IDEAS home Printed from https://ideas.repec.org/a/nat/natcom/v14y2023i1d10.1038_s41467-023-42054-3.html
   My bibliography  Save this article

Lorentz microscopy of optical fields

Author

Listed:
  • John H. Gaida

    (Max Planck Institute for Multidisciplinary Sciences
    University of Göttingen)

  • Hugo Lourenço-Martins

    (Max Planck Institute for Multidisciplinary Sciences
    University of Göttingen)

  • Sergey V. Yalunin

    (Max Planck Institute for Multidisciplinary Sciences
    University of Göttingen)

  • Armin Feist

    (Max Planck Institute for Multidisciplinary Sciences
    University of Göttingen)

  • Murat Sivis

    (Max Planck Institute for Multidisciplinary Sciences
    University of Göttingen)

  • Thorsten Hohage

    (University of Göttingen)

  • F. Javier García de Abajo

    (The Barcelona Institute of Science and Technology
    ICREA-Institució Catalana de Recerca i Estudis Avançats)

  • Claus Ropers

    (Max Planck Institute for Multidisciplinary Sciences
    University of Göttingen)

Abstract

In electron microscopy, detailed insights into nanoscale optical properties of materials are gained by spontaneous inelastic scattering leading to electron-energy loss and cathodoluminescence. Stimulated scattering in the presence of external sample excitation allows for mode- and polarization-selective photon-induced near-field electron microscopy (PINEM). This process imprints a spatial phase profile inherited from the optical fields onto the wave function of the probing electrons. Here, we introduce Lorentz-PINEM for the full-field, non-invasive imaging of complex optical near fields at high spatial resolution. We use energy-filtered defocus phase-contrast imaging and iterative phase retrieval to reconstruct the phase distribution of interfering surface-bound modes on a plasmonic nanotip. Our approach is universally applicable to retrieve the spatially varying phase of nanoscale fields and topological modes.

Suggested Citation

  • John H. Gaida & Hugo Lourenço-Martins & Sergey V. Yalunin & Armin Feist & Murat Sivis & Thorsten Hohage & F. Javier García de Abajo & Claus Ropers, 2023. "Lorentz microscopy of optical fields," Nature Communications, Nature, vol. 14(1), pages 1-8, December.
  • Handle: RePEc:nat:natcom:v:14:y:2023:i:1:d:10.1038_s41467-023-42054-3
    DOI: 10.1038/s41467-023-42054-3
    as

    Download full text from publisher

    File URL: https://www.nature.com/articles/s41467-023-42054-3
    File Function: Abstract
    Download Restriction: no

    File URL: https://libkey.io/10.1038/s41467-023-42054-3?utm_source=ideas
    LibKey link: if access is restricted and if your library uses this service, LibKey will redirect you to where you can use your library subscription to access this item
    ---><---

    References listed on IDEAS

    as
    1. Emilio A. Nanni & Wenqian R. Huang & Kyung-Han Hong & Koustuban Ravi & Arya Fallahi & Gustavo Moriena & R. J. Dwayne Miller & Franz X. Kärtner, 2015. "Terahertz-driven linear electron acceleration," Nature Communications, Nature, vol. 6(1), pages 1-8, December.
    2. Giulio Guzzinati & Armand Béché & Hugo Lourenço-Martins & Jérôme Martin & Mathieu Kociak & Jo Verbeeck, 2017. "Probing the symmetry of the potential of localized surface plasmon resonances with phase-shaped electron beams," Nature Communications, Nature, vol. 8(1), pages 1-8, April.
    3. Armin Feist & Katharina E. Echternkamp & Jakob Schauss & Sergey V. Yalunin & Sascha Schäfer & Claus Ropers, 2015. "Quantum coherent optical phase modulation in an ultrafast transmission electron microscope," Nature, Nature, vol. 521(7551), pages 200-203, May.
    4. Kangpeng Wang & Raphael Dahan & Michael Shentcis & Yaron Kauffmann & Adi Ben Hayun & Ori Reinhardt & Shai Tsesses & Ido Kaminer, 2020. "Coherent interaction between free electrons and a photonic cavity," Nature, Nature, vol. 582(7810), pages 50-54, June.
    5. J. Krehl & G. Guzzinati & J. Schultz & P. Potapov & D. Pohl & Jérôme Martin & J. Verbeeck & A. Fery & B. Büchner & A. Lubk, 2018. "Spectral field mapping in plasmonic nanostructures with nanometer resolution," Nature Communications, Nature, vol. 9(1), pages 1-6, December.
    6. Jan-Wilke Henke & Arslan Sajid Raja & Armin Feist & Guanhao Huang & Germaine Arend & Yujia Yang & F. Jasmin Kappert & Rui Ning Wang & Marcel Möller & Jiahe Pan & Junqiu Liu & Ofer Kfir & Claus Ropers , 2021. "Integrated photonics enables continuous-beam electron phase modulation," Nature, Nature, vol. 600(7890), pages 653-658, December.
    7. X. Z. Yu & Y. Onose & N. Kanazawa & J. H. Park & J. H. Han & Y. Matsui & N. Nagaosa & Y. Tokura, 2010. "Real-space observation of a two-dimensional skyrmion crystal," Nature, Nature, vol. 465(7300), pages 901-904, June.
    Full references (including those not matched with items on IDEAS)

    Most related items

    These are the items that most often cite the same works as this one and are cited by the same works as this one.
    1. Tal Fishman & Urs Haeusler & Raphael Dahan & Michael Yannai & Yuval Adiv & Tom Lenkiewicz Abudi & Roy Shiloh & Ori Eyal & Peyman Yousefi & Gadi Eisenstein & Peter Hommelhoff & Ido Kaminer, 2023. "Imaging the field inside nanophotonic accelerators," Nature Communications, Nature, vol. 14(1), pages 1-10, December.
    2. Xihang Shi & Lee Wei Wesley Wong & Sunchao Huang & Liang Jie Wong & Ido Kaminer, 2024. "Transverse recoil imprinted on free-electron radiation," Nature Communications, Nature, vol. 15(1), pages 1-11, December.
    3. Hikaru Takeda & Masataka Kawano & Kyo Tamura & Masatoshi Akazawa & Jian Yan & Takeshi Waki & Hiroyuki Nakamura & Kazuki Sato & Yasuo Narumi & Masayuki Hagiwara & Minoru Yamashita & Chisa Hotta, 2024. "Magnon thermal Hall effect via emergent SU(3) flux on the antiferromagnetic skyrmion lattice," Nature Communications, Nature, vol. 15(1), pages 1-8, December.
    4. Satoru Hayami & Tsuyoshi Okubo & Yukitoshi Motome, 2021. "Phase shift in skyrmion crystals," Nature Communications, Nature, vol. 12(1), pages 1-6, December.
    5. Fumiya Sekiguchi & Kestutis Budzinauskas & Prashant Padmanabhan & Rolf B. Versteeg & Vladimir Tsurkan & István Kézsmárki & Francesco Foggetti & Sergey Artyukhin & Paul H. M. Loosdrecht, 2022. "Slowdown of photoexcited spin dynamics in the non-collinear spin-ordered phases in skyrmion host GaV4S8," Nature Communications, Nature, vol. 13(1), pages 1-8, December.
    6. Weiwei Wang & Dongsheng Song & Wensen Wei & Pengfei Nan & Shilei Zhang & Binghui Ge & Mingliang Tian & Jiadong Zang & Haifeng Du, 2022. "Electrical manipulation of skyrmions in a chiral magnet," Nature Communications, Nature, vol. 13(1), pages 1-7, December.
    7. Yu-Tsun Shao & Sujit Das & Zijian Hong & Ruijuan Xu & Swathi Chandrika & Fernando Gómez-Ortiz & Pablo García-Fernández & Long-Qing Chen & Harold Y. Hwang & Javier Junquera & Lane W. Martin & Ramamoort, 2023. "Emergent chirality in a polar meron to skyrmion phase transition," Nature Communications, Nature, vol. 14(1), pages 1-9, December.
    8. C. J. O. Reichhardt & C. Reichhardt, 2022. "Dynamic phases and reentrant Hall effect for vortices and skyrmions on periodic pinning arrays," The European Physical Journal B: Condensed Matter and Complex Systems, Springer;EDP Sciences, vol. 95(8), pages 1-16, August.
    9. Hanqing Zhao & Boris A. Malomed & Ivan I. Smalyukh, 2023. "Topological solitonic macromolecules," Nature Communications, Nature, vol. 14(1), pages 1-12, December.
    10. Deepak Singh & Yukako Fujishiro & Satoru Hayami & Samuel H. Moody & Takuya Nomoto & Priya R. Baral & Victor Ukleev & Robert Cubitt & Nina-Juliane Steinke & Dariusz J. Gawryluk & Ekaterina Pomjakushina, 2023. "Transition between distinct hybrid skyrmion textures through their hexagonal-to-square crystal transformation in a polar magnet," Nature Communications, Nature, vol. 14(1), pages 1-12, December.
    11. Fehmi Sami Yasin & Jan Masell & Kosuke Karube & Daisuke Shindo & Yasujiro Taguchi & Yoshinori Tokura & Xiuzhen Yu, 2023. "Heat current-driven topological spin texture transformations and helical q-vector switching," Nature Communications, Nature, vol. 14(1), pages 1-8, December.
    12. Pyeongjae Park & Woonghee Cho & Chaebin Kim & Yeochan An & Yoon-Gu Kang & Maxim Avdeev & Romain Sibille & Kazuki Iida & Ryoichi Kajimoto & Ki Hoon Lee & Woori Ju & En-Jin Cho & Han-Jin Noh & Myung Joo, 2023. "Tetrahedral triple-Q magnetic ordering and large spontaneous Hall conductivity in the metallic triangular antiferromagnet Co1/3TaS2," Nature Communications, Nature, vol. 14(1), pages 1-9, December.
    13. Yong Yu & Xiao Xu & Yan Wang & Baohai Jia & Shan Huang & Xiaobin Qiang & Bin Zhu & Peijian Lin & Binbin Jiang & Shixuan Liu & Xia Qi & Kefan Pan & Di Wu & Haizhou Lu & Michel Bosman & Stephen J. Penny, 2022. "Tunable quantum gaps to decouple carrier and phonon transport leading to high-performance thermoelectrics," Nature Communications, Nature, vol. 13(1), pages 1-9, December.
    14. Yongsen Zhang & Jin Tang & Yaodong Wu & Meng Shi & Xitong Xu & Shouguo Wang & Mingliang Tian & Haifeng Du, 2024. "Stable skyrmion bundles at room temperature and zero magnetic field in a chiral magnet," Nature Communications, Nature, vol. 15(1), pages 1-9, December.
    15. Xiaowei Lv & Hualiang Lv & Yalei Huang & Ruixuan Zhang & Guanhua Qin & Yihui Dong & Min Liu & Ke Pei & Guixin Cao & Jincang Zhang & Yuxiang Lai & Renchao Che, 2024. "Distinct skyrmion phases at room temperature in two-dimensional ferromagnet Fe3GaTe2," Nature Communications, Nature, vol. 15(1), pages 1-9, December.
    16. W. S. Huxter & M. L. Palm & M. L. Davis & P. Welter & C.-H. Lambert & M. Trassin & C. L. Degen, 2022. "Scanning gradiometry with a single spin quantum magnetometer," Nature Communications, Nature, vol. 13(1), pages 1-9, December.
    17. Mona Bhukta & Takaaki Dohi & Venkata Krishna Bharadwaj & Ricardo Zarzuela & Maria-Andromachi Syskaki & Michael Foerster & Miguel Angel Niño & Jairo Sinova & Robert Frömter & Mathias Kläui, 2024. "Homochiral antiferromagnetic merons, antimerons and bimerons realized in synthetic antiferromagnets," Nature Communications, Nature, vol. 15(1), pages 1-10, December.
    18. Rina Takagi & Naofumi Matsuyama & Victor Ukleev & Le Yu & Jonathan S. White & Sonia Francoual & José R. L. Mardegan & Satoru Hayami & Hiraku Saito & Koji Kaneko & Kazuki Ohishi & Yoshichika Ōnuki & Ta, 2022. "Square and rhombic lattices of magnetic skyrmions in a centrosymmetric binary compound," Nature Communications, Nature, vol. 13(1), pages 1-7, December.
    19. Yuan Yao & Bei Ding & Jinjing Liang & Hang Li & Xi Shen & Richeng Yu & Wenhong Wang, 2022. "Chirality flips of skyrmion bubbles," Nature Communications, Nature, vol. 13(1), pages 1-7, December.
    20. Andrew Fisher & Maximilian Lenz & Alex Ody & Yining Yang & Chad Pennington & Jared Maxson & Tara Hodgetts & Ronald Agustsson & Alex Murokh & Pietro Musumeci, 2024. "Towards higher frequencies in a compact prebunched waveguide THz-FEL," Nature Communications, Nature, vol. 15(1), pages 1-9, December.

    More about this item

    Statistics

    Access and download statistics

    Corrections

    All material on this site has been provided by the respective publishers and authors. You can help correct errors and omissions. When requesting a correction, please mention this item's handle: RePEc:nat:natcom:v:14:y:2023:i:1:d:10.1038_s41467-023-42054-3. See general information about how to correct material in RePEc.

    If you have authored this item and are not yet registered with RePEc, we encourage you to do it here. This allows to link your profile to this item. It also allows you to accept potential citations to this item that we are uncertain about.

    If CitEc recognized a bibliographic reference but did not link an item in RePEc to it, you can help with this form .

    If you know of missing items citing this one, you can help us creating those links by adding the relevant references in the same way as above, for each refering item. If you are a registered author of this item, you may also want to check the "citations" tab in your RePEc Author Service profile, as there may be some citations waiting for confirmation.

    For technical questions regarding this item, or to correct its authors, title, abstract, bibliographic or download information, contact: Sonal Shukla or Springer Nature Abstracting and Indexing (email available below). General contact details of provider: http://www.nature.com .

    Please note that corrections may take a couple of weeks to filter through the various RePEc services.

    IDEAS is a RePEc service. RePEc uses bibliographic data supplied by the respective publishers.