IDEAS home Printed from https://ideas.repec.org/a/nat/natcom/v14y2023i1d10.1038_s41467-023-39979-0.html
   My bibliography  Save this article

μeV electron spectromicroscopy using free-space light

Author

Listed:
  • Yves Auad

    (Université Paris-Saclay, CNRS, Laboratoire de Physique des Solides)

  • Eduardo J. C. Dias

    (ICFO-Institut de Ciencies Fotoniques, The Barcelona Institute of Science and Technology)

  • Marcel Tencé

    (Université Paris-Saclay, CNRS, Laboratoire de Physique des Solides)

  • Jean-Denis Blazit

    (Université Paris-Saclay, CNRS, Laboratoire de Physique des Solides)

  • Xiaoyan Li

    (Université Paris-Saclay, CNRS, Laboratoire de Physique des Solides)

  • Luiz Fernando Zagonel

    (University of Campinas - UNICAMP)

  • Odile Stéphan

    (Université Paris-Saclay, CNRS, Laboratoire de Physique des Solides)

  • Luiz H. G. Tizei

    (Université Paris-Saclay, CNRS, Laboratoire de Physique des Solides)

  • F. Javier García de Abajo

    (ICFO-Institut de Ciencies Fotoniques, The Barcelona Institute of Science and Technology
    ICREA-Institució Catalana de Recerca i Estudis Avançats)

  • Mathieu Kociak

    (Université Paris-Saclay, CNRS, Laboratoire de Physique des Solides)

Abstract

The synergy between free electrons and light has recently been leveraged to reach an impressive degree of simultaneous spatial and spectral resolution, enabling applications in microscopy and quantum optics. However, the required combination of electron optics and light injection into the spectrally narrow modes of arbitrary specimens remains a challenge. Here, we demonstrate microelectronvolt spectral resolution with a sub-nanometer probe of photonic modes with quality factors as high as 104. We rely on mode matching of a tightly focused laser beam to whispering gallery modes to achieve a 108-fold increase in light-electron coupling efficiency. By adapting the shape and size of free-space optical beams to address specific physical questions, our approach allows us to interrogate any type of photonic structure with unprecedented spectral and spatial detail.

Suggested Citation

  • Yves Auad & Eduardo J. C. Dias & Marcel Tencé & Jean-Denis Blazit & Xiaoyan Li & Luiz Fernando Zagonel & Odile Stéphan & Luiz H. G. Tizei & F. Javier García de Abajo & Mathieu Kociak, 2023. "μeV electron spectromicroscopy using free-space light," Nature Communications, Nature, vol. 14(1), pages 1-6, December.
  • Handle: RePEc:nat:natcom:v:14:y:2023:i:1:d:10.1038_s41467-023-39979-0
    DOI: 10.1038/s41467-023-39979-0
    as

    Download full text from publisher

    File URL: https://www.nature.com/articles/s41467-023-39979-0
    File Function: Abstract
    Download Restriction: no

    File URL: https://libkey.io/10.1038/s41467-023-39979-0?utm_source=ideas
    LibKey link: if access is restricted and if your library uses this service, LibKey will redirect you to where you can use your library subscription to access this item
    ---><---

    References listed on IDEAS

    as
    1. Ondrej L. Krivanek & Tracy C. Lovejoy & Niklas Dellby & Toshihiro Aoki & R. W. Carpenter & Peter Rez & Emmanuel Soignard & Jiangtao Zhu & Philip E. Batson & Maureen J. Lagos & Ray F. Egerton & Peter A, 2014. "Vibrational spectroscopy in the electron microscope," Nature, Nature, vol. 514(7521), pages 209-212, October.
    2. Armin Feist & Katharina E. Echternkamp & Jakob Schauss & Sergey V. Yalunin & Sascha Schäfer & Claus Ropers, 2015. "Quantum coherent optical phase modulation in an ultrafast transmission electron microscope," Nature, Nature, vol. 521(7551), pages 200-203, May.
    3. Maureen J. Lagos & Andreas Trügler & Ulrich Hohenester & Philip E. Batson, 2017. "Mapping vibrational surface and bulk modes in a single nanocube," Nature, Nature, vol. 543(7646), pages 529-532, March.
    4. P. E. Batson & N. Dellby & O. L. Krivanek, 2002. "Sub-ångstrom resolution using aberration corrected electron optics," Nature, Nature, vol. 418(6898), pages 617-620, August.
    Full references (including those not matched with items on IDEAS)

    Citations

    Citations are extracted by the CitEc Project, subscribe to its RSS feed for this item.
    as


    Cited by:

    1. Akter, Hosne Ara & Masum, Farhad Hossain & Dwivedi, Puneet, 2024. "Life cycle emissions and unit production cost of sustainable aviation fuel from logging residues in Georgia, United States," Renewable Energy, Elsevier, vol. 228(C).

    Most related items

    These are the items that most often cite the same works as this one and are cited by the same works as this one.
    1. Ruochen Shi & Qize Li & Xiaofeng Xu & Bo Han & Ruixue Zhu & Fachen Liu & Ruishi Qi & Xiaowen Zhang & Jinlong Du & Ji Chen & Dapeng Yu & Xuetao Zhu & Jiandong Guo & Peng Gao, 2024. "Atomic-scale observation of localized phonons at FeSe/SrTiO3 interface," Nature Communications, Nature, vol. 15(1), pages 1-7, December.
    2. Zhe Cheng & Ruiyang Li & Xingxu Yan & Glenn Jernigan & Jingjing Shi & Michael E. Liao & Nicholas J. Hines & Chaitanya A. Gadre & Juan Carlos Idrobo & Eungkyu Lee & Karl D. Hobart & Mark S. Goorsky & X, 2021. "Experimental observation of localized interfacial phonon modes," Nature Communications, Nature, vol. 12(1), pages 1-10, December.
    3. Tal Fishman & Urs Haeusler & Raphael Dahan & Michael Yannai & Yuval Adiv & Tom Lenkiewicz Abudi & Roy Shiloh & Ori Eyal & Peyman Yousefi & Gadi Eisenstein & Peter Hommelhoff & Ido Kaminer, 2023. "Imaging the field inside nanophotonic accelerators," Nature Communications, Nature, vol. 14(1), pages 1-10, December.
    4. Xihang Shi & Lee Wei Wesley Wong & Sunchao Huang & Liang Jie Wong & Ido Kaminer, 2024. "Transverse recoil imprinted on free-electron radiation," Nature Communications, Nature, vol. 15(1), pages 1-11, December.
    5. John H. Gaida & Hugo Lourenço-Martins & Sergey V. Yalunin & Armin Feist & Murat Sivis & Thorsten Hohage & F. Javier García de Abajo & Claus Ropers, 2023. "Lorentz microscopy of optical fields," Nature Communications, Nature, vol. 14(1), pages 1-8, December.
    6. Tom Lee & Ji Qi & Chaitanya A. Gadre & Huaixun Huyan & Shu-Ting Ko & Yunxing Zuo & Chaojie Du & Jie Li & Toshihiro Aoki & Ruqian Wu & Jian Luo & Shyue Ping Ong & Xiaoqing Pan, 2023. "Atomic-scale origin of the low grain-boundary resistance in perovskite solid electrolyte Li0.375Sr0.4375Ta0.75Zr0.25O3," Nature Communications, Nature, vol. 14(1), pages 1-14, December.
    7. Jonathan J. P. Peters & Tiarnan Mullarkey & Emma Hedley & Karin H. Müller & Alexandra Porter & Ali Mostaed & Lewys Jones, 2023. "Electron counting detectors in scanning transmission electron microscopy via hardware signal processing," Nature Communications, Nature, vol. 14(1), pages 1-9, December.
    8. Hailing Jiang & Tao Wang & Zhenyu Zhang & Fang Liu & Ruochen Shi & Bowen Sheng & Shanshan Sheng & Weikun Ge & Ping Wang & Bo Shen & Bo Sun & Peng Gao & Lucas Lindsay & Xinqiang Wang, 2024. "Atomic-scale visualization of defect-induced localized vibrations in GaN," Nature Communications, Nature, vol. 15(1), pages 1-9, December.
    9. Ning Li & Ruochen Shi & Yifei Li & Ruishi Qi & Fachen Liu & Xiaowen Zhang & Zhetong Liu & Yuehui Li & Xiangdong Guo & Kaihui Liu & Ying Jiang & Xin-Zheng Li & Ji Chen & Lei Liu & En-Ge Wang & Peng Gao, 2023. "Phonon transition across an isotopic interface," Nature Communications, Nature, vol. 14(1), pages 1-7, December.
    10. R. Huber & F. Kern & D. D. Karnaushenko & E. Eisner & P. Lepucki & A. Thampi & A. Mirhajivarzaneh & C. Becker & T. Kang & S. Baunack & B. Büchner & D. Karnaushenko & O. G. Schmidt & A. Lubk, 2022. "Tailoring electron beams with high-frequency self-assembled magnetic charged particle micro optics," Nature Communications, Nature, vol. 13(1), pages 1-9, December.
    11. Valerio Di Giulio & F. Javier García de Abajo, 2023. "Nanophotonics for pair production," Nature Communications, Nature, vol. 14(1), pages 1-6, December.

    More about this item

    Statistics

    Access and download statistics

    Corrections

    All material on this site has been provided by the respective publishers and authors. You can help correct errors and omissions. When requesting a correction, please mention this item's handle: RePEc:nat:natcom:v:14:y:2023:i:1:d:10.1038_s41467-023-39979-0. See general information about how to correct material in RePEc.

    If you have authored this item and are not yet registered with RePEc, we encourage you to do it here. This allows to link your profile to this item. It also allows you to accept potential citations to this item that we are uncertain about.

    If CitEc recognized a bibliographic reference but did not link an item in RePEc to it, you can help with this form .

    If you know of missing items citing this one, you can help us creating those links by adding the relevant references in the same way as above, for each refering item. If you are a registered author of this item, you may also want to check the "citations" tab in your RePEc Author Service profile, as there may be some citations waiting for confirmation.

    For technical questions regarding this item, or to correct its authors, title, abstract, bibliographic or download information, contact: Sonal Shukla or Springer Nature Abstracting and Indexing (email available below). General contact details of provider: http://www.nature.com .

    Please note that corrections may take a couple of weeks to filter through the various RePEc services.

    IDEAS is a RePEc service. RePEc uses bibliographic data supplied by the respective publishers.