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Low carbon fuel production from combined solid oxide CO2 co-electrolysis and Fischer-Tropsch synthesis system: A modelling study

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  • Xu, Haoran
  • Maroto-Valer, M. Mercedes
  • Ni, Meng
  • Cao, Jun
  • Xuan, Jin

Abstract

CH4-assisted solid oxide electrolyzer cells (SOECs) can co-electrolyze H2O and CO2 effectively for simultaneous energy storage and CO2 utilization. Compared with conventional SOECs, CH4-assisted SOECs consume less electricity because CH4 in the anode provides part of the energy for electrolysis. As syngas (CO and H2 mixture) is generated from the co-electrolysis process, it is necessary to study its utilization through the subsequent processes, such as Fischer-Tropsch (F-T) synthesis to produce more value-added products. An F-T reactor can convert syngas into hydrocarbons, and thus it is very suitable for the utilization of syngas. In this paper, the combined CH4-assisted SOEC and F-T synthesis system is numerically studied. Validated 2D models for CH4-assisted SOEC and F-T processes are adopted for parametric studies. It is found that the cathode inlet H2O/CO2 ratio in the SOEC significantly affects the production components through the F-T process. Other operating parameters such as the operating temperature and applied voltage of the SOEC are found to greatly affect the productions of the system. This model is important for understanding and design optimization of the combined fuel-assisted SOEC and F-T synthesis system to achieve economical hydrocarbon generation.

Suggested Citation

  • Xu, Haoran & Maroto-Valer, M. Mercedes & Ni, Meng & Cao, Jun & Xuan, Jin, 2019. "Low carbon fuel production from combined solid oxide CO2 co-electrolysis and Fischer-Tropsch synthesis system: A modelling study," Applied Energy, Elsevier, vol. 242(C), pages 911-918.
    • Handle: RePEc:eee:appene:v:242:y:2019:i:c:p:911-918
    DOI: 10.1016/j.apenergy.2019.03.145
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    References listed on IDEAS

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    1. Choe, Changgwon & Cheon, Seunghyun & Gu, Jiwon & Lim, Hankwon, 2022. "Critical aspect of renewable syngas production for power-to-fuel via solid oxide electrolysis: Integrative assessment for potential renewable energy source," Renewable and Sustainable Energy Reviews, Elsevier, vol. 161(C).
    2. Lu, Lianmei & Liu, Wu & Wang, Jianxin & Wang, Yudong & Xia, Changrong & Zhou, Xiao-Dong & Chen, Ming & Guan, Wanbing, 2020. "Long-term stability of carbon dioxide electrolysis in a large-scale flat-tube solid oxide electrolysis cell based on double-sided air electrodes," Applied Energy, Elsevier, vol. 259(C).
    3. Sun, Yi & Qian, Tang & Zhu, Jingdong & Zheng, Nan & Han, Yu & Xiao, Gang & Ni, Meng & Xu, Haoran, 2023. "Dynamic simulation of a reversible solid oxide cell system for efficient H2 production and power generation," Energy, Elsevier, vol. 263(PA).

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