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A deep insight on the correlation between slag viscosity fluctuation and decomposition of sulfur-bearing minerals in the entrained flow gasifier

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  • Shen, Zhongjie
  • Zhou, Jie
  • Liu, Xia
  • Liang, Qinfeng
  • Liu, Haifeng

Abstract

The fluctuation behavior of the coal slag viscosity in an entrained flow gasifier will increase the instability of the slag discharge and cause a blockage issue on the slag hole. The current research work gave a deep insight about the correlation between on the viscosity fluctuating behavior and the decomposition of the sulfur-bearing minerals in the coal slag. The measured viscosity-temperature curves of four coal slags with different sulfur contents showed different fluctuation behavior, ranging from 1200 to 1400 °C. Comparing to the fitting viscosity curve, the viscosity fluctuating difference and frequency increased with the increasing released gas volume, verified with a simulation experiment with malt syrup and argon. The decomposition and reaction of anhydride and CO was found to be critical to cause the bubble formation with the main gas phase of sulfur oxide inside. The capillary number (Ca) of the slag with bubbles was calculated and compared to the relative viscosity. Theoretical analysis showed a reverse tendency between the capillary number and relative viscosity of the slag, meaning the formation and deformation of bubbles during the slag transformation at high temperature and viscosity measurement process would cause the viscosity fluctuating behavior.

Suggested Citation

  • Shen, Zhongjie & Zhou, Jie & Liu, Xia & Liang, Qinfeng & Liu, Haifeng, 2020. "A deep insight on the correlation between slag viscosity fluctuation and decomposition of sulfur-bearing minerals in the entrained flow gasifier," Energy, Elsevier, vol. 196(C).
    • Handle: RePEc:eee:energy:v:196:y:2020:i:c:s0360544220301560
    DOI: 10.1016/j.energy.2020.117049
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    References listed on IDEAS

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    1. Duan, Wenjun & Gao, Yunke & Yu, Qingbo & Wu, Tianwei & Wang, Zhimei, 2019. "Numerical simulation of coal gasification in molten slag: Gas-liquid interaction characteristic," Energy, Elsevier, vol. 183(C), pages 1233-1243.
    2. Lee, Jae Chul & Lee, Hyeon Hui & Joo, Yong Jin & Lee, Chang Ha & Oh, Min, 2014. "Process simulation and thermodynamic analysis of an IGCC (integrated gasification combined cycle) plant with an entrained coal gasifier," Energy, Elsevier, vol. 64(C), pages 58-68.
    3. Vijayaragavan Krishnamoorthy & Sarma V. Pisupati, 2015. "A Critical Review of Mineral Matter Related Issues during Gasification of Coal in Fixed, Fluidized, and Entrained Flow Gasifiers," Energies, MDPI, vol. 8(9), pages 1-34, September.
    4. A. Parmigiani & S. Faroughi & C. Huber & O. Bachmann & Y. Su, 2016. "Bubble accumulation and its role in the evolution of magma reservoirs in the upper crust," Nature, Nature, vol. 532(7600), pages 492-495, April.
    5. Sun, Yongqi & Shen, Hongwei & Wang, Hao & Wang, Xidong & Zhang, Zuotai, 2014. "Experimental investigation and modeling of cooling processes of high temperature slags," Energy, Elsevier, vol. 76(C), pages 761-767.
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