IDEAS home Printed from https://ideas.repec.org/a/nat/natcom/v14y2023i1d10.1038_s41467-023-43853-4.html
   My bibliography  Save this article

Tetrahedral triple-Q magnetic ordering and large spontaneous Hall conductivity in the metallic triangular antiferromagnet Co1/3TaS2

Author

Listed:
  • Pyeongjae Park

    (Seoul National University
    Seoul National University)

  • Woonghee Cho

    (Seoul National University
    Seoul National University)

  • Chaebin Kim

    (Seoul National University
    Seoul National University)

  • Yeochan An

    (Seoul National University
    Seoul National University)

  • Yoon-Gu Kang

    (KAIST)

  • Maxim Avdeev

    (Australian Nuclear Science and Technology Organisation (ANSTO)
    The University of Sydney)

  • Romain Sibille

    (Paul Scherrer Institut)

  • Kazuki Iida

    (Comprehensive Research Organization for Science and Society (CROSS))

  • Ryoichi Kajimoto

    (J-PARC Center, Japan Atomic Energy Agency)

  • Ki Hoon Lee

    (Incheon National University)

  • Woori Ju

    (Chonnam National University)

  • En-Jin Cho

    (Chonnam National University)

  • Han-Jin Noh

    (Chonnam National University)

  • Myung Joon Han

    (KAIST)

  • Shang-Shun Zhang

    (University of Minnesota)

  • Cristian D. Batista

    (The University of Tennessee
    Quantum Condensed Matter Division and Shull-Wollan Center, Oak Ridge National Laboratory)

  • Je-Geun Park

    (Seoul National University
    Seoul National University
    Seoul National University)

Abstract

The triangular lattice antiferromagnet (TLAF) has been the standard paradigm of frustrated magnetism for several decades. The most common magnetic ordering in insulating TLAFs is the 120° structure. However, a new triple-Q chiral ordering can emerge in metallic TLAFs, representing the short wavelength limit of magnetic skyrmion crystals. We report the metallic TLAF Co1/3TaS2 as the first example of tetrahedral triple-Q magnetic ordering with the associated topological Hall effect (non-zero σxy(H = 0)). We also present a theoretical framework that describes the emergence of this magnetic ground state, which is further supported by the electronic structure measured by angle-resolved photoemission spectroscopy. Additionally, our measurements of the inelastic neutron scattering cross section are consistent with the calculated dynamical structure factor of the tetrahedral triple-Q state.

Suggested Citation

  • Pyeongjae Park & Woonghee Cho & Chaebin Kim & Yeochan An & Yoon-Gu Kang & Maxim Avdeev & Romain Sibille & Kazuki Iida & Ryoichi Kajimoto & Ki Hoon Lee & Woori Ju & En-Jin Cho & Han-Jin Noh & Myung Joo, 2023. "Tetrahedral triple-Q magnetic ordering and large spontaneous Hall conductivity in the metallic triangular antiferromagnet Co1/3TaS2," Nature Communications, Nature, vol. 14(1), pages 1-9, December.
    • Handle: RePEc:nat:natcom:v:14:y:2023:i:1:d:10.1038_s41467-023-43853-4
    DOI: 10.1038/s41467-023-43853-4
    as

    Download full text from publisher

    File URL: https://www.nature.com/articles/s41467-023-43853-4
    File Function: Abstract
    Download Restriction: no
    File URL: https://libkey.io/10.1038/s41467-023-43853-4?utm_source=ideas
    LibKey link: if access is restricted and if your library uses this service, LibKey will redirect you to where you can use your library subscription to access this item
    ---><---

    References listed on IDEAS

    as
    1. Nirmal J. Ghimire & A. S. Botana & J. S. Jiang & Junjie Zhang & Y.-S. Chen & J. F. Mitchell, 2018. "Large anomalous Hall effect in the chiral-lattice antiferromagnet CoNb3S6," Nature Communications, Nature, vol. 9(1), pages 1-6, December.
    2. X. Z. Yu & Y. Onose & N. Kanazawa & J. H. Park & J. H. Han & Y. Matsui & N. Nagaosa & Y. Tokura, 2010. "Real-space observation of a two-dimensional skyrmion crystal," Nature, Nature, vol. 465(7300), pages 901-904, June.
    Full references (including those not matched with items on IDEAS)

    Most related items

    These are the items that most often cite the same works as this one and are cited by the same works as this one.
    1. Hikaru Takeda & Masataka Kawano & Kyo Tamura & Masatoshi Akazawa & Jian Yan & Takeshi Waki & Hiroyuki Nakamura & Kazuki Sato & Yasuo Narumi & Masayuki Hagiwara & Minoru Yamashita & Chisa Hotta, 2024. "Magnon thermal Hall effect via emergent SU(3) flux on the antiferromagnetic skyrmion lattice," Nature Communications, Nature, vol. 15(1), pages 1-8, December.
    2. Satoru Hayami & Tsuyoshi Okubo & Yukitoshi Motome, 2021. "Phase shift in skyrmion crystals," Nature Communications, Nature, vol. 12(1), pages 1-6, December.
    3. Fumiya Sekiguchi & Kestutis Budzinauskas & Prashant Padmanabhan & Rolf B. Versteeg & Vladimir Tsurkan & István Kézsmárki & Francesco Foggetti & Sergey Artyukhin & Paul H. M. Loosdrecht, 2022. "Slowdown of photoexcited spin dynamics in the non-collinear spin-ordered phases in skyrmion host GaV4S8," Nature Communications, Nature, vol. 13(1), pages 1-8, December.
    4. Weiwei Wang & Dongsheng Song & Wensen Wei & Pengfei Nan & Shilei Zhang & Binghui Ge & Mingliang Tian & Jiadong Zang & Haifeng Du, 2022. "Electrical manipulation of skyrmions in a chiral magnet," Nature Communications, Nature, vol. 13(1), pages 1-7, December.
    5. Yu-Tsun Shao & Sujit Das & Zijian Hong & Ruijuan Xu & Swathi Chandrika & Fernando Gómez-Ortiz & Pablo García-Fernández & Long-Qing Chen & Harold Y. Hwang & Javier Junquera & Lane W. Martin & Ramamoort, 2023. "Emergent chirality in a polar meron to skyrmion phase transition," Nature Communications, Nature, vol. 14(1), pages 1-9, December.
    6. C. J. O. Reichhardt & C. Reichhardt, 2022. "Dynamic phases and reentrant Hall effect for vortices and skyrmions on periodic pinning arrays," The European Physical Journal B: Condensed Matter and Complex Systems, Springer;EDP Sciences, vol. 95(8), pages 1-16, August.
    7. Hanqing Zhao & Boris A. Malomed & Ivan I. Smalyukh, 2023. "Topological solitonic macromolecules," Nature Communications, Nature, vol. 14(1), pages 1-12, December.
    8. Deepak Singh & Yukako Fujishiro & Satoru Hayami & Samuel H. Moody & Takuya Nomoto & Priya R. Baral & Victor Ukleev & Robert Cubitt & Nina-Juliane Steinke & Dariusz J. Gawryluk & Ekaterina Pomjakushina, 2023. "Transition between distinct hybrid skyrmion textures through their hexagonal-to-square crystal transformation in a polar magnet," Nature Communications, Nature, vol. 14(1), pages 1-12, December.
    9. Fehmi Sami Yasin & Jan Masell & Kosuke Karube & Daisuke Shindo & Yasujiro Taguchi & Yoshinori Tokura & Xiuzhen Yu, 2023. "Heat current-driven topological spin texture transformations and helical q-vector switching," Nature Communications, Nature, vol. 14(1), pages 1-8, December.
    10. John H. Gaida & Hugo Lourenço-Martins & Sergey V. Yalunin & Armin Feist & Murat Sivis & Thorsten Hohage & F. Javier García de Abajo & Claus Ropers, 2023. "Lorentz microscopy of optical fields," Nature Communications, Nature, vol. 14(1), pages 1-8, December.
    11. Yong Yu & Xiao Xu & Yan Wang & Baohai Jia & Shan Huang & Xiaobin Qiang & Bin Zhu & Peijian Lin & Binbin Jiang & Shixuan Liu & Xia Qi & Kefan Pan & Di Wu & Haizhou Lu & Michel Bosman & Stephen J. Penny, 2022. "Tunable quantum gaps to decouple carrier and phonon transport leading to high-performance thermoelectrics," Nature Communications, Nature, vol. 13(1), pages 1-9, December.
    12. Yongsen Zhang & Jin Tang & Yaodong Wu & Meng Shi & Xitong Xu & Shouguo Wang & Mingliang Tian & Haifeng Du, 2024. "Stable skyrmion bundles at room temperature and zero magnetic field in a chiral magnet," Nature Communications, Nature, vol. 15(1), pages 1-9, December.
    13. Xiaowei Lv & Hualiang Lv & Yalei Huang & Ruixuan Zhang & Guanhua Qin & Yihui Dong & Min Liu & Ke Pei & Guixin Cao & Jincang Zhang & Yuxiang Lai & Renchao Che, 2024. "Distinct skyrmion phases at room temperature in two-dimensional ferromagnet Fe3GaTe2," Nature Communications, Nature, vol. 15(1), pages 1-9, December.
    14. W. S. Huxter & M. L. Palm & M. L. Davis & P. Welter & C.-H. Lambert & M. Trassin & C. L. Degen, 2022. "Scanning gradiometry with a single spin quantum magnetometer," Nature Communications, Nature, vol. 13(1), pages 1-9, December.
    15. Mona Bhukta & Takaaki Dohi & Venkata Krishna Bharadwaj & Ricardo Zarzuela & Maria-Andromachi Syskaki & Michael Foerster & Miguel Angel Niño & Jairo Sinova & Robert Frömter & Mathias Kläui, 2024. "Homochiral antiferromagnetic merons, antimerons and bimerons realized in synthetic antiferromagnets," Nature Communications, Nature, vol. 15(1), pages 1-10, December.
    16. Meng Wang & Katsuhiro Tanaka & Shiro Sakai & Ziqian Wang & Ke Deng & Yingjie Lyu & Cong Li & Di Tian & Shengchun Shen & Naoki Ogawa & Naoya Kanazawa & Pu Yu & Ryotaro Arita & Fumitaka Kagawa, 2023. "Emergent zero-field anomalous Hall effect in a reconstructed rutile antiferromagnetic metal," Nature Communications, Nature, vol. 14(1), pages 1-8, December.
    17. Rina Takagi & Naofumi Matsuyama & Victor Ukleev & Le Yu & Jonathan S. White & Sonia Francoual & José R. L. Mardegan & Satoru Hayami & Hiraku Saito & Koji Kaneko & Kazuki Ohishi & Yoshichika Ōnuki & Ta, 2022. "Square and rhombic lattices of magnetic skyrmions in a centrosymmetric binary compound," Nature Communications, Nature, vol. 13(1), pages 1-7, December.
    18. Yuan Yao & Bei Ding & Jinjing Liang & Hang Li & Xi Shen & Richeng Yu & Wenhong Wang, 2022. "Chirality flips of skyrmion bubbles," Nature Communications, Nature, vol. 13(1), pages 1-7, December.
    19. Hao Zhang & Zhentao Wang & David Dahlbom & Kipton Barros & Cristian D. Batista, 2023. "CP2 skyrmions and skyrmion crystals in realistic quantum magnets," Nature Communications, Nature, vol. 14(1), pages 1-7, December.
    20. Mengfan Guo & Erxiang Xu & Houbing Huang & Changqing Guo & Hetian Chen & Shulin Chen & Shan He & Le Zhou & Jing Ma & Zhonghui Shen & Ben Xu & Di Yi & Peng Gao & Ce-Wen Nan & Neil. D. Mathur & Yang She, 2024. "Electrically and mechanically driven rotation of polar spirals in a relaxor ferroelectric polymer," Nature Communications, Nature, vol. 15(1), pages 1-9, December.

    More about this item

    Statistics

    Access and download statistics

    Corrections

    All material on this site has been provided by the respective publishers and authors. You can help correct errors and omissions. When requesting a correction, please mention this item's handle: RePEc:nat:natcom:v:14:y:2023:i:1:d:10.1038_s41467-023-43853-4. See general information about how to correct material in RePEc.

    If you have authored this item and are not yet registered with RePEc, we encourage you to do it here. This allows to link your profile to this item. It also allows you to accept potential citations to this item that we are uncertain about.

    If CitEc recognized a bibliographic reference but did not link an item in RePEc to it, you can help with this form .

    If you know of missing items citing this one, you can help us creating those links by adding the relevant references in the same way as above, for each refering item. If you are a registered author of this item, you may also want to check the "citations" tab in your RePEc Author Service profile, as there may be some citations waiting for confirmation.

    For technical questions regarding this item, or to correct its authors, title, abstract, bibliographic or download information, contact: Sonal Shukla or Springer Nature Abstracting and Indexing (email available below). General contact details of provider: http://www.nature.com .

    Please note that corrections may take a couple of weeks to filter through the various RePEc services.

    IDEAS is a RePEc service. RePEc uses bibliographic data supplied by the respective publishers.