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Influence of sewage sludge treatment on pyrolysis and combustion of dry sludge

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  • Folgueras, M.B.
  • Alonso, M.
  • Díaz, R.M.

Abstract

The influence of sewage sludge treatment on its pyrolysis and combustion and the N, S and Cl emissions was studied by thermogravimetry-mass spectrometry in the range 25–800 °C. Two types of sludge were used (L and F). L underwent anaerobic digestion and was treated with organic polyelectrolyte, while F was treated with FeCl3 and lime. The treatment with inorganic additives had a notable influence on the pyrolysis and combustion processes. During F pyrolysis, the most significant effects of CaO/CaCO3 from lime and Fe2O3 from FeCl3 were: 1) Fe2O3 promoted oxidation reactions, and char gasification at around 600 °C; 2) CaO promoted H2 formation at around 480 °C due to its action on water–shift reaction, and the partial SO2 retention by forming CaSO4. During combustion, Fe2O3 exhibited a high catalytic activity on oxidation reactions. Thus, an intense devolatilisation was produced in the range 200–377 °C, this being accompanied by a high formation of CO2, NO2 and Cl2. Also, the formation of SO2/SO3 was promoted, which were retained by CaCO3/CaO at temperatures higher than 377 °C. The nth-order reaction model describes adequately the global reaction that occurs in each stage, except for the second stage of L combustion that was described by the geometrical contraction model.

Suggested Citation

  • Folgueras, M.B. & Alonso, M. & Díaz, R.M., 2013. "Influence of sewage sludge treatment on pyrolysis and combustion of dry sludge," Energy, Elsevier, vol. 55(C), pages 426-435.
    • Handle: RePEc:eee:energy:v:55:y:2013:i:c:p:426-435
    DOI: 10.1016/j.energy.2013.03.063
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    References listed on IDEAS

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    10. Cheng, Shuo & Zhang, Hongtao & Chang, Fengmin & Zhang, Feng & Wang, Kaijun & Qin, Ya & Huang, Tixiao, 2019. "Combustion behavior and thermochemical treatment scheme analysis of oil sludges and oil sludge semicokes," Energy, Elsevier, vol. 167(C), pages 575-587.
    11. Lin, Kuo-Hsiung & Lai, Nina & Zeng, Jun-Yan & Chiang, Hung-Lung, 2020. "Microwave-pyrolysis treatment of biosludge from a chemical industrial wastewater treatment plant for exploring product characteristics and potential energy recovery," Energy, Elsevier, vol. 199(C).
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    13. Ju-Hyoung Park & Min-Ho Jin & Young-Joo Lee & Gyu-Seob Song & Jong Won Choi & Dong-Wook Lee & Young-Chan Choi & Se-Joon Park & Kwang Ho Song & Joeng-Geun Kim, 2019. "Two-in-One Fuel Synthetic Bioethanol-Lignin from Lignocellulose with Sewage Sludge and Its Air Pollutants Reduction Effects," Energies, MDPI, vol. 12(16), pages 1-15, August.
    14. Opatokun, Suraj Adebayo & Strezov, Vladimir & Kan, Tao, 2015. "Product based evaluation of pyrolysis of food waste and its digestate," Energy, Elsevier, vol. 92(P3), pages 349-354.
    15. Gabriele Di Giacomo & Pietro Romano, 2022. "Evolution and Prospects in Managing Sewage Sludge Resulting from Municipal Wastewater Purification," Energies, MDPI, vol. 15(15), pages 1-33, August.
    16. Tang, Siqi & Zheng, Chunmiao & Yan, Feng & Shao, Ningning & Tang, Yuanyuan & Zhang, Zuotai, 2018. "Product characteristics and kinetics of sewage sludge pyrolysis driven by alkaline earth metals," Energy, Elsevier, vol. 153(C), pages 921-932.
    17. Di Liang & Yimin Li & Zhongning Zhou, 2022. "Numerical Study of Thermochemistry and Trace Element Behavior during the Co-Combustion of Coal and Sludge in Boiler," Energies, MDPI, vol. 15(3), pages 1-16, January.
    18. Kim, D. & Hadigheh, S.A., 2024. "Oxidative pyrolysis of biosolid: Air concentration effects on biochar formation and kinetics," Renewable Energy, Elsevier, vol. 224(C).
    19. Luo, Juan & Ma, Rui & Lin, Junhao & Sun, Shichang & Gong, Guojin & Sun, Jiaman & Chen, Yi & Ma, Ning, 2023. "Review of microwave pyrolysis of sludge to produce high quality biogas: Multi-perspectives process optimization and critical issues proposal," Renewable and Sustainable Energy Reviews, Elsevier, vol. 173(C).

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