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Robust consistent single quantum dot strong coupling in plasmonic nanocavities

Author

Listed:
  • Shu Hu

    (University of Cambridge
    Xiamen University)

  • Junyang Huang

    (University of Cambridge)

  • Rakesh Arul

    (University of Cambridge)

  • Ana Sánchez-Iglesias

    (Basque Research and Technology Alliance (BRTA))

  • Yuling Xiong

    (University of Cambridge)

  • Luis M. Liz-Marzán

    (Basque Research and Technology Alliance (BRTA)
    Ikerbasque, Basque Foundation for Science)

  • Jeremy J. Baumberg

    (University of Cambridge)

Abstract

Strong coupling between a single quantum emitter and an optical cavity (at rate Ω) accesses fundamental quantum optics and provides an essential building block for photonic quantum technologies. However, the minimum mode volume of conventional dielectric cavities restricts their operation to cryogenic temperature for strong coupling. Here we harness surface self-assembly to make deterministic strong coupling at room temperature using CdSe/CdS quantum dots (QDs) in nanoparticle-on-mirror (NPoM) plasmonic nanocavities. We achieve a fabrication yield of ~70% for single QD strong coupling by optimizing their size and nano-assembly. A clear and reliable Rabi splitting is observed both in the scattering of each nanocavity and their photoluminescence, which are however not equal. Integrating these quantum elements with electrical pumping allows demonstration of strong coupling in their electroluminescence. This advance provides a straightforward way to achieve practical quantum devices at room temperature, and opens up exploration of their nonlinear, electrical, and quantum correlation properties.

Suggested Citation

  • Shu Hu & Junyang Huang & Rakesh Arul & Ana Sánchez-Iglesias & Yuling Xiong & Luis M. Liz-Marzán & Jeremy J. Baumberg, 2024. "Robust consistent single quantum dot strong coupling in plasmonic nanocavities," Nature Communications, Nature, vol. 15(1), pages 1-8, December.
    • Handle: RePEc:nat:natcom:v:15:y:2024:i:1:d:10.1038_s41467-024-51170-7
    DOI: 10.1038/s41467-024-51170-7
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    as
    1. Oluwafemi S. Ojambati & Rohit Chikkaraddy & William D. Deacon & Matthew Horton & Dean Kos & Vladimir A. Turek & Ulrich F. Keyser & Jeremy J. Baumberg, 2019. "Quantum electrodynamics at room temperature coupling a single vibrating molecule with a plasmonic nanocavity," Nature Communications, Nature, vol. 10(1), pages 1-7, December.
    2. Kotni Santhosh & Ora Bitton & Lev Chuntonov & Gilad Haran, 2016. "Vacuum Rabi splitting in a plasmonic cavity at the single quantum emitter limit," Nature Communications, Nature, vol. 7(1), pages 1-5, September.
    3. Dandan Ge & Sylvie Marguet & Ali Issa & Safi Jradi & Tien Hoa Nguyen & Mackrine Nahra & Jéremie Béal & Régis Deturche & Hongshi Chen & Sylvain Blaize & Jérôme Plain & Céline Fiorini & Ludovic Douillar, 2020. "Hybrid plasmonic nano-emitters with controlled single quantum emitter positioning on the local excitation field," Nature Communications, Nature, vol. 11(1), pages 1-11, December.
    4. Daniel Najer & Immo Söllner & Pavel Sekatski & Vincent Dolique & Matthias C. Löbl & Daniel Riedel & Rüdiger Schott & Sebastian Starosielec & Sascha R. Valentin & Andreas D. Wieck & Nicolas Sangouard &, 2019. "A gated quantum dot strongly coupled to an optical microcavity," Nature, Nature, vol. 575(7784), pages 622-627, November.
    5. Thang B. Hoang & Gleb M. Akselrod & Christos Argyropoulos & Jiani Huang & David R. Smith & Maiken H. Mikkelsen, 2015. "Ultrafast spontaneous emission source using plasmonic nanoantennas," Nature Communications, Nature, vol. 6(1), pages 1-7, November.
    6. Haixu Leng & Brian Szychowski & Marie-Christine Daniel & Matthew Pelton, 2018. "Strong coupling and induced transparency at room temperature with single quantum dots and gap plasmons," Nature Communications, Nature, vol. 9(1), pages 1-7, December.
    7. Kartik Srinivasan & Oskar Painter, 2007. "Linear and nonlinear optical spectroscopy of a strongly coupled microdisk–quantum dot system," Nature, Nature, vol. 450(7171), pages 862-865, December.
    8. Elena V. Shevchenko & Dmitri V. Talapin & Nicholas A. Kotov & Stephen O'Brien & Christopher B. Murray, 2006. "Structural diversity in binary nanoparticle superlattices," Nature, Nature, vol. 439(7072), pages 55-59, January.
    9. J. P. Reithmaier & G. Sęk & A. Löffler & C. Hofmann & S. Kuhn & S. Reitzenstein & L. V. Keldysh & V. D. Kulakovskii & T. L. Reinecke & A. Forchel, 2004. "Strong coupling in a single quantum dot–semiconductor microcavity system," Nature, Nature, vol. 432(7014), pages 197-200, November.
    10. Marie-Elena Kleemann & Rohit Chikkaraddy & Evgeny M. Alexeev & Dean Kos & Cloudy Carnegie & Will Deacon & Alex Casalis Pury & Christoph Große & Bart Nijs & Jan Mertens & Alexander I. Tartakovskii & Je, 2017. "Strong-coupling of WSe2 in ultra-compact plasmonic nanocavities at room temperature," Nature Communications, Nature, vol. 8(1), pages 1-7, December.
    11. K. M. Birnbaum & A. Boca & R. Miller & A. D. Boozer & T. E. Northup & H. J. Kimble, 2005. "Photon blockade in an optical cavity with one trapped atom," Nature, Nature, vol. 436(7047), pages 87-90, July.
    12. Rohit Chikkaraddy & Bart de Nijs & Felix Benz & Steven J. Barrow & Oren A. Scherman & Edina Rosta & Angela Demetriadou & Peter Fox & Ortwin Hess & Jeremy J. Baumberg, 2016. "Single-molecule strong coupling at room temperature in plasmonic nanocavities," Nature, Nature, vol. 535(7610), pages 127-130, July.
    13. Qiangbing Guo & Xiao-Zhuo Qi & Lishu Zhang & Meng Gao & Sanlue Hu & Wenju Zhou & Wenjie Zang & Xiaoxu Zhao & Junyong Wang & Bingmin Yan & Mingquan Xu & Yun-Kun Wu & Goki Eda & Zewen Xiao & Shengyuan A, 2023. "Ultrathin quantum light source with van der Waals NbOCl2 crystal," Nature, Nature, vol. 613(7942), pages 53-59, January.
    14. Satyendra Nath Gupta & Ora Bitton & Tomas Neuman & Ruben Esteban & Lev Chuntonov & Javier Aizpurua & Gilad Haran, 2021. "Complex plasmon-exciton dynamics revealed through quantum dot light emission in a nanocavity," Nature Communications, Nature, vol. 12(1), pages 1-9, December.
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