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Coupling adsorption with biotechnologies for siloxane abatement from biogas

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  • Santos-Clotas, Eric
  • Cabrera-Codony, Alba
  • Martín, Maria J.

Abstract

Biogas generated during anaerobic digestion in sewage plants contains a wide spectrum of trace impurities. Siloxanes are the most hazardous pollutants and its removal is mandatory for most energy applications. The most widely used technology is adsorption onto activated carbon (AC) despite the high operating costs. In this context, the use of biotechnologies to abate biogas pollutants could assist extending the lifetime of the AC filters. The present work evaluated at lab-scale the potentialities of implementing a biotrickling filter (BTF) before the adsorption technology. Moreover, the use of ACs with different characteristics and price was evaluated considering their selectivity towards siloxane over volatile organic compounds (VOCs). The pre-treatment of biogas in a BTF capable of eliminating VOCs like limonene increased significantly the adsorbent performance, reaching 690 m3 L−1 of biogas treated per bed volume by a phosphoric-activated carbon, a six-fold increase in the performance of currently used materials in adsorption treatment. In terms of cost, a steam-activated coal-based with a major mesoporosity contribution implied the lowest operating costs reaching 2.3 € (1000 m3treated)−1. Coupling BTF with adsorption into this same AC resulted in lower annual costs than adsorption alone due to the frequent replacements required when biogas was not pre-polished.

Suggested Citation

  • Santos-Clotas, Eric & Cabrera-Codony, Alba & Martín, Maria J., 2020. "Coupling adsorption with biotechnologies for siloxane abatement from biogas," Renewable Energy, Elsevier, vol. 153(C), pages 314-323.
    • Handle: RePEc:eee:renene:v:153:y:2020:i:c:p:314-323
    DOI: 10.1016/j.renene.2020.02.026
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    References listed on IDEAS

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    1. Eric Santos-Clotas & Alba Cabrera-Codony & Alba Castillo & Maria J. Martín & Manel Poch & Hèctor Monclús, 2019. "Environmental Decision Support System for Biogas Upgrading to Feasible Fuel," Energies, MDPI, vol. 12(8), pages 1-14, April.
    2. Zhang, Quanguo & Hu, Jianjun & Lee, Duu-Jong, 2016. "Biogas from anaerobic digestion processes: Research updates," Renewable Energy, Elsevier, vol. 98(C), pages 108-119.
    3. Tribe, M. A. & Alpine, R. L. W., 1986. "Scale economies and the "0.6 rule"," Engineering Costs and Production Economics, Elsevier, vol. 10(4), pages 271-278, March.
    4. de Arespacochaga, N. & Valderrama, C. & Raich-Montiu, J. & Crest, M. & Mehta, S. & Cortina, J.L., 2015. "Understanding the effects of the origin, occurrence, monitoring, control, fate and removal of siloxanes on the energetic valorization of sewage biogas—A review," Renewable and Sustainable Energy Reviews, Elsevier, vol. 52(C), pages 366-381.
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    1. Kazimierz Gaj & Klaudia Cichuta, 2022. "Combined Biological Method for Simultaneous Removal of Hydrogen Sulphide and Volatile Methylsiloxanes from Biogas," Energies, MDPI, vol. 16(1), pages 1-18, December.
    2. Dai, Huaming & Zhu, Huiwei, 2022. "Enhancement of partial oxidation reformer by the free-section addition for hydrogen production," Renewable Energy, Elsevier, vol. 190(C), pages 425-433.
    3. Zhang, Yuyao & Kawasaki, Yu & Oshita, Kazuyuki & Takaoka, Masaki & Minami, Daisuke & Inoue, Go & Tanaka, Toshihiro, 2021. "Economic assessment of biogas purification systems for removal of both H2S and siloxane from biogas," Renewable Energy, Elsevier, vol. 168(C), pages 119-130.
    4. Edyta Słupek & Patrycja Makoś & Jacek Gębicki, 2020. "Theoretical and Economic Evaluation of Low-Cost Deep Eutectic Solvents for Effective Biogas Upgrading to Bio-Methane," Energies, MDPI, vol. 13(13), pages 1-19, July.

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