IDEAS home Printed from https://ideas.repec.org/a/nat/natcom/v15y2024i1d10.1038_s41467-024-51170-7.html
   My bibliography  Save this article

Robust consistent single quantum dot strong coupling in plasmonic nanocavities

Author

Listed:
  • Shu Hu

    (University of Cambridge
    Xiamen University)

  • Junyang Huang

    (University of Cambridge)

  • Rakesh Arul

    (University of Cambridge)

  • Ana Sánchez-Iglesias

    (Basque Research and Technology Alliance (BRTA))

  • Yuling Xiong

    (University of Cambridge)

  • Luis M. Liz-Marzán

    (Basque Research and Technology Alliance (BRTA)
    Ikerbasque, Basque Foundation for Science)

  • Jeremy J. Baumberg

    (University of Cambridge)

Abstract

Strong coupling between a single quantum emitter and an optical cavity (at rate Ω) accesses fundamental quantum optics and provides an essential building block for photonic quantum technologies. However, the minimum mode volume of conventional dielectric cavities restricts their operation to cryogenic temperature for strong coupling. Here we harness surface self-assembly to make deterministic strong coupling at room temperature using CdSe/CdS quantum dots (QDs) in nanoparticle-on-mirror (NPoM) plasmonic nanocavities. We achieve a fabrication yield of ~70% for single QD strong coupling by optimizing their size and nano-assembly. A clear and reliable Rabi splitting is observed both in the scattering of each nanocavity and their photoluminescence, which are however not equal. Integrating these quantum elements with electrical pumping allows demonstration of strong coupling in their electroluminescence. This advance provides a straightforward way to achieve practical quantum devices at room temperature, and opens up exploration of their nonlinear, electrical, and quantum correlation properties.

Suggested Citation

  • Shu Hu & Junyang Huang & Rakesh Arul & Ana Sánchez-Iglesias & Yuling Xiong & Luis M. Liz-Marzán & Jeremy J. Baumberg, 2024. "Robust consistent single quantum dot strong coupling in plasmonic nanocavities," Nature Communications, Nature, vol. 15(1), pages 1-8, December.
    • Handle: RePEc:nat:natcom:v:15:y:2024:i:1:d:10.1038_s41467-024-51170-7
    DOI: 10.1038/s41467-024-51170-7
    as

    Download full text from publisher

    File URL: https://www.nature.com/articles/s41467-024-51170-7
    File Function: Abstract
    Download Restriction: no
    File URL: https://libkey.io/10.1038/s41467-024-51170-7?utm_source=ideas
    LibKey link: if access is restricted and if your library uses this service, LibKey will redirect you to where you can use your library subscription to access this item
    ---><---

    References listed on IDEAS

    as
    1. Oluwafemi S. Ojambati & Rohit Chikkaraddy & William D. Deacon & Matthew Horton & Dean Kos & Vladimir A. Turek & Ulrich F. Keyser & Jeremy J. Baumberg, 2019. "Quantum electrodynamics at room temperature coupling a single vibrating molecule with a plasmonic nanocavity," Nature Communications, Nature, vol. 10(1), pages 1-7, December.
    2. Kotni Santhosh & Ora Bitton & Lev Chuntonov & Gilad Haran, 2016. "Vacuum Rabi splitting in a plasmonic cavity at the single quantum emitter limit," Nature Communications, Nature, vol. 7(1), pages 1-5, September.
    3. Dandan Ge & Sylvie Marguet & Ali Issa & Safi Jradi & Tien Hoa Nguyen & Mackrine Nahra & Jéremie Béal & Régis Deturche & Hongshi Chen & Sylvain Blaize & Jérôme Plain & Céline Fiorini & Ludovic Douillar, 2020. "Hybrid plasmonic nano-emitters with controlled single quantum emitter positioning on the local excitation field," Nature Communications, Nature, vol. 11(1), pages 1-11, December.
    4. Daniel Najer & Immo Söllner & Pavel Sekatski & Vincent Dolique & Matthias C. Löbl & Daniel Riedel & Rüdiger Schott & Sebastian Starosielec & Sascha R. Valentin & Andreas D. Wieck & Nicolas Sangouard &, 2019. "A gated quantum dot strongly coupled to an optical microcavity," Nature, Nature, vol. 575(7784), pages 622-627, November.
    5. Thang B. Hoang & Gleb M. Akselrod & Christos Argyropoulos & Jiani Huang & David R. Smith & Maiken H. Mikkelsen, 2015. "Ultrafast spontaneous emission source using plasmonic nanoantennas," Nature Communications, Nature, vol. 6(1), pages 1-7, November.
    6. Haixu Leng & Brian Szychowski & Marie-Christine Daniel & Matthew Pelton, 2018. "Strong coupling and induced transparency at room temperature with single quantum dots and gap plasmons," Nature Communications, Nature, vol. 9(1), pages 1-7, December.
    7. Kartik Srinivasan & Oskar Painter, 2007. "Linear and nonlinear optical spectroscopy of a strongly coupled microdisk–quantum dot system," Nature, Nature, vol. 450(7171), pages 862-865, December.
    8. Elena V. Shevchenko & Dmitri V. Talapin & Nicholas A. Kotov & Stephen O'Brien & Christopher B. Murray, 2006. "Structural diversity in binary nanoparticle superlattices," Nature, Nature, vol. 439(7072), pages 55-59, January.
    9. J. P. Reithmaier & G. Sęk & A. Löffler & C. Hofmann & S. Kuhn & S. Reitzenstein & L. V. Keldysh & V. D. Kulakovskii & T. L. Reinecke & A. Forchel, 2004. "Strong coupling in a single quantum dot–semiconductor microcavity system," Nature, Nature, vol. 432(7014), pages 197-200, November.
    10. Marie-Elena Kleemann & Rohit Chikkaraddy & Evgeny M. Alexeev & Dean Kos & Cloudy Carnegie & Will Deacon & Alex Casalis Pury & Christoph Große & Bart Nijs & Jan Mertens & Alexander I. Tartakovskii & Je, 2017. "Strong-coupling of WSe2 in ultra-compact plasmonic nanocavities at room temperature," Nature Communications, Nature, vol. 8(1), pages 1-7, December.
    11. K. M. Birnbaum & A. Boca & R. Miller & A. D. Boozer & T. E. Northup & H. J. Kimble, 2005. "Photon blockade in an optical cavity with one trapped atom," Nature, Nature, vol. 436(7047), pages 87-90, July.
    12. Rohit Chikkaraddy & Bart de Nijs & Felix Benz & Steven J. Barrow & Oren A. Scherman & Edina Rosta & Angela Demetriadou & Peter Fox & Ortwin Hess & Jeremy J. Baumberg, 2016. "Single-molecule strong coupling at room temperature in plasmonic nanocavities," Nature, Nature, vol. 535(7610), pages 127-130, July.
    13. Qiangbing Guo & Xiao-Zhuo Qi & Lishu Zhang & Meng Gao & Sanlue Hu & Wenju Zhou & Wenjie Zang & Xiaoxu Zhao & Junyong Wang & Bingmin Yan & Mingquan Xu & Yun-Kun Wu & Goki Eda & Zewen Xiao & Shengyuan A, 2023. "Ultrathin quantum light source with van der Waals NbOCl2 crystal," Nature, Nature, vol. 613(7942), pages 53-59, January.
    14. Satyendra Nath Gupta & Ora Bitton & Tomas Neuman & Ruben Esteban & Lev Chuntonov & Javier Aizpurua & Gilad Haran, 2021. "Complex plasmon-exciton dynamics revealed through quantum dot light emission in a nanocavity," Nature Communications, Nature, vol. 12(1), pages 1-9, December.
    Full references (including those not matched with items on IDEAS)

    Most related items

    These are the items that most often cite the same works as this one and are cited by the same works as this one.
    1. Renming Liu & Ming Geng & Jindong Ai & Xinyi Fan & Zhixiang Liu & Yu-Wei Lu & Yanmin Kuang & Jing-Feng Liu & Lijun Guo & Lin Wu, 2024. "Deterministic positioning and alignment of a single-molecule exciton in plasmonic nanodimer for strong coupling," Nature Communications, Nature, vol. 15(1), pages 1-11, December.
    2. Tingting Wu & Chongwu Wang & Guangwei Hu & Zhixun Wang & Jiaxin Zhao & Zhe Wang & Ksenia Chaykun & Lin Liu & Mengxiao Chen & Dong Li & Song Zhu & Qihua Xiong & Zexiang Shen & Huajian Gao & Francisco J, 2024. "Ultrastrong exciton-plasmon couplings in WS2 multilayers synthesized with a random multi-singular metasurface at room temperature," Nature Communications, Nature, vol. 15(1), pages 1-9, December.
    3. T. Thu Ha Do & Milad Nonahal & Chi Li & Vytautas Valuckas & Hark Hoe Tan & Arseniy I. Kuznetsov & Hai Son Nguyen & Igor Aharonovich & Son Tung Ha, 2024. "Room-temperature strong coupling in a single-photon emitter-metasurface system," Nature Communications, Nature, vol. 15(1), pages 1-8, December.
    4. Nicholas A. Güsken & Ming Fu & Maximilian Zapf & Michael P. Nielsen & Paul Dichtl & Robert Röder & Alex S. Clark & Stefan A. Maier & Carsten Ronning & Rupert F. Oulton, 2023. "Emission enhancement of erbium in a reverse nanofocusing waveguide," Nature Communications, Nature, vol. 14(1), pages 1-10, December.
    5. Joel Kuttruff & Marco Romanelli & Esteban Pedrueza-Villalmanzo & Jonas Allerbeck & Jacopo Fregoni & Valeria Saavedra-Becerril & Joakim Andréasson & Daniele Brida & Alexandre Dmitriev & Stefano Corni &, 2023. "Sub-picosecond collapse of molecular polaritons to pure molecular transition in plasmonic photoswitch-nanoantennas," Nature Communications, Nature, vol. 14(1), pages 1-10, December.
    6. Junze Zhou & P. A. D. Gonçalves & Fabrizio Riminucci & Scott Dhuey & Edward S. Barnard & Adam Schwartzberg & F. Javier García de Abajo & Alexander Weber-Bargioni, 2024. "Probing plexciton emission from 2D materials on gold nanotrenches," Nature Communications, Nature, vol. 15(1), pages 1-8, December.
    7. Raj Pandya & Richard Y. S. Chen & Qifei Gu & Jooyoung Sung & Christoph Schnedermann & Oluwafemi S. Ojambati & Rohit Chikkaraddy & Jeffrey Gorman & Gianni Jacucci & Olimpia D. Onelli & Tom Willhammar &, 2021. "Microcavity-like exciton-polaritons can be the primary photoexcitation in bare organic semiconductors," Nature Communications, Nature, vol. 12(1), pages 1-11, December.
    8. Daniel Timmer & Moritz Gittinger & Thomas Quenzel & Sven Stephan & Yu Zhang & Marvin F. Schumacher & Arne Lützen & Martin Silies & Sergei Tretiak & Jin-Hui Zhong & Antonietta De Sio & Christoph Lienau, 2023. "Plasmon mediated coherent population oscillations in molecular aggregates," Nature Communications, Nature, vol. 14(1), pages 1-10, December.
    9. Zhengyi Lu & Jiamin Ji & Haiming Ye & Hao Zhang & Shunping Zhang & Hongxing Xu, 2024. "Quantifying the ultimate limit of plasmonic near-field enhancement," Nature Communications, Nature, vol. 15(1), pages 1-8, December.
    10. Sixu Wang & Wei Li & Chenguang Deng & Zijian Hong & Han-Bin Gao & Xiaolong Li & Yueliang Gu & Qiang Zheng & Yongjun Wu & Paul G. Evans & Jing-Feng Li & Ce-Wen Nan & Qian Li, 2024. "Giant electric field-induced second harmonic generation in polar skyrmions," Nature Communications, Nature, vol. 15(1), pages 1-10, December.
    11. Fuhuan Shen & Zhenghe Zhang & Yaoqiang Zhou & Jingwen Ma & Kun Chen & Huanjun Chen & Shaojun Wang & Jianbin Xu & Zefeng Chen, 2022. "Transition metal dichalcogenide metaphotonic and self-coupled polaritonic platform grown by chemical vapor deposition," Nature Communications, Nature, vol. 13(1), pages 1-9, December.
    12. Shima Rajabali & Sergej Markmann & Elsa Jöchl & Mattias Beck & Christian A. Lehner & Werner Wegscheider & Jérôme Faist & Giacomo Scalari, 2022. "An ultrastrongly coupled single terahertz meta-atom," Nature Communications, Nature, vol. 13(1), pages 1-8, December.
    13. N. Bart & C. Dangel & P. Zajac & N. Spitzer & J. Ritzmann & M. Schmidt & H. G. Babin & R. Schott & S. R. Valentin & S. Scholz & Y. Wang & R. Uppu & D. Najer & M. C. Löbl & N. Tomm & A. Javadi & N. O. , 2022. "Wafer-scale epitaxial modulation of quantum dot density," Nature Communications, Nature, vol. 13(1), pages 1-7, December.
    14. Rosario R. Riso & Tor S. Haugland & Enrico Ronca & Henrik Koch, 2022. "Molecular orbital theory in cavity QED environments," Nature Communications, Nature, vol. 13(1), pages 1-8, December.
    15. Bum Chul Park & Min Jun Ko & Young Kwang Kim & Gyu Won Kim & Myeong Soo Kim & Thomas Myeongseok Koo & Hong En Fu & Young Keun Kim, 2022. "Surface-ligand-induced crystallographic disorder–order transition in oriented attachment for the tuneable assembly of mesocrystals," Nature Communications, Nature, vol. 13(1), pages 1-11, December.
    16. Xiang-Dong Chen & En-Hui Wang & Long-Kun Shan & Ce Feng & Yu Zheng & Yang Dong & Guang-Can Guo & Fang-Wen Sun, 2021. "Focusing the electromagnetic field to 10−6λ for ultra-high enhancement of field-matter interaction," Nature Communications, Nature, vol. 12(1), pages 1-7, December.
    17. Longlong Yang & Yu Yuan & Bowen Fu & Jingnan Yang & Danjie Dai & Shushu Shi & Sai Yan & Rui Zhu & Xu Han & Hancong Li & Zhanchun Zuo & Can Wang & Yuan Huang & Kuijuan Jin & Qihuang Gong & Xiulai Xu, 2023. "Revealing broken valley symmetry of quantum emitters in WSe2 with chiral nanocavities," Nature Communications, Nature, vol. 14(1), pages 1-11, December.
    18. Christian Schäfer & Johannes Flick & Enrico Ronca & Prineha Narang & Angel Rubio, 2022. "Shining light on the microscopic resonant mechanism responsible for cavity-mediated chemical reactivity," Nature Communications, Nature, vol. 13(1), pages 1-9, December.
    19. Dengsheng Wu & Xiaoli Lu & Jianping Li & Jing Li, 2020. "Does the institutional diversity of editorial boards increase journal quality? The case economics field," Scientometrics, Springer;Akadémiai Kiadó, vol. 124(2), pages 1579-1597, August.
    20. Chi Zhang & Huatian Hu & Chunmiao Ma & Yawen Li & Xujie Wang & Dongyao Li & Artur Movsesyan & Zhiming Wang & Alexander Govorov & Quan Gan & Tao Ding, 2024. "Quantum plasmonics pushes chiral sensing limit to single molecules: a paradigm for chiral biodetections," Nature Communications, Nature, vol. 15(1), pages 1-8, December.

    More about this item

    Statistics

    Access and download statistics

    Corrections

    All material on this site has been provided by the respective publishers and authors. You can help correct errors and omissions. When requesting a correction, please mention this item's handle: RePEc:nat:natcom:v:15:y:2024:i:1:d:10.1038_s41467-024-51170-7. See general information about how to correct material in RePEc.

    If you have authored this item and are not yet registered with RePEc, we encourage you to do it here. This allows to link your profile to this item. It also allows you to accept potential citations to this item that we are uncertain about.

    If CitEc recognized a bibliographic reference but did not link an item in RePEc to it, you can help with this form .

    If you know of missing items citing this one, you can help us creating those links by adding the relevant references in the same way as above, for each refering item. If you are a registered author of this item, you may also want to check the "citations" tab in your RePEc Author Service profile, as there may be some citations waiting for confirmation.

    For technical questions regarding this item, or to correct its authors, title, abstract, bibliographic or download information, contact: Sonal Shukla or Springer Nature Abstracting and Indexing (email available below). General contact details of provider: http://www.nature.com .

    Please note that corrections may take a couple of weeks to filter through the various RePEc services.

    IDEAS is a RePEc service. RePEc uses bibliographic data supplied by the respective publishers.