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Hybrid plasmonic nano-emitters with controlled single quantum emitter positioning on the local excitation field

Author

Listed:
  • Dandan Ge

    (Light, nanomaterials, nanotechnologies (L2n) Laboratory, CNRS ERL 7004, University of Technology of Troyes
    Shenzhen Planck Innovation Technologies Co. Ltd, Shenzhen)

  • Sylvie Marguet

    (Université Paris Saclay, CEA, CNRS, NIMBE)

  • Ali Issa

    (Light, nanomaterials, nanotechnologies (L2n) Laboratory, CNRS ERL 7004, University of Technology of Troyes)

  • Safi Jradi

    (Light, nanomaterials, nanotechnologies (L2n) Laboratory, CNRS ERL 7004, University of Technology of Troyes)

  • Tien Hoa Nguyen

    (CNRS-International-NTU-Thales Research Alliance (CINTRA))

  • Mackrine Nahra

    (Light, nanomaterials, nanotechnologies (L2n) Laboratory, CNRS ERL 7004, University of Technology of Troyes)

  • Jéremie Béal

    (Light, nanomaterials, nanotechnologies (L2n) Laboratory, CNRS ERL 7004, University of Technology of Troyes)

  • Régis Deturche

    (Light, nanomaterials, nanotechnologies (L2n) Laboratory, CNRS ERL 7004, University of Technology of Troyes)

  • Hongshi Chen

    (Light, nanomaterials, nanotechnologies (L2n) Laboratory, CNRS ERL 7004, University of Technology of Troyes
    Shenzhen Planck Innovation Technologies Co. Ltd, Shenzhen)

  • Sylvain Blaize

    (Light, nanomaterials, nanotechnologies (L2n) Laboratory, CNRS ERL 7004, University of Technology of Troyes)

  • Jérôme Plain

    (Light, nanomaterials, nanotechnologies (L2n) Laboratory, CNRS ERL 7004, University of Technology of Troyes)

  • Céline Fiorini

    (Université Paris Saclay, CEA, CNRS, SPEC)

  • Ludovic Douillard

    (Université Paris Saclay, CEA, CNRS, SPEC)

  • Olivier Soppera

    (Université de Haute Alsace, CNRS, IS2M UMR 7361
    Université de Strasbourg)

  • Xuan Quyen Dinh

    (CNRS-International-NTU-Thales Research Alliance (CINTRA)
    Thales Solutions Asia Pte Ltd, R&T Department
    School of Electrical and Electronic Engineering, Nanyang Technological University, Nanyang Avenue)

  • Cuong Dang

    (CNRS-International-NTU-Thales Research Alliance (CINTRA)
    School of Electrical and Electronic Engineering, Nanyang Technological University, Nanyang Avenue)

  • Xuyong Yang

    (School of Mechatronic Engineering and Automation, Key Lab of Advanced Display and System Application, Ministry of Education, Shanghai University)

  • Tao Xu

    (School of Mechatronic Engineering and Automation, Key Lab of Advanced Display and System Application, Ministry of Education, Shanghai University
    Sino-European School of Technology, Shanghai University)

  • Bin Wei

    (School of Mechatronic Engineering and Automation, Key Lab of Advanced Display and System Application, Ministry of Education, Shanghai University)

  • Xiao Wei Sun

    (Shenzhen Planck Innovation Technologies Co. Ltd, Shenzhen
    Department of Electrical and Electronic Engineering, Southern University of Science and Technology, Shenzhen)

  • Christophe Couteau

    (Light, nanomaterials, nanotechnologies (L2n) Laboratory, CNRS ERL 7004, University of Technology of Troyes)

  • Renaud Bachelot

    (Light, nanomaterials, nanotechnologies (L2n) Laboratory, CNRS ERL 7004, University of Technology of Troyes
    Shenzhen Planck Innovation Technologies Co. Ltd, Shenzhen
    School of Mechatronic Engineering and Automation, Key Lab of Advanced Display and System Application, Ministry of Education, Shanghai University
    Sino-European School of Technology, Shanghai University)

Abstract

Hybrid plasmonic nano-emitters based on the combination of quantum dot emitters (QD) and plasmonic nanoantennas open up new perspectives in the control of light. However, precise positioning of any active medium at the nanoscale constitutes a challenge. Here, we report on the optimal overlap of antenna’s near-field and active medium whose spatial distribution is controlled via a plasmon-triggered 2-photon polymerization of a photosensitive formulation containing QDs. Au nanoparticles of various geometries are considered. The response of these hybrid nano-emitters is shown to be highly sensitive to the light polarization. Different light emission states are evidenced by photoluminescence measurements. These states correspond to polarization-sensitive nanoscale overlap between the exciting local field and the active medium distribution. The decrease of the QD concentration within the monomer formulation allows trapping of a single quantum dot in the vicinity of the Au particle. The latter objects show polarization-dependent switching in the single-photon regime.

Suggested Citation

  • Dandan Ge & Sylvie Marguet & Ali Issa & Safi Jradi & Tien Hoa Nguyen & Mackrine Nahra & Jéremie Béal & Régis Deturche & Hongshi Chen & Sylvain Blaize & Jérôme Plain & Céline Fiorini & Ludovic Douillar, 2020. "Hybrid plasmonic nano-emitters with controlled single quantum emitter positioning on the local excitation field," Nature Communications, Nature, vol. 11(1), pages 1-11, December.
    • Handle: RePEc:nat:natcom:v:11:y:2020:i:1:d:10.1038_s41467-020-17248-8
    DOI: 10.1038/s41467-020-17248-8
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    Cited by:

    1. Shu Hu & Junyang Huang & Rakesh Arul & Ana Sánchez-Iglesias & Yuling Xiong & Luis M. Liz-Marzán & Jeremy J. Baumberg, 2024. "Robust consistent single quantum dot strong coupling in plasmonic nanocavities," Nature Communications, Nature, vol. 15(1), pages 1-8, December.

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