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Dynamic electro-thermal modeling of co-electrolysis of steam and carbon dioxide in a tubular solid oxide electrolysis cell

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  • Luo, Yu
  • Shi, Yixiang
  • Li, Wenying
  • Cai, Ningsheng

Abstract

SOEC (Solid oxide electrolysis cell) has great potential to store unstable renewable energy in form of steady chemical energy. For this application, transient behavior in variable working condition is crucial. A 2D (two-dimensional) dynamic model was developed to predict the dynamic response of H2O/CO2 co-electrolysis in TSOEC (tubular solid oxide electrolysis cell). The dynamic model comprehensively considered the macroscopic fluid flow, microscopic diffusion, heat transfer and electrochemical/chemical reactions in the TSOEC. In this paper, the TNV (thermal neutral voltage) of TSOEC was specifically defined and calculated. The time constants of charge/mass/heat transport processes were evaluated. Further, the responses of current, gas concentrations, temperature, efficiency, conversions to electricity/gas flow/temperature step inputs were respectively studied. Through the study, appropriate transient operations were designed to improve efficiency and conversions.

Suggested Citation

  • Luo, Yu & Shi, Yixiang & Li, Wenying & Cai, Ningsheng, 2015. "Dynamic electro-thermal modeling of co-electrolysis of steam and carbon dioxide in a tubular solid oxide electrolysis cell," Energy, Elsevier, vol. 89(C), pages 637-647.
    • Handle: RePEc:eee:energy:v:89:y:2015:i:c:p:637-647
    DOI: 10.1016/j.energy.2015.05.150
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    6. Li, Yongwei & Fu, Zaiguo & Li, Jingfa & Shao, Yan & Zhu, Qunzhi & Yuan, Binxia, 2024. "Effects of structural parameters of double-layer electrode on co-electrolysis in a solid oxide electrolysis cell," Energy, Elsevier, vol. 287(C).
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    8. Xiao, Gang & Sun, Anwei & Liu, Hongwei & Ni, Meng & Xu, Haoran, 2023. "Thermal management of reversible solid oxide cells in the dynamic mode switching," Applied Energy, Elsevier, vol. 331(C).
    9. Luo, Yu & Shi, Yixiang & Zheng, Yi & Gang, Zhongxue & Cai, Ningsheng, 2017. "Mutual information for evaluating renewable power penetration impacts in a distributed generation system," Energy, Elsevier, vol. 141(C), pages 290-303.
    10. Zhaojian Liang & Jingyi Wang & Keda Ren & Zhenjun Jiao & Meng Ni & Liang An & Yang Wang & Jinbin Yang & Mengying Li, 2024. "Discovering two general characteristic times of transient responses in solid oxide cells," Nature Communications, Nature, vol. 15(1), pages 1-12, December.
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