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Solid oxide fuel cell operation with biomass gasification product gases: Performance- and carbon deposition risk evaluation via a CFD modelling approach

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  • Pongratz, Gernot
  • Subotić, Vanja
  • Hochenauer, Christoph
  • Scharler, Robert
  • Anca-Couce, Andrés

Abstract

Solid oxide fuel cell (SOFC) models used in the past for biomass-to-power plant simulations are limited in their predictability of the carbon deposition risk. In this work, industrial-relevant cell designs were modeled in 2D-CFD considering detailed reaction kinetics which allowed more accurate performance simulations and carbon deposition risk assessments. Via a parametric study, the influence of varying cell operating conditions on the cell performance and carbon deposition risk was quantified when utilizing product gases from steam- and air gasification with varying steam addition. Considering the results from this parameter study and carbon deposition risk assessment, recommendations for promising gasifier-SOFC configurations and cell operating points for stable long-term operation are presented. For smaller-scale biomass-to-power systems, the utilization of product gas from air gasification in anode supported cells with Ni/zirconia-based anode can be recommended, with only moderate steam dilution of the product gas at 750°C cell operating temperature. For larger scales, steam gasification might be meaningful, offering a generally higher electrical efficiency and power output in fuel cells than air gasification. However, a higher risk for carbon deposition could be determined in comparison to air gasification. Hence, a cell temperature of 850°C besides the use of cells with Ni/ceria-based anodes is recommended.

Suggested Citation

  • Pongratz, Gernot & Subotić, Vanja & Hochenauer, Christoph & Scharler, Robert & Anca-Couce, Andrés, 2022. "Solid oxide fuel cell operation with biomass gasification product gases: Performance- and carbon deposition risk evaluation via a CFD modelling approach," Energy, Elsevier, vol. 244(PB).
    • Handle: RePEc:eee:energy:v:244:y:2022:i:pb:s036054422103334x
    DOI: 10.1016/j.energy.2021.123085
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