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Evolution mechanisms of bio-oil from conventional and nitrogen-rich biomass during photo-thermal pyrolysis

Author

Listed:
  • Huang, Dexin
  • Song, Gongxiang
  • Li, Ruochen
  • Han, Hengda
  • He, Limo
  • Jiang, Long
  • Wang, Yi
  • Su, Sheng
  • Hu, Song
  • Xiang, Jun

Abstract

Photo-thermal (PT) pyrolysis has emerged as a promising technique for efficiently converting biomass into high-quality bio-oil. The pyrolysis characteristics of rice straw (RS) and rapeseed cake (RC) were analyzed using a photo-thermal reactor with heating rates of 20, 200 and 500 °C/min and compared with 20 °C/min fixed-bed (FB) pyrolysis at 750 °C. Due to the uneven temperature distribution caused by its limited heating area, fast PT heating significantly increased the presence of high molecular weight components (>650) in the bio-oil. PT pyrolysis of RS exhibited higher phenolic contents compared to FB pyrolysis, whereas RC oil showed enhanced decomposition of fatty acids through ketonization. In terms of N-compounds, PT slow pyrolysis oil contained more nitriles but fewer linear amines/amides than FB, while more cyclic amides were formed under fast PT pyrolysis. Furthermore, the analysis of heavy components revealed that more aromatic compounds with low H/C ratios were produced in fast PT pyrolysis oil. Overall, PT heating exerted dual effects by reducing secondary reactions and synergistically enhancing inner-particle reactions with fast heating. This study provides valuable insights into the mechanism of bio-oil evolution under PT pyrolysis.

Suggested Citation

  • Huang, Dexin & Song, Gongxiang & Li, Ruochen & Han, Hengda & He, Limo & Jiang, Long & Wang, Yi & Su, Sheng & Hu, Song & Xiang, Jun, 2023. "Evolution mechanisms of bio-oil from conventional and nitrogen-rich biomass during photo-thermal pyrolysis," Energy, Elsevier, vol. 282(C).
    • Handle: RePEc:eee:energy:v:282:y:2023:i:c:s0360544223022077
    DOI: 10.1016/j.energy.2023.128813
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    References listed on IDEAS

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