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Mitigation of ultrafine particulate matter emission from agricultural biomass pellet combustion by the additive of phosphoric acid modified kaolin

Author

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  • Cheng, Wei
  • Zhu, Youjian
  • Shao, Jing’ai
  • Zhang, Wennan
  • Wu, Guihao
  • Jiang, Hao
  • Hu, Junhao
  • Huang, Zhen
  • Yang, Haiping
  • Chen, Hanping

Abstract

The emission of ultrafine particulate matter (PM0.2) originated from the agricultural biomass pellet combustion poses great threat to atmospheric environment and human health, which restricts its large-scale utilization. In this study, a new phosphoric acid modification method is proposed to improve the PM0.2 reduction efficiency by kaolin additive. The effects of phosphoric acid concentration and treatment time on the physicochemical properties of kaolin and on the mitigation of PM0.2 emission from the pellet combustion are investigated. Results indicate that phosphoric acid modification destroy the internal structure of kaolin by the leaching of Al cations and the formation of active free silica. Meanwhile, the pore structure increases after modification with residual P deposited on the surface, which results in better alkali capture ability of modified kaolin. With the addition of phosphoric acid modified kaolin, significant reduction of PM0.2 emission can be achieved and the reduction ratio is proportional to the acid concentration. The maximum PM0.2 emission reduction ratio reaches 64.5% for the kaolin additive modified by 12 mol/L phosphoric acid for 6 hours. Finally, the PM0.2 reduction mechanism is proposed based on the analysis results, which provides technical knowhow for the industrial application of agricultural biomass pellet combustion.

Suggested Citation

  • Cheng, Wei & Zhu, Youjian & Shao, Jing’ai & Zhang, Wennan & Wu, Guihao & Jiang, Hao & Hu, Junhao & Huang, Zhen & Yang, Haiping & Chen, Hanping, 2021. "Mitigation of ultrafine particulate matter emission from agricultural biomass pellet combustion by the additive of phosphoric acid modified kaolin," Renewable Energy, Elsevier, vol. 172(C), pages 177-187.
    • Handle: RePEc:eee:renene:v:172:y:2021:i:c:p:177-187
    DOI: 10.1016/j.renene.2021.03.041
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    3. Cheng, Wei & Shao, Jing'ai & Zhu, Youjian & Zhang, Wennan & Jiang, Hao & Hu, Junhao & Zhang, Xiong & Yang, Haiping & Chen, Hanping, 2022. "Effect of oxidative torrefaction on particulate matter emission from agricultural biomass pellet combustion in comparison with non-oxidative torrefaction," Renewable Energy, Elsevier, vol. 189(C), pages 39-51.
    4. Nataša Dragutinović & Isabel Höfer & Martin Kaltschmitt, 2021. "Fuel Improvement Measures for Particulate Matter Emission Reduction during Corn Cob Combustion," Energies, MDPI, vol. 14(15), pages 1-23, July.
    5. Li, Yu & Tan, Zhiwu & Zhu, Youjian & Zhang, Wennan & Du, Zhenyi & Shao, Jingai & Jiang, Long & Yang, Haiping & Chen, Hanping, 2022. "Effects of P-based additives on agricultural biomass torrefaction and particulate matter emissions from fuel combustion," Renewable Energy, Elsevier, vol. 190(C), pages 66-77.
    6. Fu, Jie & Mao, Xiao & Siyal, Asif Ali & Liu, Yang & Ao, Wenya & Liu, Guangqing & Dai, Jianjun, 2021. "Pyrolysis of furfural residue pellets: Physicochemical characteristics of pyrolytic pellets and pyrolysis kinetics," Renewable Energy, Elsevier, vol. 179(C), pages 2136-2146.

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