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Mineral carbonation of flue gas desulfurization gypsum for CO2 sequestration

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  • Lee, Myung gyu
  • Jang, Young Nam
  • Ryu, Kyung won
  • Kim, Wonbeak
  • Bang, Jun-Hwan

Abstract

In this study, the technical feasibility of the mineral carbonation of flue gas desulfurization (FGD) gypsum to sequester CO2 was assessed by considering various reaction parameters. Unlike other natural and industrial materials, FGD gypsum showed very high carbonation reactivity at room temperature and atmospheric pressure. Under optimum conditions, calcium carbonate with a purity exceeding 90% could be obtained within 10 min at a carbonation rate of approximately 95%. Thus, mineral carbonation of FGD gypsum was found to be technically feasible.

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  • Lee, Myung gyu & Jang, Young Nam & Ryu, Kyung won & Kim, Wonbeak & Bang, Jun-Hwan, 2012. "Mineral carbonation of flue gas desulfurization gypsum for CO2 sequestration," Energy, Elsevier, vol. 47(1), pages 370-377.
    • Handle: RePEc:eee:energy:v:47:y:2012:i:1:p:370-377
    DOI: 10.1016/j.energy.2012.09.009
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    Cited by:

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    2. Chen, Xiaoyi & Jin, Xiaogang & Liu, Zhimin & Ling, Xiang & Wang, Yan, 2018. "Experimental investigation on the CaO/CaCO3 thermochemical energy storage with SiO2 doping," Energy, Elsevier, vol. 155(C), pages 128-138.
    3. Zhao, Zhongzhong & Liu, Wenhuan & Jiang, Yiwen & Li, Hui, 2023. "Enhancement mechanisms of spherical UFA on CO2 capture of waste slag," Energy, Elsevier, vol. 269(C).
    4. Khosa, Azhar Abbas & Yan, J. & Zhao, C.Y., 2021. "Investigating the effects of ZnO dopant on the thermodynamic and kinetic properties of CaCO3/CaO TCES system," Energy, Elsevier, vol. 215(PA).
    5. Song, Kyungsun & Jang, Young-Nam & Kim, Wonbaek & Lee, Myung Gyu & Shin, Dongbok & Bang, Jun-Hwan & Jeon, Chi Wan & Chae, Soo Chun, 2014. "Factors affecting the precipitation of pure calcium carbonate during the direct aqueous carbonation of flue gas desulfurization gypsum," Energy, Elsevier, vol. 65(C), pages 527-532.
    6. Gu, Hui & Cui, Yanfeng & Zhu, Hongxia & Xue, Rui & Si, Fengqi, 2018. "A new approach for clustering in desulfurization system based on modified framework for gypsum slurry quality monitoring," Energy, Elsevier, vol. 148(C), pages 789-801.
    7. Córdoba, Patricia & Ayora, Carlos & Moreno, Natalia & Font, Oriol & Izquierdo, Maria & Querol, Xavier, 2013. "Influence of an aluminium additive in aqueous and solid speciation of elements in flue gas desulphurisation (FGD) system," Energy, Elsevier, vol. 50(C), pages 438-444.
    8. Ukwattage, N.L. & Ranjith, P.G. & Wang, S.H., 2013. "Investigation of the potential of coal combustion fly ash for mineral sequestration of CO2 by accelerated carbonation," Energy, Elsevier, vol. 52(C), pages 230-236.
    9. Lombardi, Lidia & Carnevale, Ennio, 2013. "Economic evaluations of an innovative biogas upgrading method with CO2 storage," Energy, Elsevier, vol. 62(C), pages 88-94.

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