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Near-ideal electromechanical coupling in textured piezoelectric ceramics

Author

Listed:
  • Yongke Yan

    (Pennsylvania State University)

  • Liwei D. Geng

    (Michigan Technological University)

  • Hairui Liu

    (Pennsylvania State University)

  • Haoyang Leng

    (Pennsylvania State University)

  • Xiaotian Li

    (Pennsylvania State University)

  • Yu U. Wang

    (Michigan Technological University)

  • Shashank Priya

    (Pennsylvania State University)

Abstract

Electromechanical coupling factor, k, of piezoelectric materials determines the conversion efficiency of mechanical to electrical energy or electrical to mechanical energy. Here, we provide an fundamental approach to design piezoelectric materials that provide near-ideal magnitude of k, via exploiting the electrocrystalline anisotropy through fabrication of grain-oriented or textured ceramics. Coupled phase field simulation and experimental investigation on textured Pb(Mg1/3Nb2/3)O3-Pb(Zr,Ti)O3 ceramics illustrate that k can reach same magnitude as that for a single crystal, far beyond the average value of traditional ceramics. To provide atomistic-scale understanding of our approach, we employ a theoretical model to determine the physical origin of k in perovskite ferroelectrics and find that strong covalent bonding between B-site cation and oxygen via d-p hybridization contributes most towards the magnitude of k. This demonstration of near-ideal k value in textured ceramics will have tremendous impact on design of ultra-wide bandwidth, high efficiency, high power density, and high stability piezoelectric devices.

Suggested Citation

  • Yongke Yan & Liwei D. Geng & Hairui Liu & Haoyang Leng & Xiaotian Li & Yu U. Wang & Shashank Priya, 2022. "Near-ideal electromechanical coupling in textured piezoelectric ceramics," Nature Communications, Nature, vol. 13(1), pages 1-9, December.
    • Handle: RePEc:nat:natcom:v:13:y:2022:i:1:d:10.1038_s41467-022-31165-y
    DOI: 10.1038/s41467-022-31165-y
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    References listed on IDEAS

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    1. Shuai Yang & Jinglei Li & Yao Liu & Mingwen Wang & Liao Qiao & Xiangyu Gao & Yunfei Chang & Hongliang Du & Zhuo Xu & Shujun Zhang & Fei Li, 2021. "Textured ferroelectric ceramics with high electromechanical coupling factors over a broad temperature range," Nature Communications, Nature, vol. 12(1), pages 1-10, December.
    2. Fei Li & Shujun Zhang & Tiannan Yang & Zhuo Xu & Nan Zhang & Gang Liu & Jianjun Wang & Jianli Wang & Zhenxiang Cheng & Zuo-Guang Ye & Jun Luo & Thomas R. Shrout & Long-Qing Chen, 2016. "The origin of ultrahigh piezoelectricity in relaxor-ferroelectric solid solution crystals," Nature Communications, Nature, vol. 7(1), pages 1-9, December.
    3. Yasuyoshi Saito & Hisaaki Takao & Toshihiko Tani & Tatsuhiko Nonoyama & Kazumasa Takatori & Takahiko Homma & Toshiatsu Nagaya & Masaya Nakamura, 2004. "Lead-free piezoceramics," Nature, Nature, vol. 432(7013), pages 84-87, November.
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    1. Jinfeng Lin & Jin Qian & Guanglong Ge & Yuxuan Yang & Jiangfan Li & Xiao Wu & Guohui Li & Simin Wang & Yingchun Liu & Jialiang Zhang & Jiwei Zhai & Xiaoming Shi & Haijun Wu, 2024. "Multiscale reconfiguration induced highly saturated poling in lead-free piezoceramics for giant energy conversion," Nature Communications, Nature, vol. 15(1), pages 1-11, December.

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