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Feasibility study of the use of by-product iron oxide and industrial off-gas for application to chemical looping hydrogen production

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  • Cho, Won Chul
  • Lee, Doyeon
  • Kim, Chang Hee
  • Cho, Hyun Suk
  • Kim, Sang Done

Abstract

The chemical looping strategy for hydrogen production (CLH2) offers a potentially viable option for efficient fuel conversion to hydrogen with the simultaneous capture of CO2. Typically, this process uses an iron-based composite as an oxygen carrier and syngas or methane as a fuel. The environmental and economic concerns motivate the use of abundant by-product iron oxide and the industrial off-gas for CLH2. Here we showed that H2 could be simply recovered from the industrial off-gas in a circulating fluidized bed with a mixture of the inexpensive raw material of by-product iron oxide and sand particle. The fluidization of the by-product iron oxide powder, which showed poor fluidization behavior, is improved by adding 60 vol% of sand particle. The industrial off-gas was completely converted to CO2 and H2O in a two-stage fluidized mode with a solid reactant of Fe2O3 of the binary particles, and then H2 was produced by oxidizing the reduced by-product iron oxide powder with steam. The binary particles showed consistent catalytic activity under multiple redox cycles by providing macropores with a size of ∼5 μm which facilitated gas diffusion. These findings provided valuable information for the future development of CLH2 based on by-products.

Suggested Citation

  • Cho, Won Chul & Lee, Doyeon & Kim, Chang Hee & Cho, Hyun Suk & Kim, Sang Done, 2018. "Feasibility study of the use of by-product iron oxide and industrial off-gas for application to chemical looping hydrogen production," Applied Energy, Elsevier, vol. 216(C), pages 466-481.
    • Handle: RePEc:eee:appene:v:216:y:2018:i:c:p:466-481
    DOI: 10.1016/j.apenergy.2018.02.078
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    References listed on IDEAS

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    Cited by:

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    4. Song, Weiming & Huang, Yifeng & Chen, Xiaoqing & Jiang, Rui & Li, Yujie & Zhou, Jianan, 2023. "CO2 gasification of dry quenching dust ash catalyzed in situ by soot," Renewable Energy, Elsevier, vol. 211(C), pages 595-606.
    5. Xiang, Dong & Zhou, Yunpeng, 2018. "Concept design and techno-economic performance of hydrogen and ammonia co-generation by coke-oven gas-pressure swing adsorption integrated with chemical looping hydrogen process," Applied Energy, Elsevier, vol. 229(C), pages 1024-1034.
    6. Xiang, Dong & Huang, Weiqing & Huang, Peng, 2018. "A novel coke-oven gas-to-natural gas and hydrogen process by integrating chemical looping hydrogen with methanation," Energy, Elsevier, vol. 165(PB), pages 1024-1033.
    7. Song, Weiming & Zhou, Jianan & Li, Yujie & Yang, Jian & Cheng, Rijin, 2021. "New technology for producing high-quality combustible gas by high-temperature reaction of dust-removal coke powder in mixed atmosphere," Energy, Elsevier, vol. 233(C).
    8. Yáñez, María & Ortiz, Alfredo & Brunaud, Braulio & Grossmann, Ignacio E. & Ortiz, Inmaculada, 2018. "Contribution of upcycling surplus hydrogen to design a sustainable supply chain: The case study of Northern Spain," Applied Energy, Elsevier, vol. 231(C), pages 777-787.

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