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Highly-durable optofluidic microreactor for photocatalytic water splitting

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  • Chen, Rong
  • Li, Lin
  • Zhu, Xun
  • Wang, Hong
  • Liao, Qiang
  • Zhang, Mu-Xing

Abstract

PDMS (Polydimethylsiloxane) is a typical material used to fabricate optofluidic microreactors for photocatalytic water splitting application. However, conventional direct catalyst coating methods are unable to load catalysts firmly and uniformly on the PDMS substrate, which results in weak bond between the catalysts and substrate and thus poor durability and performance. To resolve this problem, a new casting-transfer method was proposed for loading catalysts on the PDMS substrate to fabricate the optofluidic microreactor in this work. By performing the tape testing and long-term testing, it was shown that the optofluidic microreactor fabricated by the new method exhibited critically high durability as compared to the conventional one. The hydrogen production rate was also higher than the conventionally fabricated microreactor. In addition, it was found that the optofluidic microreactor with the micro-grooved structure yielded higher hydrogen production rate than did the conventional planar optofluidic microreactor as a result of enhanced mass transport and reaction area. This method creates a new avenue to fabricate the PDMS based microreactors with high durability.

Suggested Citation

  • Chen, Rong & Li, Lin & Zhu, Xun & Wang, Hong & Liao, Qiang & Zhang, Mu-Xing, 2015. "Highly-durable optofluidic microreactor for photocatalytic water splitting," Energy, Elsevier, vol. 83(C), pages 797-804.
    • Handle: RePEc:eee:energy:v:83:y:2015:i:c:p:797-804
    DOI: 10.1016/j.energy.2015.02.097
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    References listed on IDEAS

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    1. Rossi, Federico & Nicolini, Andrea, 2012. "An experimental investigation to improve the hydrogen production by water photoelectrolysis when cyanin-chloride is used as sensibilizer," Applied Energy, Elsevier, vol. 97(C), pages 763-770.
    2. Ni, Meng & Leung, Michael K.H. & Leung, Dennis Y.C. & Sumathy, K., 2007. "A review and recent developments in photocatalytic water-splitting using TiO2 for hydrogen production," Renewable and Sustainable Energy Reviews, Elsevier, vol. 11(3), pages 401-425, April.
    3. Kazuhiko Maeda & Kentaro Teramura & Daling Lu & Tsuyoshi Takata & Nobuo Saito & Yasunobu Inoue & Kazunari Domen, 2006. "Photocatalyst releasing hydrogen from water," Nature, Nature, vol. 440(7082), pages 295-295, March.
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    1. Pala, Laxmi Prasad Rao & Peela, Nageswara Rao, 2022. "Visible light active IrO2/TiO2 films for oxygen evolution from photocatalytic water splitting in an optofluidic planar microreactor," Renewable Energy, Elsevier, vol. 197(C), pages 902-910.

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