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Influence of process parameters on carbonation rate and conversion of steelmaking slags – Introduction of the ‘carbonation weathering rate’

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  • Evangelos Georgakopoulos
  • Rafael M. Santos
  • Yi Wai Chiang
  • Vasilije Manovic

Abstract

Alkaline industrial wastes are considered potential resources for the mitigation of CO 2 emissions by simultaneously capturing and sequestering CO 2 through mineralization. Mineralization safely and permanently stores CO 2 through its reaction with alkaline earth metals. These elements are found in a variety of abundantly available industrial wastes that have high reactivity with CO 2 , and that are generated close to the emission point‐sources. Among all suitable industrial wastes, steelmaking slag has been deemed the most promising given its high CO 2 uptake potential. In this paper, we review recent publications related to the influence of process parameters on the carbonation rate and conversion extent of steelmaking slags, comparing and analyzing them in order to define the present state of the art. Furthermore, the maximum conversions resulting from different studies are directly compared using a new index, the Carbonation Weathering Rate (CWR), which normalizes the results based on particle size and reaction duration. To date, the carbonation of Basic Oxygen Furnace steelmaking slag, under mild conditions, presents both the highest carbonation conversion and CWR, with values equal to 93.5% and 0.62 μm/min, respectively. © 2016 Society of Chemical Industry and John Wiley & Sons, Ltd

Suggested Citation

  • Evangelos Georgakopoulos & Rafael M. Santos & Yi Wai Chiang & Vasilije Manovic, 2016. "Influence of process parameters on carbonation rate and conversion of steelmaking slags – Introduction of the ‘carbonation weathering rate’," Greenhouse Gases: Science and Technology, Blackwell Publishing, vol. 6(4), pages 470-491, August.
    • Handle: RePEc:wly:greenh:v:6:y:2016:i:4:p:470-491
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    File URL: http://hdl.handle.net/10.1002/ghg.1608
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    1. Zhang, Zhien & Pan, Shu-Yuan & Li, Hao & Cai, Jianchao & Olabi, Abdul Ghani & Anthony, Edward John & Manovic, Vasilije, 2020. "Recent advances in carbon dioxide utilization," Renewable and Sustainable Energy Reviews, Elsevier, vol. 125(C).

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