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Sacrificial hydrogen production over TiO2-based photocatalysts: Polyols, carboxylic acids, and saccharides

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  • Yasuda, Masahide
  • Matsumoto, Tomoko
  • Yamashita, Toshiaki

Abstract

Photocatalytic generation of H2 from water over titanium dioxide (TiO2) has received a great deal of interest for developing a renewable and clean energy source. It is initiated by charge-separation in TiO2 upon photoexcitation. The electron reduces water to generate H2 while the hole oxidizes hydroxide to generate hydroxyl radicals. However, water-splitting into O2 and H2 is not easy because of the large up-hill reaction and rapid reverse reaction. It is well known that the use of electron-donating sacrificial agents (hole scavengers) remarkably accelerates TiO2-photocatalyzed H2 evolution in which the hydroxyl radical is consumed by the sacrificial agents. Thus, sacrificial H2 production over a TiO2 photocatalyst is a convenient method to generate H2 from biomass and waste. This paper reviews the sacrificial H2 production from polyols, carboxylic acids, and saccharides, focusing on the chemical yield of H2 production.

Suggested Citation

  • Yasuda, Masahide & Matsumoto, Tomoko & Yamashita, Toshiaki, 2018. "Sacrificial hydrogen production over TiO2-based photocatalysts: Polyols, carboxylic acids, and saccharides," Renewable and Sustainable Energy Reviews, Elsevier, vol. 81(P2), pages 1627-1635.
    • Handle: RePEc:eee:rensus:v:81:y:2018:i:p2:p:1627-1635
    DOI: 10.1016/j.rser.2017.05.243
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    References listed on IDEAS

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    1. Ni, Meng & Leung, Michael K.H. & Leung, Dennis Y.C. & Sumathy, K., 2007. "A review and recent developments in photocatalytic water-splitting using TiO2 for hydrogen production," Renewable and Sustainable Energy Reviews, Elsevier, vol. 11(3), pages 401-425, April.
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    3. Balat, Mustafa & Balat, Havva, 2009. "Recent trends in global production and utilization of bio-ethanol fuel," Applied Energy, Elsevier, vol. 86(11), pages 2273-2282, November.
    4. Masahide Yasuda & Ryo Kurogi & Hikaru Tsumagari & Tsutomu Shiragami & Tomoko Matsumoto, 2014. "New Approach to Fuelization of Herbaceous Lignocelluloses through Simultaneous Saccharification and Fermentation Followed by Photocatalytic Reforming," Energies, MDPI, vol. 7(7), pages 1-11, June.
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    1. Lakhera, Sandeep Kumar & Rajan, Aswathy & T.P., Rugma & Bernaurdshaw, Neppolian, 2021. "A review on particulate photocatalytic hydrogen production system: Progress made in achieving high energy conversion efficiency and key challenges ahead," Renewable and Sustainable Energy Reviews, Elsevier, vol. 152(C).
    2. Banerjee, Debarun & Kushwaha, Nidhi & Shetti, Nagaraj P. & Aminabhavi, Tejraj M. & Ahmad, Ejaz, 2022. "Green hydrogen production via photo-reforming of bio-renewable resources," Renewable and Sustainable Energy Reviews, Elsevier, vol. 167(C).

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