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Emergent zero-field anomalous Hall effect in a reconstructed rutile antiferromagnetic metal

Author

Listed:
  • Meng Wang

    (RIKEN Center for Emergent Matter Science (CEMS))

  • Katsuhiro Tanaka

    (University of Tokyo)

  • Shiro Sakai

    (RIKEN Center for Emergent Matter Science (CEMS))

  • Ziqian Wang

    (RIKEN Center for Emergent Matter Science (CEMS))

  • Ke Deng

    (Southern University of Science and Technology (SUSTech)
    International Quantum Academy)

  • Yingjie Lyu

    (Tsinghua University)

  • Cong Li

    (Tsinghua University)

  • Di Tian

    (Tsinghua University)

  • Shengchun Shen

    (University of Science and Technology of China)

  • Naoki Ogawa

    (RIKEN Center for Emergent Matter Science (CEMS)
    University of Tokyo)

  • Naoya Kanazawa

    (The University of Tokyo)

  • Pu Yu

    (Tsinghua University)

  • Ryotaro Arita

    (RIKEN Center for Emergent Matter Science (CEMS)
    University of Tokyo)

  • Fumitaka Kagawa

    (RIKEN Center for Emergent Matter Science (CEMS)
    Tokyo Institute of Technology)

Abstract

The anomalous Hall effect (AHE) that emerges in antiferromagnetic metals shows intriguing physics and offers numerous potential applications. Magnets with a rutile crystal structure have recently received attention as a possible platform for a collinear-antiferromagnetism-induced AHE. RuO2 is a prototypical candidate material, however the AHE is prohibited at zero field by symmetry because of the high-symmetry [001] direction of the Néel vector at the ground state. Here, we show AHE at zero field in Cr-doped rutile, Ru0.8Cr0.2O2. The magnetization, transport and density functional theory calculations indicate that appropriate doping of Cr at Ru sites reconstructs the collinear antiferromagnetism in RuO2, resulting in a rotation of the Néel vector from [001] to [110] while maintaining a collinear antiferromagnetic state. The AHE with vanishing net moment in the Ru0.8Cr0.2O2 exhibits an orientation dependence consistent with the [110]-oriented Hall vector. These results demonstrate that material engineering by doping is a useful approach to manipulate AHE in antiferromagnetic metals.

Suggested Citation

  • Meng Wang & Katsuhiro Tanaka & Shiro Sakai & Ziqian Wang & Ke Deng & Yingjie Lyu & Cong Li & Di Tian & Shengchun Shen & Naoki Ogawa & Naoya Kanazawa & Pu Yu & Ryotaro Arita & Fumitaka Kagawa, 2023. "Emergent zero-field anomalous Hall effect in a reconstructed rutile antiferromagnetic metal," Nature Communications, Nature, vol. 14(1), pages 1-8, December.
    • Handle: RePEc:nat:natcom:v:14:y:2023:i:1:d:10.1038_s41467-023-43962-0
    DOI: 10.1038/s41467-023-43962-0
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    1. Yukako Fujishiro & Naoya Kanazawa & Ryosuke Kurihara & Hiroaki Ishizuka & Tomohiro Hori & Fehmi Sami Yasin & Xiuzhen Yu & Atsushi Tsukazaki & Masakazu Ichikawa & Masashi Kawasaki & Naoto Nagaosa & Mas, 2021. "Giant anomalous Hall effect from spin-chirality scattering in a chiral magnet," Nature Communications, Nature, vol. 12(1), pages 1-6, December.
    2. Satoru Nakatsuji & Naoki Kiyohara & Tomoya Higo, 2015. "Large anomalous Hall effect in a non-collinear antiferromagnet at room temperature," Nature, Nature, vol. 527(7577), pages 212-215, November.
    3. Nirmal J. Ghimire & A. S. Botana & J. S. Jiang & Junjie Zhang & Y.-S. Chen & J. F. Mitchell, 2018. "Large anomalous Hall effect in the chiral-lattice antiferromagnet CoNb3S6," Nature Communications, Nature, vol. 9(1), pages 1-6, December.
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