IDEAS home Printed from https://ideas.repec.org/a/nat/natcom/v15y2024i1d10.1038_s41467-024-51631-z.html
   My bibliography  Save this article

Nematic Ising superconductivity with hidden magnetism in few-layer 6R-TaS2

Author

Listed:
  • Shao-Bo Liu

    (Peking University)

  • Congkuan Tian

    (Peking University
    Beijing Academy of Quantum Information Sciences)

  • Yuqiang Fang

    (Shanghai Jiao Tong University)

  • Hongtao Rong

    (Southern University of Science and Technology)

  • Lu Cao

    (University of Chinese Academy of Sciences)

  • Xinjian Wei

    (Beijing Academy of Quantum Information Sciences)

  • Hang Cui

    (Peking University)

  • Mantang Chen

    (Peking University)

  • Di Chen

    (Beijing Academy of Quantum Information Sciences)

  • Yuanjun Song

    (Beijing Academy of Quantum Information Sciences)

  • Jian Cui

    (Beijing Academy of Quantum Information Sciences)

  • Jiankun Li

    (Beijing Academy of Quantum Information Sciences)

  • Shuyue Guan

    (Peking University)

  • Shuang Jia

    (Peking University)

  • Chaoyu Chen

    (Southern University of Science and Technology)

  • Wenyu He

    (ShanghaiTech University)

  • Fuqiang Huang

    (Shanghai Jiao Tong University)

  • Yuhang Jiang

    (University of Chinese Academy of Sciences)

  • Jinhai Mao

    (University of Chinese Academy of Sciences)

  • X. C. Xie

    (Peking University
    Fudan University
    Hefei National Laboratory)

  • Kam Tuen Law

    (Hong Kong University of Science and Technology)

  • Jian-Hao Chen

    (Peking University
    Beijing Academy of Quantum Information Sciences
    Hefei National Laboratory
    Peking University)

Abstract

In van der Waals heterostructures (vdWHs), the manipulation of interlayer stacking/coupling allows for the construction of customizable quantum systems exhibiting exotic physics. An illustrative example is the diverse range of states of matter achieved through varying the proximity coupling between two-dimensional (2D) quantum spin liquid (QSL) and superconductors within the TaS2 family. This study presents a demonstration of the intertwined physics of spontaneous rotational symmetry breaking, hidden magnetism, and Ising superconductivity (SC) in the three-fold rotationally symmetric, non-magnetic natural vdWHs 6R-TaS2. A distinctive phase emerges in 6R-TaS2 below a characteristic temperature (T*) of approximately 30 K, which is characterized by a remarkable set of features, including a giant extrinsic anomalous Hall effect (AHE), Kondo screening, magnetic field-tunable thermal hysteresis, and nematic magneto-resistance. At lower temperatures, a coexistence of nematicity and Kondo screening with Ising superconductivity is observed, providing compelling evidence of hidden magnetism within a superconductor. This research not only sheds light on unexpected emergent physics resulting from the coupling of itinerant electrons and localized/correlated electrons in natural vdWHs but also emphasizes the potential for tailoring exotic quantum states through the manipulation of interlayer interactions.

Suggested Citation

  • Shao-Bo Liu & Congkuan Tian & Yuqiang Fang & Hongtao Rong & Lu Cao & Xinjian Wei & Hang Cui & Mantang Chen & Di Chen & Yuanjun Song & Jian Cui & Jiankun Li & Shuyue Guan & Shuang Jia & Chaoyu Chen & W, 2024. "Nematic Ising superconductivity with hidden magnetism in few-layer 6R-TaS2," Nature Communications, Nature, vol. 15(1), pages 1-8, December.
    • Handle: RePEc:nat:natcom:v:15:y:2024:i:1:d:10.1038_s41467-024-51631-z
    DOI: 10.1038/s41467-024-51631-z
    as

    Download full text from publisher

    File URL: https://www.nature.com/articles/s41467-024-51631-z
    File Function: Abstract
    Download Restriction: no
    File URL: https://libkey.io/10.1038/s41467-024-51631-z?utm_source=ideas
    LibKey link: if access is restricted and if your library uses this service, LibKey will redirect you to where you can use your library subscription to access this item
    ---><---

    References listed on IDEAS

    as
    1. Y. G. Liang & S. Lee & H. S. Yu & H. R. Zhang & Y. J. Liang & P. Y. Zavalij & X. Chen & R. D. James & L. A. Bendersky & A. V. Davydov & X. H. Zhang & I. Takeuchi, 2020. "Tuning the hysteresis of a metal-insulator transition via lattice compatibility," Nature Communications, Nature, vol. 11(1), pages 1-8, December.
    2. I. Silber & S. Mathimalar & I. Mangel & A. K. Nayak & O. Green & N. Avraham & H. Beidenkopf & I. Feldman & A. Kanigel & A. Klein & M. Goldstein & A. Banerjee & E. Sela & Y. Dagan, 2024. "Two-component nematic superconductivity in 4Hb-TaS2," Nature Communications, Nature, vol. 15(1), pages 1-6, December.
    3. Yukako Fujishiro & Naoya Kanazawa & Ryosuke Kurihara & Hiroaki Ishizuka & Tomohiro Hori & Fehmi Sami Yasin & Xiuzhen Yu & Atsushi Tsukazaki & Masakazu Ichikawa & Masashi Kawasaki & Naoto Nagaosa & Mas, 2021. "Giant anomalous Hall effect from spin-chirality scattering in a chiral magnet," Nature Communications, Nature, vol. 12(1), pages 1-6, December.
    4. Chunyu Guo & Carsten Putzke & Sofia Konyzheva & Xiangwei Huang & Martin Gutierrez-Amigo & Ion Errea & Dong Chen & Maia G. Vergniory & Claudia Felser & Mark H. Fischer & Titus Neupert & Philip J. W. Mo, 2022. "Switchable chiral transport in charge-ordered kagome metal CsV3Sb5," Nature, Nature, vol. 611(7936), pages 461-466, November.
    5. Zhong Wan & Gang Qiu & Huaying Ren & Qi Qian & Yaochen Li & Dong Xu & Jingyuan Zhou & Jingxuan Zhou & Boxuan Zhou & Laiyuan Wang & Ting-Hsun Yang & Zdeněk Sofer & Yu Huang & Kang L. Wang & Xiangfeng D, 2024. "Unconventional superconductivity in chiral molecule–TaS2 hybrid superlattices," Nature, Nature, vol. 632(8023), pages 69-74, August.
    6. Sergio C. Barrera & Michael R. Sinko & Devashish P. Gopalan & Nikhil Sivadas & Kyle L. Seyler & Kenji Watanabe & Takashi Taniguchi & Adam W. Tsen & Xiaodong Xu & Di Xiao & Benjamin M. Hunt, 2018. "Tuning Ising superconductivity with layer and spin–orbit coupling in two-dimensional transition-metal dichalcogenides," Nature Communications, Nature, vol. 9(1), pages 1-8, December.
    7. Yo Machida & Satoru Nakatsuji & Shigeki Onoda & Takashi Tayama & Toshiro Sakakibara, 2010. "Time-reversal symmetry breaking and spontaneous Hall effect without magnetic dipole order," Nature, Nature, vol. 463(7278), pages 210-213, January.
    8. Z. Guguchia & D. J. Gawryluk & S. Shin & Z. Hao & C. Mielke III & D. Das & I. Plokhikh & L. Liborio & J. Kane Shenton & Y. Hu & V. Sazgari & M. Medarde & H. Deng & Y. Cai & C. Chen & Y. Jiang & A. Ama, 2023. "Hidden magnetism uncovered in a charge ordered bilayer kagome material ScV6Sn6," Nature Communications, Nature, vol. 14(1), pages 1-8, December.
    9. Eylon Persky & Anders V. Bjørlig & Irena Feldman & Avior Almoalem & Ehud Altman & Erez Berg & Itamar Kimchi & Jonathan Ruhman & Amit Kanigel & Beena Kalisky, 2022. "Magnetic memory and spontaneous vortices in a van der Waals superconductor," Nature, Nature, vol. 607(7920), pages 692-696, July.
    Full references (including those not matched with items on IDEAS)

    Most related items

    These are the items that most often cite the same works as this one and are cited by the same works as this one.
    1. Avior Almoalem & Irena Feldman & Ilay Mangel & Michael Shlafman & Yuval E. Yaish & Mark H. Fischer & Michael Moshe & Jonathan Ruhman & Amit Kanigel, 2024. "The observation of π-shifts in the Little-Parks effect in 4Hb-TaS2," Nature Communications, Nature, vol. 15(1), pages 1-8, December.
    2. Robin Guehne & Jonathan Noky & Changjiang Yi & Chandra Shekhar & Maia G. Vergniory & Michael Baenitz & Claudia Felser, 2024. "Orbital selective commensurate modulations of the local density of states in ScV6Sn6 probed by nuclear spins," Nature Communications, Nature, vol. 15(1), pages 1-10, December.
    3. J. N. Graham & C. Mielke III & D. Das & T. Morresi & V. Sazgari & A. Suter & T. Prokscha & H. Deng & R. Khasanov & S. D. Wilson & A. C. Salinas & M. M. Martins & Y. Zhong & K. Okazaki & Z. Wang & M. Z, 2024. "Depth-dependent study of time-reversal symmetry-breaking in the kagome superconductor AV3Sb5," Nature Communications, Nature, vol. 15(1), pages 1-9, December.
    4. Yong Hu & Junzhang Ma & Yinxiang Li & Yuxiao Jiang & Dariusz Jakub Gawryluk & Tianchen Hu & Jérémie Teyssier & Volodymyr Multian & Zhouyi Yin & Shuxiang Xu & Soohyeon Shin & Igor Plokhikh & Xinloong H, 2024. "Phonon promoted charge density wave in topological kagome metal ScV6Sn6," Nature Communications, Nature, vol. 15(1), pages 1-9, December.
    5. Hang Chi & Yunbo Ou & Tim B. Eldred & Wenpei Gao & Sohee Kwon & Joseph Murray & Michael Dreyer & Robert E. Butera & Alexandre C. Foucher & Haile Ambaye & Jong Keum & Alice T. Greenberg & Yuhang Liu & , 2023. "Strain-tunable Berry curvature in quasi-two-dimensional chromium telluride," Nature Communications, Nature, vol. 14(1), pages 1-8, December.
    6. Junlin Xiong & Jiao Xie & Bin Cheng & Yudi Dai & Xinyu Cui & Lizheng Wang & Zenglin Liu & Ji Zhou & Naizhou Wang & Xianghan Xu & Xianhui Chen & Sang-Wook Cheong & Shi-Jun Liang & Feng Miao, 2024. "Electrical switching of Ising-superconducting nonreciprocity for quantum neuronal transistor," Nature Communications, Nature, vol. 15(1), pages 1-10, December.
    7. Yi-Hong Gao & Dong-Hui Wang & Feng-Xia Hu & Qing-Zhen Huang & You-Ting Song & Shuai-Kang Yuan & Zheng-Ying Tian & Bing-Jie Wang & Zi-Bing Yu & Hou-Bo Zhou & Yue Kan & Yuan Lin & Jing Wang & Yun-liang , 2024. "Low pressure reversibly driving colossal barocaloric effect in two-dimensional vdW alkylammonium halides," Nature Communications, Nature, vol. 15(1), pages 1-13, December.
    8. E. S. Bozin & M. Abeykoon & S. Conradson & G. Baldinozzi & P. Sutar & D. Mihailovic, 2023. "Crystallization of polarons through charge and spin ordering transitions in 1T-TaS2," Nature Communications, Nature, vol. 14(1), pages 1-9, December.
    9. I. Silber & S. Mathimalar & I. Mangel & A. K. Nayak & O. Green & N. Avraham & H. Beidenkopf & I. Feldman & A. Kanigel & A. Klein & M. Goldstein & A. Banerjee & E. Sela & Y. Dagan, 2024. "Two-component nematic superconductivity in 4Hb-TaS2," Nature Communications, Nature, vol. 15(1), pages 1-6, December.
    10. Xinjian Wei & Congkuan Tian & Hang Cui & Yuxin Zhai & Yongkai Li & Shaobo Liu & Yuanjun Song & Ya Feng & Miaoling Huang & Zhiwei Wang & Yi Liu & Qihua Xiong & Yugui Yao & X. C. Xie & Jian-Hao Chen, 2024. "Three-dimensional hidden phase probed by in-plane magnetotransport in kagome metal CsV3Sb5 thin flakes," Nature Communications, Nature, vol. 15(1), pages 1-8, December.
    11. Chenli Huang & Rong Sun & Lipiao Bao & Xinyue Tian & Changwang Pan & Mengyang Li & Wangqiang Shen & Kun Guo & Bingwu Wang & Xing Lu & Song Gao, 2023. "A hard molecular nanomagnet from confined paramagnetic 3d-4f spins inside a fullerene cage," Nature Communications, Nature, vol. 14(1), pages 1-8, December.
    12. Asish K. Kundu & Xiong Huang & Eric Seewald & Ethan Ritz & Santanu Pakhira & Shuai Zhang & Dihao Sun & Simon Turkel & Sara Shabani & Turgut Yilmaz & Elio Vescovo & Cory R. Dean & David C. Johnston & T, 2024. "Low-energy electronic structure in the unconventional charge-ordered state of ScV6Sn6," Nature Communications, Nature, vol. 15(1), pages 1-9, December.
    13. Meng Wang & Katsuhiro Tanaka & Shiro Sakai & Ziqian Wang & Ke Deng & Yingjie Lyu & Cong Li & Di Tian & Shengchun Shen & Naoki Ogawa & Naoya Kanazawa & Pu Yu & Ryotaro Arita & Fumitaka Kagawa, 2023. "Emergent zero-field anomalous Hall effect in a reconstructed rutile antiferromagnetic metal," Nature Communications, Nature, vol. 14(1), pages 1-8, December.
    14. Y. Hayashi & Y. Okamura & N. Kanazawa & T. Yu & T. Koretsune & R. Arita & A. Tsukazaki & M. Ichikawa & M. Kawasaki & Y. Tokura & Y. Takahashi, 2021. "Magneto-optical spectroscopy on Weyl nodes for anomalous and topological Hall effects in chiral MnGe," Nature Communications, Nature, vol. 12(1), pages 1-7, December.
    15. Georgy A. Ermolaev & Kirill V. Voronin & Adilet N. Toksumakov & Dmitriy V. Grudinin & Ilia M. Fradkin & Arslan Mazitov & Aleksandr S. Slavich & Mikhail K. Tatmyshevskiy & Dmitry I. Yakubovsky & Valent, 2024. "Wandering principal optical axes in van der Waals triclinic materials," Nature Communications, Nature, vol. 15(1), pages 1-8, December.
    16. Alexander Jarjour & G. M. Ferguson & Brian T. Schaefer & Menyoung Lee & Yen Lee Loh & Nandini Trivedi & Katja C. Nowack, 2023. "Superfluid response of an atomically thin gate-tuned van der Waals superconductor," Nature Communications, Nature, vol. 14(1), pages 1-8, December.
    17. Cong Li & Jianfeng Zhang & Yang Wang & Hongxiong Liu & Qinda Guo & Emile Rienks & Wanyu Chen & Francois Bertran & Huancheng Yang & Dibya Phuyal & Hanna Fedderwitz & Balasubramanian Thiagarajan & Macie, 2023. "Emergence of Weyl fermions by ferrimagnetism in a noncentrosymmetric magnetic Weyl semimetal," Nature Communications, Nature, vol. 14(1), pages 1-8, December.
    18. A. Korshunov & H. Hu & D. Subires & Y. Jiang & D. Călugăru & X. Feng & A. Rajapitamahuni & C. Yi & S. Roychowdhury & M. G. Vergniory & J. Strempfer & C. Shekhar & E. Vescovo & D. Chernyshov & A. H. Sa, 2023. "Softening of a flat phonon mode in the kagome ScV6Sn6," Nature Communications, Nature, vol. 14(1), pages 1-8, December.
    19. Jiangang Yang & Xinwei Yi & Zhen Zhao & Yuyang Xie & Taimin Miao & Hailan Luo & Hao Chen & Bo Liang & Wenpei Zhu & Yuhan Ye & Jing-Yang You & Bo Gu & Shenjin Zhang & Fengfeng Zhang & Feng Yang & Zhimi, 2023. "Observation of flat band, Dirac nodal lines and topological surface states in Kagome superconductor CsTi3Bi5," Nature Communications, Nature, vol. 14(1), pages 1-8, December.
    20. Z. Guguchia & D. J. Gawryluk & S. Shin & Z. Hao & C. Mielke III & D. Das & I. Plokhikh & L. Liborio & J. Kane Shenton & Y. Hu & V. Sazgari & M. Medarde & H. Deng & Y. Cai & C. Chen & Y. Jiang & A. Ama, 2023. "Hidden magnetism uncovered in a charge ordered bilayer kagome material ScV6Sn6," Nature Communications, Nature, vol. 14(1), pages 1-8, December.

    More about this item

    Statistics

    Access and download statistics

    Corrections

    All material on this site has been provided by the respective publishers and authors. You can help correct errors and omissions. When requesting a correction, please mention this item's handle: RePEc:nat:natcom:v:15:y:2024:i:1:d:10.1038_s41467-024-51631-z. See general information about how to correct material in RePEc.

    If you have authored this item and are not yet registered with RePEc, we encourage you to do it here. This allows to link your profile to this item. It also allows you to accept potential citations to this item that we are uncertain about.

    If CitEc recognized a bibliographic reference but did not link an item in RePEc to it, you can help with this form .

    If you know of missing items citing this one, you can help us creating those links by adding the relevant references in the same way as above, for each refering item. If you are a registered author of this item, you may also want to check the "citations" tab in your RePEc Author Service profile, as there may be some citations waiting for confirmation.

    For technical questions regarding this item, or to correct its authors, title, abstract, bibliographic or download information, contact: Sonal Shukla or Springer Nature Abstracting and Indexing (email available below). General contact details of provider: http://www.nature.com .

    Please note that corrections may take a couple of weeks to filter through the various RePEc services.

    IDEAS is a RePEc service. RePEc uses bibliographic data supplied by the respective publishers.