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Single-molecule strong coupling at room temperature in plasmonic nanocavities

Author

Listed:
  • Rohit Chikkaraddy

    (NanoPhotonics Centre, Cavendish Laboratory, University of Cambridge)

  • Bart de Nijs

    (NanoPhotonics Centre, Cavendish Laboratory, University of Cambridge)

  • Felix Benz

    (NanoPhotonics Centre, Cavendish Laboratory, University of Cambridge)

  • Steven J. Barrow

    (Melville Laboratory for Polymer Synthesis, University of Cambridge)

  • Oren A. Scherman

    (Melville Laboratory for Polymer Synthesis, University of Cambridge)

  • Edina Rosta

    (King’s College London)

  • Angela Demetriadou

    (Blackett Laboratory, Prince Consort Road, Imperial College)

  • Peter Fox

    (Blackett Laboratory, Prince Consort Road, Imperial College)

  • Ortwin Hess

    (Blackett Laboratory, Prince Consort Road, Imperial College)

  • Jeremy J. Baumberg

    (NanoPhotonics Centre, Cavendish Laboratory, University of Cambridge)

Abstract

Placing a light emitter in an ultra-small optical cavity results in coupling between matter and light, generating new forms of emission that can be exploited in practical or fundamental applications; here, a system is described in which strong light–matter coupling occurs at room temperature and in ambient conditions by aligning single dye molecules in the optical cavities between gold nanoparticles and surfaces.

Suggested Citation

  • Rohit Chikkaraddy & Bart de Nijs & Felix Benz & Steven J. Barrow & Oren A. Scherman & Edina Rosta & Angela Demetriadou & Peter Fox & Ortwin Hess & Jeremy J. Baumberg, 2016. "Single-molecule strong coupling at room temperature in plasmonic nanocavities," Nature, Nature, vol. 535(7610), pages 127-130, July.
    • Handle: RePEc:nat:nature:v:535:y:2016:i:7610:d:10.1038_nature17974
    DOI: 10.1038/nature17974
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    Cited by:

    1. Rosario R. Riso & Tor S. Haugland & Enrico Ronca & Henrik Koch, 2022. "Molecular orbital theory in cavity QED environments," Nature Communications, Nature, vol. 13(1), pages 1-8, December.
    2. Raj Pandya & Richard Y. S. Chen & Qifei Gu & Jooyoung Sung & Christoph Schnedermann & Oluwafemi S. Ojambati & Rohit Chikkaraddy & Jeffrey Gorman & Gianni Jacucci & Olimpia D. Onelli & Tom Willhammar &, 2021. "Microcavity-like exciton-polaritons can be the primary photoexcitation in bare organic semiconductors," Nature Communications, Nature, vol. 12(1), pages 1-11, December.
    3. Daniel Timmer & Moritz Gittinger & Thomas Quenzel & Sven Stephan & Yu Zhang & Marvin F. Schumacher & Arne Lützen & Martin Silies & Sergei Tretiak & Jin-Hui Zhong & Antonietta De Sio & Christoph Lienau, 2023. "Plasmon mediated coherent population oscillations in molecular aggregates," Nature Communications, Nature, vol. 14(1), pages 1-10, December.
    4. Fabijan Pavošević & Robert L. Smith & Angel Rubio, 2023. "Computational study on the catalytic control of endo/exo Diels-Alder reactions by cavity quantum vacuum fluctuations," Nature Communications, Nature, vol. 14(1), pages 1-8, December.
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    6. Zhengyi Lu & Jiamin Ji & Haiming Ye & Hao Zhang & Shunping Zhang & Hongxing Xu, 2024. "Quantifying the ultimate limit of plasmonic near-field enhancement," Nature Communications, Nature, vol. 15(1), pages 1-8, December.
    7. Fuhuan Shen & Zhenghe Zhang & Yaoqiang Zhou & Jingwen Ma & Kun Chen & Huanjun Chen & Shaojun Wang & Jianbin Xu & Zefeng Chen, 2022. "Transition metal dichalcogenide metaphotonic and self-coupled polaritonic platform grown by chemical vapor deposition," Nature Communications, Nature, vol. 13(1), pages 1-9, December.
    8. Chi Zhang & Huatian Hu & Chunmiao Ma & Yawen Li & Xujie Wang & Dongyao Li & Artur Movsesyan & Zhiming Wang & Alexander Govorov & Quan Gan & Tao Ding, 2024. "Quantum plasmonics pushes chiral sensing limit to single molecules: a paradigm for chiral biodetections," Nature Communications, Nature, vol. 15(1), pages 1-8, December.
    9. Shima Rajabali & Sergej Markmann & Elsa Jöchl & Mattias Beck & Christian A. Lehner & Werner Wegscheider & Jérôme Faist & Giacomo Scalari, 2022. "An ultrastrongly coupled single terahertz meta-atom," Nature Communications, Nature, vol. 13(1), pages 1-8, December.
    10. Shu Hu & Junyang Huang & Rakesh Arul & Ana Sánchez-Iglesias & Yuling Xiong & Luis M. Liz-Marzán & Jeremy J. Baumberg, 2024. "Robust consistent single quantum dot strong coupling in plasmonic nanocavities," Nature Communications, Nature, vol. 15(1), pages 1-8, December.
    11. Xiang-Dong Chen & En-Hui Wang & Long-Kun Shan & Ce Feng & Yu Zheng & Yang Dong & Guang-Can Guo & Fang-Wen Sun, 2021. "Focusing the electromagnetic field to 10−6λ for ultra-high enhancement of field-matter interaction," Nature Communications, Nature, vol. 12(1), pages 1-7, December.
    12. Renming Liu & Ming Geng & Jindong Ai & Xinyi Fan & Zhixiang Liu & Yu-Wei Lu & Yanmin Kuang & Jing-Feng Liu & Lijun Guo & Lin Wu, 2024. "Deterministic positioning and alignment of a single-molecule exciton in plasmonic nanodimer for strong coupling," Nature Communications, Nature, vol. 15(1), pages 1-11, December.
    13. Guang-Can Li & Dangyuan Lei & Meng Qiu & Wei Jin & Sheng Lan & Anatoly V. Zayats, 2021. "Light-induced symmetry breaking for enhancing second-harmonic generation from an ultrathin plasmonic nanocavity," Nature Communications, Nature, vol. 12(1), pages 1-8, December.
    14. Kaihong Sun & Raphael F. Ribeiro, 2024. "Theoretical formulation of chemical equilibrium under vibrational strong coupling," Nature Communications, Nature, vol. 15(1), pages 1-12, December.
    15. Mingu Kang & Hyunwoo Kim & Elham Oleiki & Yeonjeong Koo & Hyeongwoo Lee & Huitae Joo & Jinseong Choi & Taeyong Eom & Geunsik Lee & Yung Doug Suh & Kyoung-Duck Park, 2022. "Conformational heterogeneity of molecules physisorbed on a gold surface at room temperature," Nature Communications, Nature, vol. 13(1), pages 1-9, December.
    16. Junze Zhou & P. A. D. Gonçalves & Fabrizio Riminucci & Scott Dhuey & Edward S. Barnard & Adam Schwartzberg & F. Javier García de Abajo & Alexander Weber-Bargioni, 2024. "Probing plexciton emission from 2D materials on gold nanotrenches," Nature Communications, Nature, vol. 15(1), pages 1-8, December.
    17. Nicholas A. Güsken & Ming Fu & Maximilian Zapf & Michael P. Nielsen & Paul Dichtl & Robert Röder & Alex S. Clark & Stefan A. Maier & Carsten Ronning & Rupert F. Oulton, 2023. "Emission enhancement of erbium in a reverse nanofocusing waveguide," Nature Communications, Nature, vol. 14(1), pages 1-10, December.
    18. Longlong Yang & Yu Yuan & Bowen Fu & Jingnan Yang & Danjie Dai & Shushu Shi & Sai Yan & Rui Zhu & Xu Han & Hancong Li & Zhanchun Zuo & Can Wang & Yuan Huang & Kuijuan Jin & Qihuang Gong & Xiulai Xu, 2023. "Revealing broken valley symmetry of quantum emitters in WSe2 with chiral nanocavities," Nature Communications, Nature, vol. 14(1), pages 1-11, December.
    19. Tingting Wu & Chongwu Wang & Guangwei Hu & Zhixun Wang & Jiaxin Zhao & Zhe Wang & Ksenia Chaykun & Lin Liu & Mengxiao Chen & Dong Li & Song Zhu & Qihua Xiong & Zexiang Shen & Huajian Gao & Francisco J, 2024. "Ultrastrong exciton-plasmon couplings in WS2 multilayers synthesized with a random multi-singular metasurface at room temperature," Nature Communications, Nature, vol. 15(1), pages 1-9, December.
    20. Ferry Anggoro Ardy Nugroho & Ping Bai & Iwan Darmadi & Gabriel W. Castellanos & Joachim Fritzsche & Christoph Langhammer & Jaime Gómez Rivas & Andrea Baldi, 2022. "Inverse designed plasmonic metasurface with parts per billion optical hydrogen detection," Nature Communications, Nature, vol. 13(1), pages 1-10, December.

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