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Spin defects in hBN as promising temperature, pressure and magnetic field quantum sensors

Author

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  • Andreas Gottscholl

    (Experimental Physics 6 and Würzburg-Dresden Cluster of Excellence ct.qmat, Julius Maximilian University of Würzburg)

  • Matthias Diez

    (Experimental Physics 6 and Würzburg-Dresden Cluster of Excellence ct.qmat, Julius Maximilian University of Würzburg)

  • Victor Soltamov

    (Experimental Physics 6 and Würzburg-Dresden Cluster of Excellence ct.qmat, Julius Maximilian University of Würzburg
    Ioffe Institute)

  • Christian Kasper

    (Experimental Physics 6 and Würzburg-Dresden Cluster of Excellence ct.qmat, Julius Maximilian University of Würzburg)

  • Dominik Krauße

    (Experimental Physics 6 and Würzburg-Dresden Cluster of Excellence ct.qmat, Julius Maximilian University of Würzburg)

  • Andreas Sperlich

    (Experimental Physics 6 and Würzburg-Dresden Cluster of Excellence ct.qmat, Julius Maximilian University of Würzburg)

  • Mehran Kianinia

    (University of Technology Sydney
    University of Technology Sydney)

  • Carlo Bradac

    (Trent University)

  • Igor Aharonovich

    (University of Technology Sydney
    University of Technology Sydney)

  • Vladimir Dyakonov

    (Experimental Physics 6 and Würzburg-Dresden Cluster of Excellence ct.qmat, Julius Maximilian University of Würzburg)

Abstract

Spin defects in solid-state materials are strong candidate systems for quantum information technology and sensing applications. Here we explore in details the recently discovered negatively charged boron vacancies (VB−) in hexagonal boron nitride (hBN) and demonstrate their use as atomic scale sensors for temperature, magnetic fields and externally applied pressure. These applications are possible due to the high-spin triplet ground state and bright spin-dependent photoluminescence of the VB−. Specifically, we find that the frequency shift in optically detected magnetic resonance measurements is not only sensitive to static magnetic fields, but also to temperature and pressure changes which we relate to crystal lattice parameters. We show that spin-rich hBN films are potentially applicable as intrinsic sensors in heterostructures made of functionalized 2D materials.

Suggested Citation

  • Andreas Gottscholl & Matthias Diez & Victor Soltamov & Christian Kasper & Dominik Krauße & Andreas Sperlich & Mehran Kianinia & Carlo Bradac & Igor Aharonovich & Vladimir Dyakonov, 2021. "Spin defects in hBN as promising temperature, pressure and magnetic field quantum sensors," Nature Communications, Nature, vol. 12(1), pages 1-8, December.
    • Handle: RePEc:nat:natcom:v:12:y:2021:i:1:d:10.1038_s41467-021-24725-1
    DOI: 10.1038/s41467-021-24725-1
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    Cited by:

    1. Xingyu Gao & Sumukh Vaidya & Saakshi Dikshit & Peng Ju & Kunhong Shen & Yuanbin Jin & Shixiong Zhang & Tongcang Li, 2024. "Nanotube spin defects for omnidirectional magnetic field sensing," Nature Communications, Nature, vol. 15(1), pages 1-8, December.
    2. Ruotian Gong & Xinyi Du & Eli Janzen & Vincent Liu & Zhongyuan Liu & Guanghui He & Bingtian Ye & Tongcang Li & Norman Y. Yao & James H. Edgar & Erik A. Henriksen & Chong Zu, 2024. "Isotope engineering for spin defects in van der Waals materials," Nature Communications, Nature, vol. 15(1), pages 1-9, December.
    3. Sam C. Scholten & Priya Singh & Alexander J. Healey & Islay O. Robertson & Galya Haim & Cheng Tan & David A. Broadway & Lan Wang & Hiroshi Abe & Takeshi Ohshima & Mehran Kianinia & Philipp Reineck & I, 2024. "Multi-species optically addressable spin defects in a van der Waals material," Nature Communications, Nature, vol. 15(1), pages 1-8, December.
    4. Andrew J. Ramsay & Reza Hekmati & Charlie J. Patrickson & Simon Baber & David R. M. Arvidsson-Shukur & Anthony J. Bennett & Isaac J. Luxmoore, 2023. "Coherence protection of spin qubits in hexagonal boron nitride," Nature Communications, Nature, vol. 14(1), pages 1-8, December.
    5. Nikhil Mathur & Arunabh Mukherjee & Xingyu Gao & Jialun Luo & Brendan A. McCullian & Tongcang Li & A. Nick Vamivakas & Gregory D. Fuchs, 2022. "Excited-state spin-resonance spectroscopy of V $${}_{{{{{{{{\rm{B}}}}}}}}}^{-}$$ B − defect centers in hexagonal boron nitride," Nature Communications, Nature, vol. 13(1), pages 1-7, December.
    6. Nai-Jie Guo & Song Li & Wei Liu & Yuan-Ze Yang & Xiao-Dong Zeng & Shang Yu & Yu Meng & Zhi-Peng Li & Zhao-An Wang & Lin-Ke Xie & Rong-Chun Ge & Jun-Feng Wang & Qiang Li & Jin-Shi Xu & Yi-Tao Wang & Ji, 2023. "Coherent control of an ultrabright single spin in hexagonal boron nitride at room temperature," Nature Communications, Nature, vol. 14(1), pages 1-8, December.
    7. Roberto Rizzato & Martin Schalk & Stephan Mohr & Jens C. Hermann & Joachim P. Leibold & Fleming Bruckmaier & Giovanna Salvitti & Chenjiang Qian & Peirui Ji & Georgy V. Astakhov & Ulrich Kentsch & Manf, 2023. "Extending the coherence of spin defects in hBN enables advanced qubit control and quantum sensing," Nature Communications, Nature, vol. 14(1), pages 1-9, December.

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