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Economic assessment of biogas purification systems for removal of both H2S and siloxane from biogas

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  • Zhang, Yuyao
  • Kawasaki, Yu
  • Oshita, Kazuyuki
  • Takaoka, Masaki
  • Minami, Daisuke
  • Inoue, Go
  • Tanaka, Toshihiro

Abstract

Biogas is a promising renewable biofuel, but hydrogen sulfide (H2S) and siloxanes are major obstacles in the conversion of bioenergy from biogas because they damage biogas-processing equipment. This study evaluated two biogas-purification systems for a simultaneous efficient removal of H2S and decamethylcyclopentasiloxane (D5), and compared their economic performance. An acidic biotrickling filter (BTF) was operated continuously for 90 days to investigate its performance under different H2S and D5 concentrations. Meanwhile, commercial iron-oxide-based adsorbents (IOBAs) and activated carbon (AC) were used in adsorption filters for H2S and D5, respectively. The results show that in terms of the ratio of D5 and H2S concentration (RD5:H2S) and pH of the recycling liquid, which are crucial BTF operating parameters, high elimination for both H2S (1.86 kg/(m3·d)) and D5 (0.282 kg/(m3·d)) was achieved at RD5:H2S of 3.7:16 and pH of 0.86. Economic analysis confirmed that BTF-AC was more profitable than IOBA-AC adsorption over a life span of 10 years because the pre-removal of D5 by a BTF significantly decreased the costs of IOBAs and AC, despite BTFs requiring a higher initial capital investment. In terms of the economic benefit of biogas production of 1200 Nm3/h, the competitive annual cost of 90.5 k$/year indicated that BTF was more profitable, yielding both cost saving and the benefit of providing heat. The advantage of BTF-AC adsorption was a more radical D5-abatament, enabling profit by selling the electricity produced from biogas to the grid.

Suggested Citation

  • Zhang, Yuyao & Kawasaki, Yu & Oshita, Kazuyuki & Takaoka, Masaki & Minami, Daisuke & Inoue, Go & Tanaka, Toshihiro, 2021. "Economic assessment of biogas purification systems for removal of both H2S and siloxane from biogas," Renewable Energy, Elsevier, vol. 168(C), pages 119-130.
    • Handle: RePEc:eee:renene:v:168:y:2021:i:c:p:119-130
    DOI: 10.1016/j.renene.2020.12.058
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    2. Kazimierz Gaj & Klaudia Cichuta, 2022. "Combined Biological Method for Simultaneous Removal of Hydrogen Sulphide and Volatile Methylsiloxanes from Biogas," Energies, MDPI, vol. 16(1), pages 1-18, December.
    3. Zheng, Yanhui & Hou, Xifeng & Liu, Yuheng & Ma, Zichuan, 2021. "Hexamethyldisiloxane removal from biogas using reduced graphene-oxide aerogels as adsorbents," Renewable Energy, Elsevier, vol. 178(C), pages 153-161.
    4. Becker, C.M. & Marder, M. & Junges, E. & Konrad, O., 2022. "Technologies for biogas desulfurization - An overview of recent studies," Renewable and Sustainable Energy Reviews, Elsevier, vol. 159(C).
    5. Lianghu Su & Mei Chen & Guihua Zhuo & Rongting Ji & Saier Wang & Longjiang Zhang & Mingzhu Zhang & Haidong Li, 2021. "Comparison of Biochar Materials Derived from Coconut Husks and Various Types of Livestock Manure, and Their Potential for Use in Removal of H 2 S from Biogas," Sustainability, MDPI, vol. 13(11), pages 1-13, June.
    6. Hou, Xifeng & Zheng, Yanhui & Lv, Siqi & Ma, Zichuan & Ma, Xiaolong, 2022. "Effective removal of hexamethyldisiloxane using a citric acid modified three-dimensional graphene aerogel," Renewable Energy, Elsevier, vol. 199(C), pages 62-70.
    7. Lv, Siqi & Zhang, Rui & He, Yuanping & Ma, Zichuan & Ma, Xiaolong, 2024. "Efficient reactive adsorption of hexamethyldisiloxane on MCM-41 supported sulfuric acid," Renewable Energy, Elsevier, vol. 224(C).
    8. Mulu, Elshaday & M'Arimi, Milton M. & Ramkat, Rose C., 2021. "A review of recent developments in application of low cost natural materials in purification and upgrade of biogas," Renewable and Sustainable Energy Reviews, Elsevier, vol. 145(C).
    9. Pallavicini, Jacopo & Fedeli, Matteo & Scolieri, Giacomo Domenico & Tagliaferri, Francesca & Parolin, Jacopo & Sironi, Selena & Manenti, Flavio, 2023. "Digital twin-based optimization and demo-scale validation of absorption columns using sodium hydroxide/water mixtures for the purification of biogas streams subject to impurity fluctuations," Renewable Energy, Elsevier, vol. 219(P1).

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