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Determination of organic silicon compounds in biogas from wastewater treatments plants, landfills, and co-digestion plants

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  • Rasi, Saija
  • Lehtinen, Jenni
  • Rintala, Jukka

Abstract

The study determined the organic silicon compounds in biogases from landfills, wastewater treatment plants (WWTPs), and biogas plants processing different organic material. The aim was to provide information for gas utilisation applications, as siloxanes are reported to shorten the life time of engines when biogas is used for energy production. In total, 48 samples were measured. The total concentration of organic silicon compounds in landfill and WWTP gases varied from 77 to 2460 μg/m3 while the concentrations in biogases from biogas plants varied from 24 to 820 μg/m3. The total concentration of organic silicon compounds was lowest (24 μg/m3) in the biogas plant processing grass and maize, and highest (2460 μg/m3) in one of the studied WWTP. The most common compounds in WWTPs and in biogas plants processing also sewage sludge were D4 and D5 while in landfills the most common compounds were D4 and L2 followed by trimethyl silanol. The effect of condensation of biogas on concentrations of organic silicon compounds was studied in one of the landfills and a negligible effect on concentrations was detected.

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  • Rasi, Saija & Lehtinen, Jenni & Rintala, Jukka, 2010. "Determination of organic silicon compounds in biogas from wastewater treatments plants, landfills, and co-digestion plants," Renewable Energy, Elsevier, vol. 35(12), pages 2666-2673.
    • Handle: RePEc:eee:renene:v:35:y:2010:i:12:p:2666-2673
    DOI: 10.1016/j.renene.2010.04.012
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    1. Rasi, S. & Veijanen, A. & Rintala, J., 2007. "Trace compounds of biogas from different biogas production plants," Energy, Elsevier, vol. 32(8), pages 1375-1380.
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    1. Rey, M.D. & Font, R. & Aracil, I., 2013. "Biogas from MSW landfill: Composition and determination of chlorine content with the AOX (adsorbable organically bound halogens) technique," Energy, Elsevier, vol. 63(C), pages 161-167.
    2. Kazimierz Gaj, 2020. "Adsorptive Biogas Purification from Siloxanes—A Critical Review," Energies, MDPI, vol. 13(10), pages 1-10, May.
    3. Vita, A. & Italiano, C. & Previtali, D. & Fabiano, C. & Palella, A. & Freni, F. & Bozzano, G. & Pino, L. & Manenti, F., 2018. "Methanol synthesis from biogas: A thermodynamic analysis," Renewable Energy, Elsevier, vol. 118(C), pages 673-684.
    4. Surita, Sharon C. & Tansel, Berrin, 2015. "Preliminary investigation to characterize deposits forming during combustion of biogas from anaerobic digesters and landfills," Renewable Energy, Elsevier, vol. 80(C), pages 674-681.
    5. Di Capua, Francesco & Spasiano, Danilo & Giordano, Andrea & Adani, Fabrizio & Fratino, Umberto & Pirozzi, Francesco & Esposito, Giovanni, 2020. "High-solid anaerobic digestion of sewage sludge: challenges and opportunities," Applied Energy, Elsevier, vol. 278(C).
    6. Rasi, S. & Seppälä, M. & Rintala, J., 2013. "Organic silicon compounds in biogases produced from grass silage, grass and maize in laboratory batch assays," Energy, Elsevier, vol. 52(C), pages 137-142.
    7. Tiwari, Prince & Wang, Tiantian & Indlekofer, Julian & El Haddad, Imad & Biollaz, Serge & Prevot, Andre Stephan Henry & Lamkaddam, Houssni, 2022. "Online detection of trace volatile organic sulfur compounds in a complex biogas mixture with proton-transfer-reaction mass spectrometry," Renewable Energy, Elsevier, vol. 196(C), pages 1197-1203.
    8. Calbry-Muzyka, Adelaide & Tarik, Mohamed & Gandiglio, Marta & Li, Jianrong & Foppiano, Debora & de Krom, Iris & Heikens, Dita & Ludwig, Christian & Biollaz, Serge, 2021. "Sampling, on-line and off-line measurement of organic silicon compounds at an industrial biogas-fed 175-kWe SOFC plant," Renewable Energy, Elsevier, vol. 177(C), pages 61-71.
    9. Paraskevi Panagiotopoulou & Christina Papadopoulou & Haris Matralis & Xenophon Verykios, 2014. "Production of renewable hydrogen by reformation of biofuels," Wiley Interdisciplinary Reviews: Energy and Environment, Wiley Blackwell, vol. 3(3), pages 231-253, May.
    10. Calbry-Muzyka, Adelaide & Madi, Hossein & Rüsch-Pfund, Florian & Gandiglio, Marta & Biollaz, Serge, 2022. "Biogas composition from agricultural sources and organic fraction of municipal solid waste," Renewable Energy, Elsevier, vol. 181(C), pages 1000-1007.
    11. Zhang, Yuyao & Kawasaki, Yu & Oshita, Kazuyuki & Takaoka, Masaki & Minami, Daisuke & Inoue, Go & Tanaka, Toshihiro, 2021. "Economic assessment of biogas purification systems for removal of both H2S and siloxane from biogas," Renewable Energy, Elsevier, vol. 168(C), pages 119-130.
    12. de Arespacochaga, N. & Valderrama, C. & Raich-Montiu, J. & Crest, M. & Mehta, S. & Cortina, J.L., 2015. "Understanding the effects of the origin, occurrence, monitoring, control, fate and removal of siloxanes on the energetic valorization of sewage biogas—A review," Renewable and Sustainable Energy Reviews, Elsevier, vol. 52(C), pages 366-381.

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