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Experimental study on the performance of hydrogen production from miniature methanol–steam reformer integrated with Swiss-roll type combustor for PEMFC

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  • Chein, Rei-Yu
  • Chen, Yen-Cho
  • Chang, Che-Ming
  • Chung, J.N.

Abstract

A miniature plate-type hydrogen production reactor using methanol as fuel was designed and tested. This reactor is composed of a catalytic combustor, vaporizer, reformer, and methanator. All components were fabricated on one piece of rectangular quartz glass plate 50mm×44mm×7mm in size. The combustor was fabricated on one side of the glass plate with a Swiss-roll type channel in which the Pt/Al2O3 particles were loaded in segmented form to catalyze the combustion. A spiral channel was fabricated on the other side of the plate and divided into three sections: a vaporizer for liquid methanol–water mixture vaporization, a reformer for methanol–steam reforming catalyzed by CuO/ZnO/Al2O3 particles and a methanator for carbon monoxide (CO) removal catalyzed by Ru/Al2O3 particles.

Suggested Citation

  • Chein, Rei-Yu & Chen, Yen-Cho & Chang, Che-Ming & Chung, J.N., 2013. "Experimental study on the performance of hydrogen production from miniature methanol–steam reformer integrated with Swiss-roll type combustor for PEMFC," Applied Energy, Elsevier, vol. 105(C), pages 86-98.
    • Handle: RePEc:eee:appene:v:105:y:2013:i:c:p:86-98
    DOI: 10.1016/j.apenergy.2012.12.040
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    References listed on IDEAS

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    1. Shirsat, V. & Gupta, A.K., 2011. "A review of progress in heat recirculating meso-scale combustors," Applied Energy, Elsevier, vol. 88(12), pages 4294-4309.
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    1. Perng, Shiang-Wuu & Horng, Rong-Fang & Wu, Horng-Wen, 2017. "Effect of a diffuser on performance enhancement of a cylindrical methanol steam reformer by computational fluid dynamic analysis," Applied Energy, Elsevier, vol. 206(C), pages 312-328.
    2. Jaggi, Vikas & Jayanti, S., 2013. "A conceptual model of a high-efficiency, stand-alone power unit based on a fuel cell stack with an integrated auto-thermal ethanol reformer," Applied Energy, Elsevier, vol. 110(C), pages 295-303.
    3. Chen, Wei-Hsin & Guo, Yu-Zhi & Chen, Chih-Chun, 2018. "Methanol partial oxidation accompanied by heat recirculation in a Swiss-roll reactor," Applied Energy, Elsevier, vol. 232(C), pages 79-88.
    4. Ribeirinha, P. & Abdollahzadeh, M. & Sousa, J.M. & Boaventura, M. & Mendes, A., 2017. "Modelling of a high-temperature polymer electrolyte membrane fuel cell integrated with a methanol steam reformer cell," Applied Energy, Elsevier, vol. 202(C), pages 6-19.
    5. Wang, Yancheng & Liu, Haiyu & Mei, Deqing & Yu, Shizheng, 2022. "Direct ink writing of 3D SiC scaffold as catalyst support for thermally autonomous methanol steam reforming microreactor," Renewable Energy, Elsevier, vol. 187(C), pages 923-932.
    6. Chen, Wei-Hsin & Chen, Chia-Yang, 2020. "Water gas shift reaction for hydrogen production and carbon dioxide capture: A review," Applied Energy, Elsevier, vol. 258(C).
    7. Lu, Buchu & Yan, Xiangyu & Liu, Qibin, 2023. "Enhanced solar hydrogen generation with the direct coupling of photo and thermal energy – An experimental and mechanism study," Applied Energy, Elsevier, vol. 331(C).
    8. Ribeirinha, P. & Abdollahzadeh, M. & Pereira, A. & Relvas, F. & Boaventura, M. & Mendes, A., 2018. "High temperature PEM fuel cell integrated with a cellular membrane methanol steam reformer: Experimental and modelling," Applied Energy, Elsevier, vol. 215(C), pages 659-669.
    9. Ribeirinha, P. & Abdollahzadeh, M. & Boaventura, M. & Mendes, A., 2017. "H2 production with low carbon content via MSR in packed bed membrane reactors for high-temperature polymeric electrolyte membrane fuel cell," Applied Energy, Elsevier, vol. 188(C), pages 409-419.
    10. Cheng, Chin-Hsiang & Huang, Yu-Xian & King, Shun-Chih & Lee, Chun-I & Leu, Chih-Hsing, 2014. "CFD (computational fluid dynamics)-based optimal design of a micro-reformer by integrating computational a fluid dynamics code using a simplified conjugate-gradient method," Energy, Elsevier, vol. 70(C), pages 355-365.
    11. Pourali, Mostafa & Esfahani, Javad Abolfazli, 2022. "Performance analysis of a micro-scale integrated hydrogen production system by analytical approach, machine learning, and response surface methodology," Energy, Elsevier, vol. 255(C).
    12. Liu, Yangxu & Zhou, Wei & Lin, Yu & Chen, Lu & Chu, Xuyang & Zheng, Tianqing & Wan, Shaolong & Lin, Jingdong, 2019. "Novel copper foam with ordered hole arrays as catalyst support for methanol steam reforming microreactor," Applied Energy, Elsevier, vol. 246(C), pages 24-37.
    13. Perng, Shiang-Wuu & Wu, Horng-Wen, 2022. "Influence of inlet-nozzle and outlet-diffuser mounted in the plate-shape reactor on PEMFC net power output and methanol steam reforming performance," Applied Energy, Elsevier, vol. 323(C).
    14. Mohammed Abbas, Akhtar Hasnain & Cheralathan, Kanakkampalayam Krishnan & Porpatham, Ekambaram & Arumugam, Senthil Kumar, 2024. "Hydrogen generation using methanol steam reforming – catalysts, reactors, and thermo-chemical recuperation," Renewable and Sustainable Energy Reviews, Elsevier, vol. 191(C).
    15. Wang, Qing-Hui & Yang, Song & Zhou, Wei & Li, Jing-Rong & Xu, Zhi-Jia & Ke, Yu-Zhi & Yu, Wei & Hu, Guang-Hua, 2018. "Optimizing the porosity configuration of porous copper fiber sintered felt for methanol steam reforming micro-reactor based on flow distribution," Applied Energy, Elsevier, vol. 216(C), pages 243-261.
    16. Kim, Taegyu & Jo, Sungkwon & Song, Young-Hoon & Lee, Dae Hoon, 2014. "Synergetic mechanism of methanol–steam reforming reaction in a catalytic reactor with electric discharges," Applied Energy, Elsevier, vol. 113(C), pages 1692-1699.

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