope engineering for spin defects in van der Waals materials," Nature Communications, Nature, vol. 15(1), pages 1-9, December.

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