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Form-stable phase change material based on Na2CO3·10H2O-Na2HPO4·12H2O eutectic hydrated salt/expanded graphite oxide composite: The influence of chemical structures of expanded graphite oxide

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  • Liu, Yushi
  • Yang, Yingzi

Abstract

Two types of form-stable phase change materials (PCMs) were developed by impregnation of Na2CO3·10H2O-Na2HPO4·12H2O eutectic hydrated salt (EHS) into expanded graphite (EG) and expanded graphite oxide (EGO). The effects and mechanisms of chemical structures of EG and EGO on thermal properties were thoroughly discussed, in which the chemical structures were revealed by XPS, Raman spectra and XRD, and the thermal properties were assessed using the DSC analysis and thermal conductivity test. The results indicated that the EHS/EGO composite possessed higher latent heat, favorable thermal conductivity and lower supercooling degree because of the more surface oxygen-containing groups and surface defects as well as larger interlayer spacing in the EGO. Furthermore, the EHS/EGO composite remained thermally stable after 200 thermal cycles. This work will provide insights into the performance improvement of form-stable PCM composites by means of tailoring the chemical structures of porous supports.

Suggested Citation

  • Liu, Yushi & Yang, Yingzi, 2018. "Form-stable phase change material based on Na2CO3·10H2O-Na2HPO4·12H2O eutectic hydrated salt/expanded graphite oxide composite: The influence of chemical structures of expanded graphite oxide," Renewable Energy, Elsevier, vol. 115(C), pages 734-740.
    • Handle: RePEc:eee:renene:v:115:y:2018:i:c:p:734-740
    DOI: 10.1016/j.renene.2017.08.097
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    5. Honcová, Pavla & Sádovská, Galina & Pastvová, Jana & Koštál, Petr & Seidel, Jürgen & Sazama, Petr & Pilař, Radim, 2021. "Improvement of thermal energy accumulation by incorporation of carbon nanomaterial into magnesium chloride hexahydrate and magnesium nitrate hexahydrate," Renewable Energy, Elsevier, vol. 168(C), pages 1015-1026.
    6. Zhang, Suling & Wu, Wei & Wang, Shuangfeng, 2018. "Experimental investigations of Alum/expanded graphite composite phase change material for thermal energy storage and its compatibility with metals," Energy, Elsevier, vol. 161(C), pages 508-516.
    7. Wang, Yan & Sui, Jiahao & Xu, Zijie, 2022. "Preparation and characterization of CaCl2·6H2O based binary inorganic eutectic system for low temperature thermal energy storage," Energy, Elsevier, vol. 259(C).
    8. Wang, Chengjun & Liang, Weidong & Yang, Yueyue & Liu, Fang & Sun, Hanxue & Zhu, Zhaoqi & Li, An, 2020. "Biomass carbon aerogels based shape-stable phase change composites with high light-to-thermal efficiency for energy storage," Renewable Energy, Elsevier, vol. 153(C), pages 182-192.
    9. Yu, Kunyang & Liu, Yushi & Yang, Yingzi, 2021. "Review on form-stable inorganic hydrated salt phase change materials: Preparation, characterization and effect on the thermophysical properties," Applied Energy, Elsevier, vol. 292(C).
    10. Lin, Yaxue & Alva, Guruprasad & Fang, Guiyin, 2018. "Review on thermal performances and applications of thermal energy storage systems with inorganic phase change materials," Energy, Elsevier, vol. 165(PA), pages 685-708.
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