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Carbon dioxide capture and storage by pH swing mineralization using recyclable ammonium salts and flue gas mixtures

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  • Xiaolong Wang
  • Aimaro Sanna
  • M. Mercedes Maroto‐Valer
  • Tom Paulson

Abstract

CO 2 mineral sequestration through the employment of silicate rocks such as serpentine is an important technology for the mitigation of CO 2 emissions. Most mineral carbonation works in this study use pure CO 2 . The indirect carbonation process employed different flue gases (5, 15, 25% CO 2 ) and the presence of SOx and NOx. Also, the direct contact of CO 2 with the Mg source was compared to the indirect reaction of Mg with CO 2 as NH 4 CO 3 . The impact of variables such as temperature, solid‐liquid ration (S/L), and molar ratio of additives on carbonation rate and degree was studied. An average carbonation efficiency of about 90% was achieved at 80°C after 30 min for indirect mineral carbonation process. The carbonation efficiency decreased to 50‒60% when the process was directly employed. The carbonation efficiency obtained in the presence of 15‒25% CO 2 was very similar to that with 100% CO 2 at 140°C, while at 80°C, the carbonation efficiency in presence of flue gas (40‒55%) was much larger compared to that using pure C0 2 (10% after 3 h). SOx and NOx co‐removal efficiency was 54.4% and 18% at 140˚C and 20 bar, respectively.

Suggested Citation

  • Xiaolong Wang & Aimaro Sanna & M. Mercedes Maroto‐Valer & Tom Paulson, 2015. "Carbon dioxide capture and storage by pH swing mineralization using recyclable ammonium salts and flue gas mixtures," Greenhouse Gases: Science and Technology, Blackwell Publishing, vol. 5(4), pages 389-402, August.
    • Handle: RePEc:wly:greenh:v:5:y:2015:i:4:p:389-402
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    File URL: http://hdl.handle.net/10.1002/ghg.1494
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    References listed on IDEAS

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    1. Wang, Xiaolong & Maroto-Valer, M. Mercedes, 2013. "Optimization of carbon dioxide capture and storage with mineralisation using recyclable ammonium salts," Energy, Elsevier, vol. 51(C), pages 431-438.
    2. Teir, Sebastian & Eloneva, Sanni & Fogelholm, Carl-Johan & Zevenhoven, Ron, 2007. "Dissolution of steelmaking slags in acetic acid for precipitated calcium carbonate production," Energy, Elsevier, vol. 32(4), pages 528-539.
    3. Lackner, Klaus S. & Wendt, Christopher H. & Butt, Darryl P. & Joyce, Edward L. & Sharp, David H., 1995. "Carbon dioxide disposal in carbonate minerals," Energy, Elsevier, vol. 20(11), pages 1153-1170.
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