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Optimization of carbon dioxide capture and storage with mineralisation using recyclable ammonium salts

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  • Wang, Xiaolong
  • Maroto-Valer, M. Mercedes

Abstract

Optimization of CCSM (carbon dioxide capture and storage with mineralisation) using RAS (recyclable ammonium salts) was studied here in order to minimize the energy consumption of this process. Water evaporation is required for the recycling of ammonium salts in the process, however the water evaporation technologies normally impose high energy penalty. In the optimized process, solid to liquid (S/L) ratio was increased to reduce water usage, but this change impacts dissolution efficiency, where the dissolution efficiency decreased from 100% at S/L of 50 g/l to 71% at S/L of 300 g/l. However, a 6% increase of dissolution efficiency was reported when the S/L ratio increased from 200 g/l to 300 g/l, probably due to increasing mineral inter-collisions. Besides, the optimized process employed the pressurized reactor, this change resulted in the mineral phase of product changed from hydromagnesite to magnesite. The carbon fixation efficiency was significantly improved by using (NH4)2CO3 compared to NH4HCO3, and the highest CO2 fixation efficiency achieved was 46.6% at S/L of 300 g/l. The mass balance for the optimized process was 4.9 t of serpentine, 0.6 t of NH4HSO4, 4.7 t of (NH4)2CO3 and 16 t of water required to sequester 1 t CO2.

Suggested Citation

  • Wang, Xiaolong & Maroto-Valer, M. Mercedes, 2013. "Optimization of carbon dioxide capture and storage with mineralisation using recyclable ammonium salts," Energy, Elsevier, vol. 51(C), pages 431-438.
    • Handle: RePEc:eee:energy:v:51:y:2013:i:c:p:431-438
    DOI: 10.1016/j.energy.2013.01.021
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    1. Bernard Jomari B. Razote & Mark Kenneth M. Maranan & Ramon Christian P. Eusebio & Richard D. Alorro & Arnel B. Beltran & Aileen H. Orbecido, 2019. "Determination of the Carbon Dioxide Sequestration Potential of a Nickel Mine Mixed Dump through Leaching Tests," Energies, MDPI, vol. 12(15), pages 1-19, July.
    2. Baena-Moreno, Francisco M. & Rodríguez-Galán, Mónica & Vega, Fernando & Reina, T.R. & Vilches, Luis F. & Navarrete, Benito, 2019. "Converting CO2 from biogas and MgCl2 residues into valuable magnesium carbonate: A novel strategy for renewable energy production," Energy, Elsevier, vol. 180(C), pages 457-464.
    3. Cheng Cao & Hejuan Liu & Zhengmeng Hou & Faisal Mehmood & Jianxing Liao & Wentao Feng, 2020. "A Review of CO 2 Storage in View of Safety and Cost-Effectiveness," Energies, MDPI, vol. 13(3), pages 1-45, January.
    4. Xiaolong Wang & Aimaro Sanna & M. Mercedes Maroto‐Valer & Tom Paulson, 2015. "Carbon dioxide capture and storage by pH swing mineralization using recyclable ammonium salts and flue gas mixtures," Greenhouse Gases: Science and Technology, Blackwell Publishing, vol. 5(4), pages 389-402, August.
    5. Jun-Hwan Bang & Seung-Woo Lee & Chiwan Jeon & Sangwon Park & Kyungsun Song & Whan Joo Jo & Soochun Chae, 2016. "Leaching of Metal Ions from Blast Furnace Slag by Using Aqua Regia for CO 2 Mineralization," Energies, MDPI, vol. 9(12), pages 1-13, November.
    6. Dri, Marco & Sanna, Aimaro & Maroto-Valer, M. Mercedes, 2014. "Mineral carbonation from metal wastes: Effect of solid to liquid ratio on the efficiency and characterization of carbonated products," Applied Energy, Elsevier, vol. 113(C), pages 515-523.
    7. Lombardi, L. & Carnevale, E.A., 2016. "Analysis of an innovative process for landfill gas quality improvement," Energy, Elsevier, vol. 109(C), pages 1107-1117.
    8. Leung, Dennis Y.C. & Caramanna, Giorgio & Maroto-Valer, M. Mercedes, 2014. "An overview of current status of carbon dioxide capture and storage technologies," Renewable and Sustainable Energy Reviews, Elsevier, vol. 39(C), pages 426-443.
    9. Park, Sangwon & Song, Kyungsun & Jo, Hwanju, 2017. "Laboratory-scale experiment on a novel mineralization-based method of CO2 capture using alkaline solution," Energy, Elsevier, vol. 124(C), pages 589-598.
    10. Ji, Long & Yu, Hai & Li, Kangkang & Yu, Bing & Grigore, Mihaela & Yang, Qi & Wang, Xiaolong & Chen, Zuliang & Zeng, Ming & Zhao, Shuaifei, 2018. "Integrated absorption-mineralisation for low-energy CO2 capture and sequestration," Applied Energy, Elsevier, vol. 225(C), pages 356-366.
    11. Natália R. Galina & Gretta L. A. F. Arce & Mercedes Maroto-Valer & Ivonete Ávila, 2023. "Experimental Study on Mineral Dissolution and Carbonation Efficiency Applied to pH-Swing Mineral Carbonation for Improved CO 2 Sequestration," Energies, MDPI, vol. 16(5), pages 1-19, March.
    12. Zevenhoven, Ron & Slotte, Martin & Åbacka, Jacob & Highfield, James, 2016. "A comparison of CO2 mineral sequestration processes involving a dry or wet carbonation step," Energy, Elsevier, vol. 117(P2), pages 604-611.
    13. Hosseini, Tahereh & Haque, Nawshad & Selomulya, Cordelia & Zhang, Lian, 2016. "Mineral carbonation of Victorian brown coal fly ash using regenerative ammonium chloride – Process simulation and techno-economic analysis," Applied Energy, Elsevier, vol. 175(C), pages 54-68.

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